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Experimental density and an improved Helmholtz-energy-explicit mixture model for (CO2 + CO)

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  • Souza, Lorena F.S.
  • Herrig, Stefan
  • Span, Roland
  • Trusler, J.P. Martin

Abstract

This study reports new density measurements of the (CO2 + CO) system at temperatures from (283 to 373) K and pressures up to 48 MPa for four different mixtures, with compositions ranging from (5 to 50) mol% CO. A commercial vibrating-tube densimeter was used to measure the density of each mixture as a function of pressure and temperature. Temperature and pressure were measured with expanded uncertainties (k = 2) of 0.05 K and 0.035 MPa, respectively. The relative combined expanded uncertainty (k = 2) of the density was estimated to be between (0.2 and 1.8) %, with values ≤1% for most state points. The new data significantly expand the pressure and composition ranges of the available density data for the (CO2 + CO) system. Together with recently published vapour-liquid-equilibrium data, the new data enabled the development of an improved Helmholtz-energy-explicit mixture model. The new model is based on the mathematical approach of the GERG-2008 and EOS-CG models with new adjustable parameters. As a result, the new mixture model allows for a significantly more accurate description of the thermodynamic properties of the (CO2 + CO) system than GERG-2008 and EOS-CG. A detailed comparison among our density data, experimental data from the literature and the different mixture models is presented.

Suggested Citation

  • Souza, Lorena F.S. & Herrig, Stefan & Span, Roland & Trusler, J.P. Martin, 2019. "Experimental density and an improved Helmholtz-energy-explicit mixture model for (CO2 + CO)," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    • Handle: RePEc:eee:appene:v:251:y:2019:i:c:101
    DOI: 10.1016/j.apenergy.2019.113398
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    1. Munkejord, Svend Tollak & Hammer, Morten & Løvseth, Sigurd W., 2016. "CO2 transport: Data and models – A review," Applied Energy, Elsevier, vol. 169(C), pages 499-523.
    2. Li, Hailong & Jakobsen, Jana P. & Wilhelmsen, Øivind & Yan, Jinyue, 2011. "PVTxy properties of CO2 mixtures relevant for CO2 capture, transport and storage: Review of available experimental data and theoretical models," Applied Energy, Elsevier, vol. 88(11), pages 3567-3579.
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