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Mass Transfer Performance Study for CO 2 Absorption into Non-Precipitated Potassium Carbonate Promoted with Glycine Using Packed Absorption Column

Author

Listed:
  • Nur Farhana Ajua Mustafa

    (CO2 Research Centre (CO2RES), Institute of Contaminant Management, Chemical Engineering Department, Universiti Teknologi PETRONAS, Seri Iskandar 32610, Perak, Malaysia)

  • Azmi Mohd Shariff

    (CO2 Research Centre (CO2RES), Institute of Contaminant Management, Chemical Engineering Department, Universiti Teknologi PETRONAS, Seri Iskandar 32610, Perak, Malaysia)

  • Wee Horng Tay

    (CO2 Research Centre (CO2RES), Institute of Contaminant Management, Chemical Engineering Department, Universiti Teknologi PETRONAS, Seri Iskandar 32610, Perak, Malaysia)

  • Hairul Nazirah Abdul Halim

    (School of Bioprocess Engineering, Universiti Malaysia Perlis, Kompleks Pengajian Jejawi 3, Arau 02600, Perlis, Malaysia
    Center of Excellent for Biomass Utilization, Universiti Malaysia Perlis, Arau 02600, Perlis, Malaysia)

  • Siti Munirah Mhd Yusof

    (CO2 Research Centre (CO2RES), Institute of Contaminant Management, Chemical Engineering Department, Universiti Teknologi PETRONAS, Seri Iskandar 32610, Perak, Malaysia)

Abstract

The removal of carbon dioxide (CO 2 ) at offshore operation requires an absorption system with an environmentally friendly solvent that can operate at elevated pressure. Potassium carbonate promoted with glycine, PCGLY, is a green solvent that has potential for offshore applications. For high solvent concentrations at elevated pressure, the by-product of CO 2 absorption consists of precipitates that increase operational difficulty. Therefore, this study was done to assess the CO 2 absorption performance of non-precipitated PCGLY with concentration 15wt%PC+3wt%GLY, which is known to have comparable solubility performance with MDEA. A packed absorption column was used to identify the CO 2 removal efficiency, mass transfer coefficient in liquid film, k l a e , and overall volumetric mass transfer coefficient, K G a v . A simplified rate-based model was used to determine k l a e and K G a v based on the experimental data with a maximum MAE value, 0.057. The results showed that liquid flow rates and liquid temperature gives significant effects on the k l a e and K G a v profile, whereas gas flow rate and operating pressure had little effect. The CO 2 removal efficiency of PCGLY was found to be 77%, which was only 2% lower than 1.2 kmol/m 3 MDEA. K G a v of PCGLY is comparable with MDEA. The absorption process using PCGLY shows potential in the CO 2 sweetening process at offshore.

Suggested Citation

  • Nur Farhana Ajua Mustafa & Azmi Mohd Shariff & Wee Horng Tay & Hairul Nazirah Abdul Halim & Siti Munirah Mhd Yusof, 2020. "Mass Transfer Performance Study for CO 2 Absorption into Non-Precipitated Potassium Carbonate Promoted with Glycine Using Packed Absorption Column," Sustainability, MDPI, vol. 12(9), pages 1-17, May.
    • Handle: RePEc:gam:jsusta:v:12:y:2020:i:9:p:3873-:d:355899
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    References listed on IDEAS

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