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A comparative thermodynamic analysis of isothermal and non-isothermal CeO2-based solar thermochemical cycle with methane-driven reduction

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  • Ma, Tianzeng
  • Wang, Lei
  • Chang, Chun
  • Akhatov, Jasurjon S.
  • Fu, Mingkai
  • Li, Xin

Abstract

Induced by promising hydrogen production of CeO2-based solar thermochemical cycle and evident temperature decreasing effect of methane reduction, a moderately high-temperature solar thermochemical ceria-methane cycle is investigated thermodynamically. In this paper, isothermal and non-isothermal solar-to-fuel efficiencies (ηsolar-to-fuel) under different temperatures and reactant ratios are compared carefully. The calculated results indicate that the condition of CH4:CeO2 = 0.5 is favorable for oxygen release, fuel selectivity and methane conversion. The introduction of methane could increase the maximum yield of H2, and more solar energy could be converted to chemical energy as the increase of nH2O:nCeO2. nH2O:nCeO2 = 0.5, Tred = 1400 K and Toxi = 750 K are suggested for the maximum non-isothermal ηsolar-to-fuel of 0.35, which is larger than the maximum isothermal ηsolar-to-fuel of 0.24. The result shows that non-isothermal solar thermochemical ceria-methane cycle is more feasible for fuel production.

Suggested Citation

  • Ma, Tianzeng & Wang, Lei & Chang, Chun & Akhatov, Jasurjon S. & Fu, Mingkai & Li, Xin, 2019. "A comparative thermodynamic analysis of isothermal and non-isothermal CeO2-based solar thermochemical cycle with methane-driven reduction," Renewable Energy, Elsevier, vol. 143(C), pages 915-921.
    • Handle: RePEc:eee:renene:v:143:y:2019:i:c:p:915-921
    DOI: 10.1016/j.renene.2019.05.047
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    References listed on IDEAS

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    1. Fosheim, Jesse R. & Hathaway, Brandon J. & Davidson, Jane H., 2019. "High efficiency solar chemical-looping methane reforming with ceria in a fixed-bed reactor," Energy, Elsevier, vol. 169(C), pages 597-612.
    2. Christopher L. Muhich & Brian D. Ehrhart & Ibraheam Al-Shankiti & Barbara J. Ward & Charles B. Musgrave & Alan W. Weimer, 2016. "A review and perspective of efficient hydrogen generation via solar thermal water splitting," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 5(3), pages 261-287, May.
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    1. Gao, Ke & Liu, Xianglei & Jiang, Zhixing & Zheng, Hangbin & Song, Chao & Wang, Xinrui & Tian, Cheng & Dang, Chunzhuo & Sun, Nan & Xuan, Yimin, 2022. "Direct solar thermochemical CO2 splitting based on Ca- and Al- doped SmMnO3 perovskites: Ultrahigh CO yield within small temperature swing," Renewable Energy, Elsevier, vol. 194(C), pages 482-494.
    2. Mao, Yanpeng & Gao, Yibo & Dong, Wei & Wu, Han & Song, Zhanlong & Zhao, Xiqiang & Sun, Jing & Wang, Wenlong, 2020. "Hydrogen production via a two-step water splitting thermochemical cycle based on metal oxide – A review," Applied Energy, Elsevier, vol. 267(C).

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