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Wet impregnation of a commercial low cost silica using DETA for a fast post-combustion CO2 capture process

Author

Listed:
  • Martín, C.F.
  • Sweatman, M.B.
  • Brandani, S.
  • Fan, X.

Abstract

This work presents an economic and simple method to manufacture low cost, but effective adsorbents for CO2 capture through impregnating DETA to a low cost, porous silica gel. The results have demonstrated that the low cost silica gel impregnated by low molecular-weight amine is stable and work very well at a temperature up to 130°C. The developed adsorbent has a fast adsorption kinetics and can be regenerated at a low temperature. This will significantly reduce the energy used to desorb CO2, therefore the energy penalty. The effect of amine loading on the textural properties, thermal stability, and CO2 capture performance of the impregnated silica gel is also reported in this paper. 10% amine loading gives the best porosity, stability and the highest adsorption capacity.

Suggested Citation

  • Martín, C.F. & Sweatman, M.B. & Brandani, S. & Fan, X., 2016. "Wet impregnation of a commercial low cost silica using DETA for a fast post-combustion CO2 capture process," Applied Energy, Elsevier, vol. 183(C), pages 1705-1721.
    • Handle: RePEc:eee:appene:v:183:y:2016:i:c:p:1705-1721
    DOI: 10.1016/j.apenergy.2016.09.081
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    References listed on IDEAS

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    1. Kevin P. Resnik & James T. Yeh & Henry W. Pennline, 2004. "Aqua ammonia process for simultaneous removal of CO 2 , SO 2 and NO x," International Journal of Environmental Technology and Management, Inderscience Enterprises Ltd, vol. 4(1/2), pages 89-104.
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    Cited by:

    1. Lai, Qinghua & Diao, Zhijun & Kong, Lingli & Adidharma, Hertanto & Fan, Maohong, 2018. "Amine-impregnated silicic acid composite as an efficient adsorbent for CO2 capture," Applied Energy, Elsevier, vol. 223(C), pages 293-301.
    2. Hu, Xiayi (Eric) & Liu, Libin & Luo, Xiao & Xiao, Gongkui & Shiko, Elenica & Zhang, Rui & Fan, Xianfeng & Zhou, Yefeng & Liu, Yang & Zeng, Zhaogang & Li, Chao'en, 2020. "A review of N-functionalized solid adsorbents for post-combustion CO2 capture," Applied Energy, Elsevier, vol. 260(C).
    3. Chao, Cong & Deng, Yimin & Dewil, Raf & Baeyens, Jan & Fan, Xianfeng, 2021. "Post-combustion carbon capture," Renewable and Sustainable Energy Reviews, Elsevier, vol. 138(C).
    4. Zhang, Xiaowen & Huang, Yufei & Gao, Hongxia & Luo, Xiao & Liang, Zhiwu & Tontiwachwuthikul, Paitoon, 2019. "Zeolite catalyst-aided tri-solvent blend amine regeneration: An alternative pathway to reduce the energy consumption in amine-based CO2 capture process," Applied Energy, Elsevier, vol. 240(C), pages 827-841.
    5. Li, Xiangyu & Wang, Zhiqing & Liu, Zheyu & Feng, Ru & Song, Shuangshuang & Huang, Jiejie & Fang, Yitian, 2022. "A novel preparation of solid amine sorbents for enhancing CO2 adsorption capacity using alumina-extracted waste," Energy, Elsevier, vol. 248(C).
    6. Chen, S.J. & Zhu, M. & Fu, Y. & Huang, Y.X. & Tao, Z.C. & Li, W.L., 2017. "Using 13X, LiX, and LiPdAgX zeolites for CO2 capture from post-combustion flue gas," Applied Energy, Elsevier, vol. 191(C), pages 87-98.
    7. Wang, Dandan & Li, Sheng & Liu, Feng & Gao, Lin & Sui, Jun, 2018. "Post combustion CO2 capture in power plant using low temperature steam upgraded by double absorption heat transformer," Applied Energy, Elsevier, vol. 227(C), pages 603-612.
    8. Tao, Huayu & Qian, Xi & Zhou, Yi & Cheng, Hongfei, 2022. "Research progress of clay minerals in carbon dioxide capture," Renewable and Sustainable Energy Reviews, Elsevier, vol. 164(C).

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    Keywords

    CO2 capture; Adsorption; Amine; DETA; Impregnation; Thermal stability;
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