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Steam reforming of methane using double-walled reformer tubes containing high-temperature thermal storage Na2CO3/MgO composites for solar fuel production

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  • Gokon, Nobuyuki
  • Nakamura, Shohei
  • Hatamachi, Tsuyoshi
  • Kodama, Tatsuya

Abstract

Double-walled reactor tubes containing thermal storage materials based on the molten carbonate salts—100 wt% Na2CO3 molten salt, 90 wt% Na2CO3/10 wt% MgO and 80 wt% Na2CO3/20 wt% MgO composite materials—were studied for the performances of the reactor during the heat charging mode, while those of methane reforming with steam during heat discharging mode for solar steam reforming. The variations in the temperatures of the catalyst and storage material, methane conversion, duration of reforming for obtaining high levels of methane conversion (>90%), higher heating value (HHV) power of reformed gas and efficiency of the reactor tubes were evaluated for the double-walled reactor tubes and a single-wall reactor tube without the thermal storage. The results for the heat charging mode indicated that the composite thermal storage could successfully store the heat transferred from the exterior wall of the reactor in comparison to the pure molten-salt. The double-walled reactor tubes with the 90 wt% Na2CO3/10 wt% MgO composite material was the most desirable for steam reforming of methane to realize large HHV amounts of reformed gas and higher efficiencies during heat-discharging mode.

Suggested Citation

  • Gokon, Nobuyuki & Nakamura, Shohei & Hatamachi, Tsuyoshi & Kodama, Tatsuya, 2014. "Steam reforming of methane using double-walled reformer tubes containing high-temperature thermal storage Na2CO3/MgO composites for solar fuel production," Energy, Elsevier, vol. 68(C), pages 773-782.
    • Handle: RePEc:eee:energy:v:68:y:2014:i:c:p:773-782
    DOI: 10.1016/j.energy.2014.01.107
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    3. Fukahori, Ryo & Nomura, Takahiro & Zhu, Chunyu & Sheng, Nan & Okinaka, Noriyuki & Akiyama, Tomohiro, 2016. "Macro-encapsulation of metallic phase change material using cylindrical-type ceramic containers for high-temperature thermal energy storage," Applied Energy, Elsevier, vol. 170(C), pages 324-328.
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    5. Haiming Long & Yunkun Lu & Liang Chang & Haifeng Zhang & Jingcen Zhang & Gaoqun Zhang & Junjie Hao, 2022. "Molecular Dynamics Simulation of Thermophysical Properties and the Microstructure of Na 2 CO 3 Heat Storage Materials," Energies, MDPI, vol. 15(19), pages 1-13, September.
    6. Nomura, Takahiro & Sheng, Nan & Zhu, Chunyu & Saito, Genki & Hanzaki, Daiki & Hiraki, Takehito & Akiyama, Tomohiro, 2017. "Microencapsulated phase change materials with high heat capacity and high cyclic durability for high-temperature thermal energy storage and transportation," Applied Energy, Elsevier, vol. 188(C), pages 9-18.
    7. Jiang, Dongyue & Yang, Wenming & Tang, Aikun, 2016. "A refractory selective solar absorber for high performance thermochemical steam reforming," Applied Energy, Elsevier, vol. 170(C), pages 286-292.
    8. Jin, Jian & Wang, Hongsheng & Shen, Yili & Shu, Ziyun & Liu, Taixiu & Li, Wenjia, 2023. "Thermodynamic analysis of methane to methanol through a two-step process driven by concentrated solar energy," Energy, Elsevier, vol. 273(C).
    9. Gokon, Nobuyuki & Yamaguchi, Tomoya & Kodama, Tatsuya, 2016. "Cyclic thermal storage/discharge performances of a hypereutectic Cu-Si alloy under vacuum for solar thermochemical process," Energy, Elsevier, vol. 113(C), pages 1099-1108.
    10. Jiang, Feng & Zhang, Lingling & She, Xiaohui & Li, Chuan & Cang, Daqiang & Liu, Xianglei & Xuan, Yimin & Ding, Yulong, 2020. "Skeleton materials for shape-stabilization of high temperature salts based phase change materials: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 119(C).
    11. Gu, Rong & Ding, Jing & Wang, Yarong & Yuan, Qinquan & Wang, Weilong & Lu, Jianfeng, 2019. "Heat transfer and storage performance of steam methane reforming in tubular reactor with focused solar simulator," Applied Energy, Elsevier, vol. 233, pages 789-801.

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