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Modified fly ash, a waste material from the energy industry, as a catalyst for the CO2 reduction to methane

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  • Czuma, Natalia
  • Samojeden, Bogdan
  • Zarębska, Katarzyna
  • Motak, Monika
  • Da Costa, Patrick

Abstract

A novel approach was used as support for synthesis of fly ash derived catalyst from waste fly ashes from the energy sector was used as support in the preparation of Ni-catalysts for CO2 methanation. The catalysts were characterized by XRD, H2 -TPR, CO2 -TPD and N2 low-temperature nitrogen sorption. As a result of application of new approach using a ball-mill mechanical energy, carbon dioxide conversion to methane of 58% was obtained at 350 °C. The conversion long with economical aspects of catalyst preparation, including waste material reuse, leads to highly promising results. The results indicate that the catalyst for the methanation process can be easily obtained by the mechanical activation of waste from the energy sector. The chemical modification is more complicated and does not give significantly better results. This approach to waste transformation is innovative, ecological, and economical. It meets the assumptions of the circular economy concept and allows to reuse of waste materials.

Suggested Citation

  • Czuma, Natalia & Samojeden, Bogdan & Zarębska, Katarzyna & Motak, Monika & Da Costa, Patrick, 2022. "Modified fly ash, a waste material from the energy industry, as a catalyst for the CO2 reduction to methane," Energy, Elsevier, vol. 243(C).
    • Handle: RePEc:eee:energy:v:243:y:2022:i:c:s0360544221029674
    DOI: 10.1016/j.energy.2021.122718
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    References listed on IDEAS

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    1. Arnette, Andrew N., 2017. "Renewable energy and carbon capture and sequestration for a reduced carbon energy plan: An optimization model," Renewable and Sustainable Energy Reviews, Elsevier, vol. 70(C), pages 254-265.
    2. Jack P. C. Kleijnen, 2015. "Response Surface Methodology," International Series in Operations Research & Management Science, in: Michael C Fu (ed.), Handbook of Simulation Optimization, edition 127, chapter 0, pages 81-104, Springer.
    3. Thonemann, Nils, 2020. "Environmental impacts of CO2-based chemical production: A systematic literature review and meta-analysis," Applied Energy, Elsevier, vol. 263(C).
    4. Ghaib, Karim & Ben-Fares, Fatima-Zahrae, 2018. "Power-to-Methane: A state-of-the-art review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 81(P1), pages 433-446.
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    Cited by:

    1. Katarzyna Zarębska & Jakub Szczurowski & Magdalena Gazda-Grzywacz & Wojciech Wróbel & Jakub Bator & Paweł Baran, 2023. "Geopolymer Building Materials Based on Fly Ash in Terms of Removing SO 2 , CO 2 , and Water Vapor," Energies, MDPI, vol. 16(13), pages 1-18, July.

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    Keywords

    Fly ashes; Synthesis; Nickel; CO2 methanation;
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