IDEAS home Printed from https://ideas.repec.org/a/eee/energy/v172y2019icp68-78.html
   My bibliography  Save this article

Theoretical simulation of the optimal relation between active material, binder and conductive additive for lithium-ion battery cathodes

Author

Listed:
  • Miranda, D.
  • Gören, A.
  • Costa, C.M.
  • Silva, M.M.
  • Almeida, A.M.
  • Lanceros-Méndez, S.

Abstract

The cathode formulation for lithium-ion batteries has been optimized taking into consideration different active material, polymer binder and conductive additive ratios. Theoretical simulations have been carried out to evaluate the influence of different materials relative contents in the electrode performance, at various discharge rates. Simulations were performed by the finite element method applying the Doyle/Fuller/Newman model for two different active materials (C-LiFePO4 and LiMn2O4) and some results were compared with experimental data. The optimization of the electrode formulation is dependent on the maximum value of n, defined as the ratio polymer binder/conductive additive. The electrical conductivity of the cathode depends on the conductive material, thus it is dependent on the ratio n. The optimum balance of the cathode components is reported considering the performance and the mechanical stability.

Suggested Citation

  • Miranda, D. & Gören, A. & Costa, C.M. & Silva, M.M. & Almeida, A.M. & Lanceros-Méndez, S., 2019. "Theoretical simulation of the optimal relation between active material, binder and conductive additive for lithium-ion battery cathodes," Energy, Elsevier, vol. 172(C), pages 68-78.
    • Handle: RePEc:eee:energy:v:172:y:2019:i:c:p:68-78
    DOI: 10.1016/j.energy.2019.01.122
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S0360544219301306
    Download Restriction: Full text for ScienceDirect subscribers only
    File URL: https://libkey.io/10.1016/j.energy.2019.01.122?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. J.-M. Tarascon & M. Armand, 2001. "Issues and challenges facing rechargeable lithium batteries," Nature, Nature, vol. 414(6861), pages 359-367, November.
    2. Eric C. Evarts, 2015. "Lithium batteries: To the limits of lithium," Nature, Nature, vol. 526(7575), pages 93-95, October.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. João C. Barbosa & Renato Gonçalves & Carlos M. Costa & Senentxu Lanceros-Mendez, 2021. "Recent Advances on Materials for Lithium-Ion Batteries," Energies, MDPI, vol. 14(11), pages 1-36, May.
    2. Shabani, Masoume & Wallin, Fredrik & Dahlquist, Erik & Yan, Jinyue, 2023. "The impact of battery operating management strategies on life cycle cost assessment in real power market for a grid-connected residential battery application," Energy, Elsevier, vol. 270(C).
    3. Gao, Yizhao & Zhu, Chong & Zhang, Xi & Guo, Bangjun, 2021. "Implementation and evaluation of a practical electrochemical- thermal model of lithium-ion batteries for EV battery management system," Energy, Elsevier, vol. 221(C).

