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Giant polarization ripple in transverse pyroelectricity

Author

Listed:
  • Yi Zhou

    (National University of Singapore
    Southern University of Science and Technology)

  • Tianpeng Ding

    (National University of Singapore
    University of Electronic Science and Technology of China)

  • Jun Guo

    (National University of Singapore)

  • Guoqiang Xu

    (National University of Singapore)

  • Mingqiang Cheng

    (Southern University of Science and Technology)

  • Chen Zhang

    (National University of Singapore)

  • Xiao-Qiao Wang

    (National University of Singapore)

  • Wanheng Lu

    (National University of Singapore)

  • Wei Li Ong

    (National University of Singapore)

  • Jiangyu Li

    (Southern University of Science and Technology)

  • Jiaqing He

    (Southern University of Science and Technology)

  • Cheng-Wei Qiu

    (National University of Singapore)

  • Ghim Wei Ho

    (National University of Singapore
    National University of Singapore
    A*STAR (Agency for Science, Technology and Research))

Abstract

Pyroelectricity originates from spontaneous polarization variation, promising in omnipresent non-static thermodynamic energy harvesting. Particularly, changing spontaneous polarization via out-of-plane uniform heat perturbations has been shown in solar pyroelectrics. However, these approaches present unequivocal inefficiency due to spatially coupled low temperature change and duration along the longitudinal direction. Here we demonstrate unconventional giant polarization ripples in transverse pyroelectrics, without increasing the total energy input, into electricity with an efficiency of 5-fold of conventional longitudinal counterparts. The non-uniform graded temperature variation arises from decoupled heat localization and propagation, leading to anomalous in-plane heat perturbation (29-fold) and enhanced thermal disequilibrium effects. This in turn triggers an augmented polarization ripple, fundamentally enabling unprecedented electricity generation performance. Notably, the device generates a power density of 38 mW m−2 at 1 sun illumination, which is competitive with solar thermoelectrics and ferrophotovoltaics. Our findings provide a viable paradigm, not only for universal practical pyroelectric heat harvesting but for flexible manipulation of transverse heat transfer towards sustainable energy harvesting and management.

Suggested Citation

  • Yi Zhou & Tianpeng Ding & Jun Guo & Guoqiang Xu & Mingqiang Cheng & Chen Zhang & Xiao-Qiao Wang & Wanheng Lu & Wei Li Ong & Jiangyu Li & Jiaqing He & Cheng-Wei Qiu & Ghim Wei Ho, 2023. "Giant polarization ripple in transverse pyroelectricity," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-35900-x
    DOI: 10.1038/s41467-023-35900-x
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    References listed on IDEAS

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    Cited by:

    1. Kailun Zou & Peijia Bai & Kanghua Li & Fangyuan Luo & Jiajie Liang & Ling Lin & Rujun Ma & Qi Li & Shenglin Jiang & Qing Wang & Guangzu Zhang, 2024. "Electronic cooling and energy harvesting using ferroelectric polymer composites," Nature Communications, Nature, vol. 15(1), pages 1-10, December.

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