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Efficient and stable SiO2-encapsulated NiPt/HY catalyst for catalytic cracking of β-O-4 linkage compound

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  • Song, Wenjing
  • Song, Mengxue
  • Cai, Wenqing
  • Li, Weichu
  • Jiang, Xingmao
  • Fang, Weiping
  • Lai, Weikun

Abstract

Development of highly active and stable catalyst for C–O bonds cracking is important in biomass conversion, in this work, we report a SiO2-encapsulated NiPt/HY core-shell catalyst for phenethoxybenzene (PEB) catalytic cracking. The as-grown silica shell with defined pores serves as a ‘storage’ to enhance local concentration of PEB and intermediate isomers and promotes catalytic cracking on NiPt/HY core. With the increase of silica shell thickness from 0 to 40 nm, PEB reaction rate has increased more than five times, and the major cracking product selectivity is raised to above 90%, which is attributed to the continuous conversion of PEB isomers within the shell. This designed structure endows the NiPt/HY@SiO2 with a high activity and no obvious deactivation in PEB cracking to corresponding phenol and aromatics. The outstanding performance benefit from the enrichment effect on the unique core-shell structure, as well as the moderate acidity originated from silica regulation. This work can be extended to the modulation of microenvironment to promote the catalytic behavior of core-shell catalysts.

Suggested Citation

  • Song, Wenjing & Song, Mengxue & Cai, Wenqing & Li, Weichu & Jiang, Xingmao & Fang, Weiping & Lai, Weikun, 2022. "Efficient and stable SiO2-encapsulated NiPt/HY catalyst for catalytic cracking of β-O-4 linkage compound," Renewable Energy, Elsevier, vol. 198(C), pages 334-342.
    • Handle: RePEc:eee:renene:v:198:y:2022:i:c:p:334-342
    DOI: 10.1016/j.renene.2022.08.042
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