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Dong Hou & Zhengrui Xu & Zhijie Yang & Chunguang Kuai & Zhijia Du & Cheng-Jun Sun & Yang Ren & Jue Liu & Xianghui Xiao & Feng Lin, 2022. "Effect of the grain arrangements on the thermal stability of polycrystalline nickel-rich lithium-based battery cathodes," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    2. Mohammadmahdi Ghiji & Vasily Novozhilov & Khalid Moinuddin & Paul Joseph & Ian Burch & Brigitta Suendermann & Grant Gamble, 2020. "A Review of Lithium-Ion Battery Fire Suppression," Energies, MDPI, vol. 13(19), pages 1-30, October.
    3. Zhang, Chao & Wei, Yi-Li & Cao, Peng-Fei & Lin, Meng-Chang, 2018. "Energy storage system: Current studies on batteries and power condition system," Renewable and Sustainable Energy Reviews, Elsevier, vol. 82(P3), pages 3091-3106.
    4. Ziheng Zhang & Maxim Avdeev & Huaican Chen & Wen Yin & Wang Hay Kan & Guang He, 2022. "Lithiated Prussian blue analogues as positive electrode active materials for stable non-aqueous lithium-ion batteries," Nature Communications, Nature, vol. 13(1), pages 1-13, December.
    5. Zhi Chang & Huijun Yang & Xingyu Zhu & Ping He & Haoshen Zhou, 2022. "A stable quasi-solid electrolyte improves the safe operation of highly efficient lithium-metal pouch cells in harsh environments," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    6. Matthew Sadd & Shizhao Xiong & Jacob R. Bowen & Federica Marone & Aleksandar Matic, 2023. "Investigating microstructure evolution of lithium metal during plating and stripping via operando X-ray tomographic microscopy," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    7. Yanjie Yi & Jingshun Zhuang & Chao Liu & Lirong Lei & Shuaiming He & Yi Hou, 2022. "Emerging Lignin-Based Materials in Electrochemical Energy Systems," Energies, MDPI, vol. 15(24), pages 1-22, December.
    8. Jack E. N. Swallow & Michael W. Fraser & Nis-Julian H. Kneusels & Jodie F. Charlton & Christopher G. Sole & Conor M. E. Phelan & Erik Björklund & Peter Bencok & Carlos Escudero & Virginia Pérez-Dieste, 2022. "Revealing solid electrolyte interphase formation through interface-sensitive Operando X-ray absorption spectroscopy," Nature Communications, Nature, vol. 13(1), pages 1-14, December.
    9. Sewon Kim & Ju-Sik Kim & Lincoln Miara & Yan Wang & Sung-Kyun Jung & Seong Yong Park & Zhen Song & Hyungsub Kim & Michael Badding & JaeMyung Chang & Victor Roev & Gabin Yoon & Ryounghee Kim & Jung-Hwa, 2022. "High-energy and durable lithium metal batteries using garnet-type solid electrolytes with tailored lithium-metal compatibility," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    10. Shenxiang Zhang & Xian Wei & Xue Cao & Meiwen Peng & Min Wang & Lin Jiang & Jian Jin, 2024. "Solar-driven membrane separation for direct lithium extraction from artificial salt-lake brine," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    11. Chao Wang & Ming Liu & Michel Thijs & Frans G. B. Ooms & Swapna Ganapathy & Marnix Wagemaker, 2021. "High dielectric barium titanate porous scaffold for efficient Li metal cycling in anode-free cells," Nature Communications, Nature, vol. 12(1), pages 1-11, December.
    12. Ma, Mina & Li, Xiaoyu & Gao, Wei & Sun, Jinhua & Wang, Qingsong & Mi, Chris, 2022. "Multi-fault diagnosis for series-connected lithium-ion battery pack with reconstruction-based contribution based on parallel PCA-KPCA," Applied Energy, Elsevier, vol. 324(C).
    13. Liao, Xiaolin & Sun, Peiyi & Xu, Mengqing & Xing, Lidan & Liao, Youhao & Zhang, Liping & Yu, Le & Fan, Weizhen & Li, Weishan, 2016. "Application of tris(trimethylsilyl)borate to suppress self-discharge of layered nickel cobalt manganese oxide for high energy battery," Applied Energy, Elsevier, vol. 175(C), pages 505-511.
    14. Irina Stenina & Ruslan Shaydullin & Tatiana Kulova & Anna Kuz’mina & Nataliya Tabachkova & Andrey Yaroslavtsev, 2020. "Effect of Carbon Additives on the Electrochemical Performance of Li 4 Ti 5 O 12 /C Anodes," Energies, MDPI, vol. 13(15), pages 1-15, August.
    15. Toyabur Rahman, M. & Sohel Rana, SM & Salauddin, Md. & Maharjan, Pukar & Bhatta, Trilochan & Kim, Hyunsik & Cho, Hyunok & Park, Jae Yeong, 2020. "A highly miniaturized freestanding kinetic-impact-based non-resonant hybridized electromagnetic-triboelectric nanogenerator for human induced vibrations harvesting," Applied Energy, Elsevier, vol. 279(C).
    16. Abdulrahman S. Binfaris & Alexander G. Zestos & Jandro L. Abot, 2023. "Development of Carbon Nanotube Yarn Supercapacitors and Energy Storage for Integrated Structural Health Monitoring," Energies, MDPI, vol. 16(15), pages 1-14, August.
    17. Wang, Zhenpo & Hong, Jichao & Liu, Peng & Zhang, Lei, 2017. "Voltage fault diagnosis and prognosis of battery systems based on entropy and Z-score for electric vehicles," Applied Energy, Elsevier, vol. 196(C), pages 289-302.
    18. Ma, Mina & Wang, Yu & Duan, Qiangling & Wu, Tangqin & Sun, Jinhua & Wang, Qingsong, 2018. "Fault detection of the connection of lithium-ion power batteries in series for electric vehicles based on statistical analysis," Energy, Elsevier, vol. 164(C), pages 745-756.
    19. Lukman Noerochim & Wahyu Caesarendra & Abdulloh Habib & Widyastuti & Suwarno & Yatim Lailun Ni’mah & Achmad Subhan & Bambang Prihandoko & Buyung Kosasih, 2020. "Role of TiO 2 Phase Composition Tuned by LiOH on The Electrochemical Performance of Dual-Phase Li 4 Ti 5 O 12 -TiO 2 Microrod as an Anode for Lithium-Ion Battery," Energies, MDPI, vol. 13(20), pages 1-15, October.
    20. Guo-Rui Zhu & Qin Zhang & Qing-Song Liu & Qi-Yao Bai & Yi-Zhou Quan & You Gao & Gang Wu & Yu-Zhong Wang, 2023. "Non-flammable solvent-free liquid polymer electrolyte for lithium metal batteries," Nature Communications, Nature, vol. 14(1), pages 1-12, December.

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:energy:v:172:y:2019:i:c:p:68-78. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.journals.elsevier.com/energy .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.