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Effect of different digestate biochars as promoters via sludge anaerobic digestion on subsequent pyrolysis products: Focusing on the nitrogen, sulfur, and chlorine releasing characteristics

Author

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  • Wu, Yan
  • Yu, Yue
  • Zhu, Ailing
  • Fu, Junjie
  • Xia, Yaping
  • Lan, Guoxing
  • Fu, Chuan
  • Ma, Zhicheng
  • Xue, Jianfu
  • Tao, Lin
  • Xie, Xinrui

Abstract

Anaerobic digestion generates a significant amount of byproduct known as digestate, necessitating resourceful disposal. However, the digestate biochar may exert certain impacts on the pyrolysis of sludge, especially regarding the release of N/S/Cl during the pyrolysis process. This may lead to environmental risks and impose restrictions on the recycling of digestate. There is limited existing research on this topic. In this study, the impact and mechanism of digestate biochar on pyrolysis products were analyzed through kinetic analysis, TG-MS, and Py-GC/MS, with a specific focus on the release characteristics of polluting elements during the pyrolysis process. The findings indicate that the Fe-containing digestate biochar, owing to the larger specific surface area, richer functional groups and catalytic activity associated with Fe3+, enhances the production of C/H/O gases during pyrolysis while reducing the release of NH3, NO2, and H2S. Particularly, Fe-containing digestate biochar significantly enhances the release of Cl-containing gases. The decrease in tar content indicates that Fe-containing digestate biochar promotes the catalytic removal of tar. A comprehensive comparison and analysis of the reaction mechanism were conducted in this study, providing a theoretical basis for the release of pollutants from digestate pyrolysis while enhancing the control and management of pollutants containing N/S/Cl.

Suggested Citation

  • Wu, Yan & Yu, Yue & Zhu, Ailing & Fu, Junjie & Xia, Yaping & Lan, Guoxing & Fu, Chuan & Ma, Zhicheng & Xue, Jianfu & Tao, Lin & Xie, Xinrui, 2024. "Effect of different digestate biochars as promoters via sludge anaerobic digestion on subsequent pyrolysis products: Focusing on the nitrogen, sulfur, and chlorine releasing characteristics," Renewable Energy, Elsevier, vol. 226(C).
    • Handle: RePEc:eee:renene:v:226:y:2024:i:c:s0960148124004312
    DOI: 10.1016/j.renene.2024.120366
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    1. Zhang, Li & Yao, Zonglu & Zhao, Lixin & Li, Zhihe & Yi, Weiming & Kang, Kang & Jia, Jixiu, 2021. "Synthesis and characterization of different activated biochar catalysts for removal of biomass pyrolysis tar," Energy, Elsevier, vol. 232(C).
    2. Raza, Mohsin & Abu-Jdayil, Basim & Al-Marzouqi, Ali H. & Inayat, Abrar, 2022. "Kinetic and thermodynamic analyses of date palm surface fibers pyrolysis using Coats-Redfern method," Renewable Energy, Elsevier, vol. 183(C), pages 67-77.
    3. Ge, Lichao & Zhao, Can & Zuo, Mingjin & Du, Yuying & Yao, Lei & Li, Dongyang & Chu, Huaqiang & Wang, Yang & Xu, Chang, 2023. "Effect of Fe on the pyrolysis products of lignin, cellulose and hemicellulose, and the formation of carbon nanotubes," Renewable Energy, Elsevier, vol. 211(C), pages 13-20.
    4. Ma, Mingyan & Xu, Donghai & Gong, Xuehan & Diao, Yunfei & Feng, Peng & Kapusta, Krzysztof, 2023. "Municipal sewage sludge product recirculation catalytic pyrolysis mechanism from a kinetic perspective," Renewable Energy, Elsevier, vol. 215(C).
    5. Wang, Chengxin & Bi, Haobo & Lin, Qizhao & Jiang, Xuedan & Jiang, Chunlong, 2020. "Co-pyrolysis of sewage sludge and rice husk by TG–FTIR–MS: Pyrolysis behavior, kinetics, and condensable/non-condensable gases characteristics," Renewable Energy, Elsevier, vol. 160(C), pages 1048-1066.
    6. Liu, Zhiyuan & Li, Yan & Sun, Yong & Feng, Fang & Tagawa, Kotaro, 2023. "Preparation of biochar-based photothermal superhydrophobic coating based on corn straw biogas residue and blade anti-icing performance by wind tunnel test," Renewable Energy, Elsevier, vol. 210(C), pages 618-626.
    7. Kor-Bicakci, Gokce & Eskicioglu, Cigdem, 2019. "Recent developments on thermal municipal sludge pretreatment technologies for enhanced anaerobic digestion," Renewable and Sustainable Energy Reviews, Elsevier, vol. 110(C), pages 423-443.
    8. Xing, Xinxin & Zhao, Hongyu & Zhou, Lili & Wang, Yangang & Chen, Haijun & Gao, Ying & Wang, Yinfeng & Zhu, Yuezhao, 2022. "Pyrolysis kinetics, thermodynamics of PTA sludge and product characterization of cyclic in-situ catalytic pyrolysis by using recycled char as a catalyst," Energy, Elsevier, vol. 251(C).
    9. Xia, Sunwen & Yang, Haiping & Lei, shuaishuai & Lu, Wang & Cai, Ning & Xiao, Haoyu & Chen, Yingquan & Chen, Hanping, 2023. "Iron salt catalytic pyrolysis of biomass: Influence of iron salt type," Energy, Elsevier, vol. 262(PA).
    10. Chen, Renjie & Yuan, Shijie & Wang, Xiankai & Dai, Xiaohu & Guo, Yali & Li, Chong & Wu, Haibin & Dong, Bin, 2023. "Mechanistic insight into the effect of hydrothermal treatment of sewage sludge on subsequent pyrolysis: Evolution of volatile and their interaction with pyrolysis kinetic and products compositions," Energy, Elsevier, vol. 266(C).
    11. Escalante, Jamin & Chen, Wei-Hsin & Tabatabaei, Meisam & Hoang, Anh Tuan & Kwon, Eilhann E. & Andrew Lin, Kun-Yi & Saravanakumar, Ayyadurai, 2022. "Pyrolysis of lignocellulosic, algal, plastic, and other biomass wastes for biofuel production and circular bioeconomy: A review of thermogravimetric analysis (TGA) approach," Renewable and Sustainable Energy Reviews, Elsevier, vol. 169(C).
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