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Biomass carbon aerogels based shape-stable phase change composites with high light-to-thermal efficiency for energy storage

Author

Listed:
  • Wang, Chengjun
  • Liang, Weidong
  • Yang, Yueyue
  • Liu, Fang
  • Sun, Hanxue
  • Zhu, Zhaoqi
  • Li, An

Abstract

The development of high-performance shape-stable phase change materials composites (ss-PCMCs) with enhanced thermal conductivity and high phase change enthalpy is of great importance for thermal energy storage. Herein, we report the creation of novel ss-PCMCs by incorporation of organic PCMs (1-hexadecanamine (HDA) and palmitic acid (PA)) into the biomass carbon aerogels (BCAs refer to sunflower receptacle spongy carbon aerogel (r-CA) and sunflower stem carbon aerogel (s-CA)) through a simple vacuum infusion. Due to their abundant porosity, light weight and high specific surface area, organic PCMs can be spontaneously loaded into BCAs with an ultrahigh loading rate of up to 1988 wt%. The obtained of PCM/BCAs composites show high phase change enthalpy of ranging from 207.9 kJ kg−1 to 271 kJ kg−1, in addition to their excellent thermal stability and recyclability, e.g., their phase change enthalpy nearly remains unchanged even after 50 times of melting/freezing cycles. The PCM/BCAs composites also show an enhanced thermal conductivity. Furthermore, the light-to-thermal conversion efficiency was found to be promising candidates for light-to-thermal energy storage applications on basis of their 75.6% for HDA/r-CA and 67.8% for HDA/s-CA, respectively, making them abundant resource, cost-efficiency, simple and scalable fabrication process.

Suggested Citation

  • Wang, Chengjun & Liang, Weidong & Yang, Yueyue & Liu, Fang & Sun, Hanxue & Zhu, Zhaoqi & Li, An, 2020. "Biomass carbon aerogels based shape-stable phase change composites with high light-to-thermal efficiency for energy storage," Renewable Energy, Elsevier, vol. 153(C), pages 182-192.
    • Handle: RePEc:eee:renene:v:153:y:2020:i:c:p:182-192
    DOI: 10.1016/j.renene.2020.02.008
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    2. Du, Yu & Huang, Haowei & Hu, Xinpeng & Liu, Shuang & Sheng, Xinxin & Li, Xiaolong & Lu, Xiang & Qu, Jinping, 2021. "Melamine foam/polyethylene glycol composite phase change material synergistically modified by polydopamine/MXene with enhanced solar-to-thermal conversion," Renewable Energy, Elsevier, vol. 171(C), pages 1-10.
    3. Cheng, Jiaji & Niu, Shaoshuai & Kang, Moyun & Liu, Yuqi & Zhang, Feng & Qu, Wenjuan & Guan, Yu & Li, Shaoxiang, 2022. "The thermal behavior and flame retardant performance of phase change material microcapsules with modified carbon nanotubes," Energy, Elsevier, vol. 240(C).
    4. Sarı, Ahmet & Hekimoğlu, Gökhan & Karabayır, Yasemin & Sharma, R.K. & Arslanoğlu, Hasan & Gencel, Osman & Tyagi, V.V., 2022. "Capric-stearic acid mixture impregnated carbonized waste sugar beet pulp as leak-resistive composite phase change material with effective thermal conductivity and thermal energy storage performance," Energy, Elsevier, vol. 247(C).
    5. Wang, Linqiang & Liang, Weidong & Wang, Chengjun & Fan, Yukang & Liu, Yi & Xiao, Chaohu & Sun, Hanxue & Zhu, Zhaoqi & Li, An, 2021. "Dodecylamine/Ti3C2-pectin form-stable phase change composites with enhanced light-to-thermal conversion and mechanical properties," Renewable Energy, Elsevier, vol. 176(C), pages 663-674.

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