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A Review on Buried Interface of Perovskite Solar Cells

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  • Yu Pu

    (State Key Laboratory of Solidification Processing, Northwestern Polytechnical University, Xi’an 710072, China)

  • Haijun Su

    (State Key Laboratory of Solidification Processing, Northwestern Polytechnical University, Xi’an 710072, China
    Research & Development Institute, Northwestern Polytechnical University, Shenzhen 518057, China)

  • Congcong Liu

    (State Key Laboratory of Solidification Processing, Northwestern Polytechnical University, Xi’an 710072, China)

  • Min Guo

    (State Key Laboratory of Solidification Processing, Northwestern Polytechnical University, Xi’an 710072, China)

  • Lin Liu

    (State Key Laboratory of Solidification Processing, Northwestern Polytechnical University, Xi’an 710072, China)

  • Hengzhi Fu

    (State Key Laboratory of Solidification Processing, Northwestern Polytechnical University, Xi’an 710072, China)

Abstract

Perovskite solar cells (PSCs) have been developed rapidly in recent years because of their excellent photoelectric performance. However, interfacial non-radiative recombination hinders the improvement of device performance. The buried interface modification strategy can minimize the non-radiation recombination in the interface and can obtain the high efficiency and stability of PSCs. In this review, we introduce the device structure and the charge carrier dynamics (charge transfer, extraction, and collection) at the interface. We further summarize the main sources of non-radiative recombination at the interface, such as energy alignment mismatch and interface defects, and methods to characterize them. In contrast to the previous review of perovskite solar cells, the important roles of buried interfaces in regulating energy level alignment, passivating surface defects, modulating morphology, and so on are reviewed in detail based on the latest research, and strategies for reducing interfacial nonradiative recombination are provided. In the end, the potential development and challenges of buried interfaces for high-performance and stable PSCs are presented.

Suggested Citation

  • Yu Pu & Haijun Su & Congcong Liu & Min Guo & Lin Liu & Hengzhi Fu, 2023. "A Review on Buried Interface of Perovskite Solar Cells," Energies, MDPI, vol. 16(13), pages 1-30, June.
  • Handle: RePEc:gam:jeners:v:16:y:2023:i:13:p:5015-:d:1181801
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    References listed on IDEAS

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