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Modelling, simulation and analysis of intensified regenerator for solvent based carbon capture using rotating packed bed technology

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  • Joel, Atuman S.
  • Wang, Meihong
  • Ramshaw, Colin
  • Oko, Eni

Abstract

Intensified regenerator/stripper using rotating packed bed (RPB) for regeneration of rich-MEA solvent in post-combustion CO2 capture with chemical absorption process was studied through modelling and simulation in this paper. This is the first systematic study of RPB regenerator through modelling as there is no such publication in the open literature. Correlations for liquid and gas mass transfer coefficients, heat transfer coefficient, liquid hold-up, interfacial area and pressure drop which are suitable for RPB regenerator were written in visual FORTRAN as subroutines and then dynamically linked with Aspen Plus® rate-based model to replace the default mass and heat transfer correlations in the Aspen Plus®. The model now represents intensified regenerator/stripper. Model validation shows good agreement between model predictions and experimental data from literature. Process analyses were performed to investigate the effect of rotor speed on the regeneration efficiency and regeneration energy (including motor power). The rotor speed was varied from 200 to 1200rpm, which was selected to cover the validation range of rotor speed. Impact of reboiler temperature on the rate of CO2 stripping was also investigated. Effect of rich-MEA flow rate on regeneration energy and regeneration efficiency was studied. All the process analyses were done for wide range of MEA concentration (32.6wt%, 50wt% and 60wt%). Comparative study between regenerator using packed column and intensified regenerator using RPB was performed and the study shows a size reduction of 9.691 times. This study indicates that RPB process has great potential in thermal regeneration application.

Suggested Citation

  • Joel, Atuman S. & Wang, Meihong & Ramshaw, Colin & Oko, Eni, 2017. "Modelling, simulation and analysis of intensified regenerator for solvent based carbon capture using rotating packed bed technology," Applied Energy, Elsevier, vol. 203(C), pages 11-25.
    • Handle: RePEc:eee:appene:v:203:y:2017:i:c:p:11-25
    DOI: 10.1016/j.apenergy.2017.05.157
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    References listed on IDEAS

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    1. Wang, Meihong & Joel, Atuman S. & Ramshaw, Colin & Eimer, Dag & Musa, Nuhu M., 2015. "Process intensification for post-combustion CO2 capture with chemical absorption: A critical review," Applied Energy, Elsevier, vol. 158(C), pages 275-291.
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    Cited by:

    1. Wu, Xiao & Wang, Meihong & Liao, Peizhi & Shen, Jiong & Li, Yiguo, 2020. "Solvent-based post-combustion CO2 capture for power plants: A critical review and perspective on dynamic modelling, system identification, process control and flexible operation," Applied Energy, Elsevier, vol. 257(C).
    2. Oko, Eni & Ramshaw, Colin & Wang, Meihong, 2018. "Study of intercooling for rotating packed bed absorbers in intensified solvent-based CO2 capture process," Applied Energy, Elsevier, vol. 223(C), pages 302-316.
    3. Muhammad Asif & Muhammad Suleman & Ihtishamul Haq & Syed Asad Jamal, 2018. "Post‐combustion CO2 capture with chemical absorption and hybrid system: current status and challenges," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 8(6), pages 998-1031, December.
    4. Mohd Mu’Izzuddin Mohd Pauzi & Nurulhuda Azmi & Kok Keong Lau, 2022. "Emerging Solvent Regeneration Technologies for CO 2 Capture through Offshore Natural Gas Purification Processes," Sustainability, MDPI, vol. 14(7), pages 1-18, April.
    5. Wang, Tao & Yu, Wei & Le Moullec, Yann & Liu, Fei & Xiong, Yili & He, Hui & Lu, Jiahui & Hsu, Emily & Fang, Mengxiang & Luo, Zhongyang, 2017. "Solvent regeneration by novel direct non-aqueous gas stripping process for post-combustion CO2 capture," Applied Energy, Elsevier, vol. 205(C), pages 23-32.
    6. Fang, Guochang & Tian, Lixin & Liu, Menghe & Fu, Min & Sun, Mei, 2018. "How to optimize the development of carbon trading in China—Enlightenment from evolution rules of the EU carbon price," Applied Energy, Elsevier, vol. 211(C), pages 1039-1049.
    7. Otitoju, Olajide & Oko, Eni & Wang, Meihong, 2023. "Modelling, scale-up and techno-economic assessment of rotating packed bed absorber for CO2 capture from a 250 MWe combined cycle gas turbine power plant," Applied Energy, Elsevier, vol. 335(C).

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