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Hierarchical porous carbon@PbO1-x composite for high-performance lead-carbon battery towards renewable energy storage

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Listed:
  • Yin, Jian
  • Lin, Nan
  • Lin, ZheQi
  • Wang, Yue
  • Chen, CaiLing
  • Shi, Jun
  • Bao, JinPeng
  • Lin, HaiBo
  • Feng, ShouHua
  • Zhang, WenLi

Abstract

Utility lead-carbon batteries in renewable energy storage applications require fast charge ability and long-term cycling stability, which introduces a fundamental problem that how to improve the electrode kinetics and cycling stability of lead-carbon electrode. Herein, we present an oxygen-deficient PbO decorated rice-husk-based hierarchical porous carbon (RHHPC@PbO1-x) composite as an effective additive of negative electrode in lead-carbon battery. The RHHPC@PbO1-x composite was prepared from a facile sol-gel/annealing method. The obtained RHHPC@PbO1-x composite and the lead-carbon electrode with RHHPC@PbO1-x additives were characterized by various physicochemical methods, such as scanning electron microscopy, transmission electron microscopy, X-ray diffraction, and multiple electrochemical methods. The RHHPC@PbO1-x composite enhances the electrochemical active surface area and strengthens the structural stability of lead-carbon electrode, which improves the electrode kinetics and the cycling stability of lead-carbon negative electrode. As a result, the cycling life of a 2 V/4 Ah valve-regulated lead-carbon battery with RHHPC@PbO1-x composite additives exhibited a lifespan of 900 cycles (triple of the blank battery). Our work gives an insight for interphase and porosity tuning of lead-carbon additives used in lead-carbon battery. Based on the existing mature production facilities of lead-acid battery, it is promising for this RHHPC@PbO1-x additive to be used in commercial lead-carbon batteryies for renewable energy storage.

Suggested Citation

  • Yin, Jian & Lin, Nan & Lin, ZheQi & Wang, Yue & Chen, CaiLing & Shi, Jun & Bao, JinPeng & Lin, HaiBo & Feng, ShouHua & Zhang, WenLi, 2020. "Hierarchical porous carbon@PbO1-x composite for high-performance lead-carbon battery towards renewable energy storage," Energy, Elsevier, vol. 193(C).
    • Handle: RePEc:eee:energy:v:193:y:2020:i:c:s0360544219323709
    DOI: 10.1016/j.energy.2019.116675
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    References listed on IDEAS

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    1. Posada, Jorge Omar Gil & Rennie, Anthony J.R. & Villar, Sofia Perez & Martins, Vitor L. & Marinaccio, Jordan & Barnes, Alistair & Glover, Carol F. & Worsley, David A. & Hall, Peter J., 2017. "Aqueous batteries as grid scale energy storage solutions," Renewable and Sustainable Energy Reviews, Elsevier, vol. 68(P2), pages 1174-1182.
    2. ChunLei Yang & Sven Modell, 2013. "Power and performance," Accounting, Auditing & Accountability Journal, Emerald Group Publishing Limited, vol. 26(1), pages 101-132, January.
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    Cited by:

    1. Wang, Yue & Wu, Jue & Lin, Nan & Liu, Debo & Liu, Zhiqiang & Lin, Haibo, 2023. "Enabling stable cycling performance with rice husk silica positive additive in lead-acid battery," Energy, Elsevier, vol. 269(C).
    2. Jakub Lach & Kamil Wróbel & Justyna Wróbel & Andrzej Czerwiński, 2021. "Applications of Carbon in Rechargeable Electrochemical Power Sources: A Review," Energies, MDPI, vol. 14(9), pages 1-29, May.
    3. Yanamandra, Kaushik & Pinisetty, Dinesh & Gupta, Nikhil, 2023. "Impact of carbon additives on lead-acid battery electrodes: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 173(C).

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