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Valorisation of spent coffee grounds as CO2 adsorbents for postcombustion capture applications

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  • Plaza, M.G.
  • González, A.S.
  • Pevida, C.
  • Pis, J.J.
  • Rubiera, F.

Abstract

In this work spent coffee grounds from single-use capsules were used as the starting material for producing low-cost activated carbons. The activation conditions were selected and optimised to produce microporous carbons with high CO2 adsorption capacity and selectivity, thus with potential to be used as adsorbents in postcombustion CO2 capture applications. Two activation methods are compared: physical activation with CO2 and chemical activation with KOH. The first method is considered less contaminant; however, leads to carbons with lower textural development and thus lower CO2 adsorption capacity than those obtained by activation with KOH. On the other hand, multicomponent adsorption cyclic experiments pointed out that the CO2/N2 selectivity of physically activated carbons is higher than that of chemically activated carbons.

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  • Plaza, M.G. & González, A.S. & Pevida, C. & Pis, J.J. & Rubiera, F., 2012. "Valorisation of spent coffee grounds as CO2 adsorbents for postcombustion capture applications," Applied Energy, Elsevier, vol. 99(C), pages 272-279.
    • Handle: RePEc:eee:appene:v:99:y:2012:i:c:p:272-279
    DOI: 10.1016/j.apenergy.2012.05.028
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    7. R. Maniarasu & Sushil Kumar Rathore & S. Murugan, 2023. "Biomass-based activated carbon for CO2 adsorption–A review," Energy & Environment, , vol. 34(5), pages 1674-1721, August.
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    13. Fernando Rubiera & Carlos Córdoba & Tamara Pena & Marta G. Plaza, 2024. "Production of Sustainable Adsorbents for CO 2 Capture Applications from Food Biowastes," Energies, MDPI, vol. 17(5), pages 1-20, March.
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    15. Alexandre Vandeponseele & Micheline Draye & Christine Piot & Gregory Chatel, 2021. "Study of Influential Parameters of the Caffeine Extraction from Spent Coffee Grounds: From Brewing Coffee Method to the Waste Treatment Conditions," Clean Technol., MDPI, vol. 3(2), pages 1-16, April.
    16. Yaumi, A.L. & Bakar, M.Z. Abu & Hameed, B.H., 2018. "Melamine-nitrogenated mesoporous activated carbon derived from rice husk for carbon dioxide adsorption in fixed-bed," Energy, Elsevier, vol. 155(C), pages 46-55.
    17. Zhang, Minkai & Guo, Yincheng, 2013. "Rate based modeling of absorption and regeneration for CO2 capture by aqueous ammonia solution," Applied Energy, Elsevier, vol. 111(C), pages 142-152.
    18. Nausika Querejeta & M. Victoria Gil & Fernando Rubiera & Covadonga Pevida, 2018. "Sustainable coffee†based CO2 adsorbents: toward a greener production via hydrothermal carbonization," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 8(2), pages 309-323, April.
    19. Marcelina Sołtysik & Izabela Majchrzak-Kucęba & Dariusz Wawrzyńczak, 2022. "Bio-Waste as a Substitute for the Production of Carbon Dioxide Adsorbents: A Review," Energies, MDPI, vol. 15(19), pages 1-23, September.
    20. Lachman, Jakub & Lisý, Martin & Baláš, Marek & Matúš, Miloš & Lisá, Hana & Milčák, Pavel, 2022. "Spent coffee grounds and wood co-firing: Fuel preparation, properties, thermal decomposition, and emissions," Renewable Energy, Elsevier, vol. 193(C), pages 464-474.
    21. Amira Alazmi & Sabina A. Nicolae & Pierpaolo Modugno & Bashir E. Hasanov & Maria M. Titirici & Pedro M. F. J. Costa, 2021. "Activated Carbon from Palm Date Seeds for CO 2 Capture," IJERPH, MDPI, vol. 18(22), pages 1-11, November.
    22. Plaza, M.G. & Durán, I. & Rubiera, F. & Pevida, C., 2015. "CO2 adsorbent pellets produced from pine sawdust: Effect of coal tar pitch addition," Applied Energy, Elsevier, vol. 144(C), pages 182-192.
    23. Guo, Yafei & Zhao, Chuanwen & Chen, Xiaoping & Li, Changhai, 2015. "CO2 capture and sorbent regeneration performances of some wood ash materials," Applied Energy, Elsevier, vol. 137(C), pages 26-36.
    24. Dissanayake, Pavani Dulanja & Choi, Seung Wan & Igalavithana, Avanthi Deshani & Yang, Xiao & Tsang, Daniel C.W. & Wang, Chi-Hwa & Kua, Harn Wei & Lee, Ki Bong & Ok, Yong Sik, 2020. "Sustainable gasification biochar as a high efficiency adsorbent for CO2 capture: A facile method to designer biochar fabrication," Renewable and Sustainable Energy Reviews, Elsevier, vol. 124(C).
    25. Huang, Yu-Fong & Cheng, Pei-Hsin & Chiueh, Pei-Te & Lo, Shang-Lien, 2017. "Leucaena biochar produced by microwave torrefaction: Fuel properties and energy efficiency," Applied Energy, Elsevier, vol. 204(C), pages 1018-1025.

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    Keywords

    CO2 capture; Activated carbon; Coffee residues;
    All these keywords.

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