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Investigation of the absorption performance and viscosity for CO2 capture process using [Bmim][Gly] promoted MDEA (N-methyldiethanolamine) aqueous solution

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  • Fu, Dong
  • Zhang, Pan

Abstract

The absorption performance of CO2 in 1-butyl-3-methylimidazolium glycinate ([Bmim][Gly]) promoted MDEA (N-methyldiethanolamine) aqueous solution was investigated. The influences of temperature and mass fraction on CO2 solubility were determined. The time dependence of CO2 solubility demonstrated that the absorption rate of CO2 significantly increased when MDEA aqueous solution was promoted by small amount of [Bmim][Gly]. The viscosities of both CO2-unloaded and CO2-loaded MDEA-[Bmim][Gly] aqueous solutions were measured at temperatures ranging from 303.2 K to 323.2 K and calculated by using the Weiland equation. The effects of temperature, mass fraction of MDEA and [Bmim][Gly], and CO2 loading on viscosities were demonstrated on the basis of experiments and calculations. Our work showed that when the mass fraction of [Bmim][Gly] ranged from 0.10 to 0.15 and the total mass fraction of MDEA and [Bmim][Gly] was around 0.5, high absorption rate, large absorption capacity and appropriate viscosity can be simultaneously achieved.

Suggested Citation

  • Fu, Dong & Zhang, Pan, 2015. "Investigation of the absorption performance and viscosity for CO2 capture process using [Bmim][Gly] promoted MDEA (N-methyldiethanolamine) aqueous solution," Energy, Elsevier, vol. 87(C), pages 165-172.
    • Handle: RePEc:eee:energy:v:87:y:2015:i:c:p:165-172
    DOI: 10.1016/j.energy.2015.04.099
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    References listed on IDEAS

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    1. Lynnette A. Blanchard & Dan Hancu & Eric J. Beckman & Joan F. Brennecke, 1999. "Green processing using ionic liquids and CO2," Nature, Nature, vol. 399(6731), pages 28-29, May.
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    1. Fu, Dong & Zhang, Pan & Mi, ChenLu, 2016. "Effects of concentration and viscosity on the absorption of CO2 in [N1111][Gly] promoted MDEA (methyldiethanolamine) aqueous solution," Energy, Elsevier, vol. 101(C), pages 288-295.
    2. Fu, Dong & Zhang, Pan & Wang, LeMeng, 2016. "Absorption performance of CO2 in high concentrated [Bmim][Lys]-MDEA aqueous solution," Energy, Elsevier, vol. 113(C), pages 1-8.
    3. Bikash K. Mondal & Syamalendu S. Bandyopadhyay & Amar N. Samanta, 2017. "Equilibrium solubility measurement and Kent‐Eisenberg modeling of CO 2 absorption in aqueous mixture of N‐methyldiethanolamine and hexamethylenediamine," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 7(1), pages 202-214, February.
    4. Zhang, Pan & Tian, XiangFeng & Fu, Dong, 2018. "CO2 removal in tray tower by using AAILs activated MDEA aqueous solution," Energy, Elsevier, vol. 161(C), pages 1122-1132.
    5. Wang, Rujie & Liu, Shanshan & Wang, Lidong & Li, Qiangwei & Zhang, Shihan & Chen, Bo & Jiang, Lei & Zhang, Yifeng, 2019. "Superior energy-saving splitter in monoethanolamine-based biphasic solvents for CO2 capture from coal-fired flue gas," Applied Energy, Elsevier, vol. 242(C), pages 302-310.

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