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The influence of Ni loading on coke formation in steam reforming of acetic acid

Author

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  • An, Lu
  • Dong, Changqing
  • Yang, Yongping
  • Zhang, Junjiao
  • He, Lei

Abstract

Steam reforming of acetic acid on Ni/γ-Al2O3 with different nickel loading for hydrogen production was investigated in a tubular reactor at 600 °C, 1 atm, H2O/HAc = 4, and WHSV = 5.01 g-acetic acid/g-cata.h−1. The catalysts were characterized by temperature programmed oxidation (TPO) and differential thermal analysis (DTA), X-ray photoelectron spectroscopy (XPS) and transmission electron microscopy (TEM). The results showed that the amount of deposited carbidic-like carbon decreased and graphitic-like carbon increased with Ni loading increasing from 9 to 15 wt%. The Ni/γ-Al2O3 catalyst with 12 wt% Ni loading had higher catalytic activity and lower coke deposited rate.

Suggested Citation

  • An, Lu & Dong, Changqing & Yang, Yongping & Zhang, Junjiao & He, Lei, 2011. "The influence of Ni loading on coke formation in steam reforming of acetic acid," Renewable Energy, Elsevier, vol. 36(3), pages 930-935.
    • Handle: RePEc:eee:renene:v:36:y:2011:i:3:p:930-935
    DOI: 10.1016/j.renene.2010.08.029
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    Cited by:

    1. Park, Seo Yun & Oh, Gunung & Kim, Kwangyul & Seo, Myung Won & Ra, Ho Won & Mun, Tae Young & Lee, Jae Goo & Yoon, Sang Jun, 2017. "Deactivation characteristics of Ni and Ru catalysts in tar steam reforming," Renewable Energy, Elsevier, vol. 105(C), pages 76-83.
    2. Pravakar Mohanty & Kamal K. Pant & Ritesh Mittal, 2015. "Hydrogen generation from biomass materials: challenges and opportunities," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 4(2), pages 139-155, March.
    3. Pang, Yunji & Wu, Yuting & Chen, Yisheng & Luo, Fuliang & Chen, Junjun, 2020. "Degradation effect of Ce/Al2O3 catalyst on pyrolysis volatility of pine," Renewable Energy, Elsevier, vol. 162(C), pages 134-143.
    4. Resende, K.A. & Ávila-Neto, C.N. & Rabelo-Neto, R.C. & Noronha, F.B. & Hori, C.E., 2015. "Thermodynamic analysis and reaction routes of steam reforming of bio-oil aqueous fraction," Renewable Energy, Elsevier, vol. 80(C), pages 166-176.
    5. Paraskevi Panagiotopoulou & Christina Papadopoulou & Haris Matralis & Xenophon Verykios, 2014. "Production of renewable hydrogen by reformation of biofuels," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 3(3), pages 231-253, May.
    6. Chen, Guanyi & Tao, Junyu & Liu, Caixia & Yan, Beibei & Li, Wanqing & Li, Xiangping, 2017. "Hydrogen production via acetic acid steam reforming: A critical review on catalysts," Renewable and Sustainable Energy Reviews, Elsevier, vol. 79(C), pages 1091-1098.
    7. Ruocco, Concetta & Palma, Vincenzo & Cortese, Marta & Martino, Marco, 2022. "Stability of bimetallic Ni/CeO2–SiO2 catalysts during fuel grade bioethanol reforming in a fluidized bed reactor," Renewable Energy, Elsevier, vol. 182(C), pages 913-922.

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