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Thermochemical behavior of perovskite oxides based on LaxSr1-x(Mn, Fe, Co)O3-δ and BaySr1-yCoO3-δ redox system for thermochemical energy storage at high temperatures

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  • Gokon, Nobuyuki
  • Yawata, Takehiro
  • Bellan, Selvan
  • Kodama, Tatsuya
  • Cho, Hyun-Seok

Abstract

LaxSr1-x(Mn, Fe, Co)O3-δ, and BaySr1-yCoO3-δ perovskite oxide powders were investigated as potential thermochemical energy storage (TES) materials operated at high temperatures above 600 °C. The purpose of the research is to provide complete characterization of the impact of partial A- and B-site substitution on the reactivity, kinetics, redox reaction repeatability and charging/discharging storage capacity. The perovskite oxides were investigated by thermogravimetric analysis (TGA) and differential scanning calorimetry (DSC) at temperatures of 500–1100 °C. Thermal energy storage was evaluated in terms of the enthalpy of the reversible reactions of oxygen release (reduction) and uptake (oxidation) upon heating the oxide materials in air stream. Among the perovskites tested, Ba0.3Sr0.7CoO3-δ and Ba0.7Sr0.3CoO3-δ powders were suitable thermochemical storage materials operating at above 600 °C in terms of chemical reactivity, charging/discharging temperatures and storage capacities, kinetics of oxygen uptake/release, and repeatability of thermochemical cycling. Further, charging/discharging capacity for both perovskites was comparable to that for Fe-doped manganese oxide.

Suggested Citation

  • Gokon, Nobuyuki & Yawata, Takehiro & Bellan, Selvan & Kodama, Tatsuya & Cho, Hyun-Seok, 2019. "Thermochemical behavior of perovskite oxides based on LaxSr1-x(Mn, Fe, Co)O3-δ and BaySr1-yCoO3-δ redox system for thermochemical energy storage at high temperatures," Energy, Elsevier, vol. 171(C), pages 971-980.
    • Handle: RePEc:eee:energy:v:171:y:2019:i:c:p:971-980
    DOI: 10.1016/j.energy.2019.01.081
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    1. Selvan Bellan & Tatsuya Kodama & Nobuyuki Gokon & Koji Matsubara, 2022. "A review on high‐temperature thermochemical heat storage: Particle reactors and materials based on solid–gas reactions," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 11(5), September.
    2. Laurie André & Stéphane Abanades, 2020. "Recent Advances in Thermochemical Energy Storage via Solid–Gas Reversible Reactions at High Temperature," Energies, MDPI, vol. 13(22), pages 1-23, November.
    3. Nobuyuki Gokon & Kosuke Hayashi & Hiroki Sawaguri & Fumiya Ohashi, 2022. "Long-Term Thermal Cycling Test and Heat-Charging Kinetics of Fe-Substituted Mn 2 O 3 for Next-Generation Concentrated Solar Power Using Thermochemical Energy Storage at High Temperatures," Energies, MDPI, vol. 15(13), pages 1-23, June.
    4. Nobuyuki Gokon & Fumiya Ohashi & Hiroki Sawaguri & Kosuke Hayashi, 2023. "Comparative Study of Heat-Discharging Kinetics of Fe-Substituted Mn 2 O 3 /Mn 3 O 4 Being Subjected to Long-Term Cycling for Thermochemical Energy Storage," Energies, MDPI, vol. 16(8), pages 1-23, April.

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