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Thermal fractionation and catalytic upgrading of lignocellulosic biomass to biofuels: Process synthesis and analysis

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  • Won, Wangyun
  • Maravelias, Christos T.

Abstract

Multi-stage thermal biomass decomposition coupled with catalytic upgrading has a number of advantages over conventional single-stage pyrolysis with hydrotreating. However, significant gaps still exist in our understanding of the design of such processes. In this paper, we synthesize alternative catalytic upgrading strategies through integration of different chemistries. Using experimental data, we develop a process model for all strategies and conduct heat integration to minimize utility requirements. Then, using a wide range of technoeconomic analyses, we identify (1) the relationship between process complexity and the resulting fuel-range carbon yields and economic feasibility, (2) the economic advantage of integrating different thermal decomposition fractions, and (3) the key cost drivers of the integrated processes.

Suggested Citation

  • Won, Wangyun & Maravelias, Christos T., 2017. "Thermal fractionation and catalytic upgrading of lignocellulosic biomass to biofuels: Process synthesis and analysis," Renewable Energy, Elsevier, vol. 114(PB), pages 357-366.
    • Handle: RePEc:eee:renene:v:114:y:2017:i:pb:p:357-366
    DOI: 10.1016/j.renene.2017.07.023
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    References listed on IDEAS

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    1. Chew, J.J. & Doshi, V., 2011. "Recent advances in biomass pretreatment – Torrefaction fundamentals and technology," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(8), pages 4212-4222.
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    1. Ahn, Byeongchan & Park, Chulhwan & Liu, J. Jay & Ok, Yong Sik & Won, Wangyun, 2023. "Maximizing the utilization of lignocellulosic biomass: Process development and analysis," Renewable Energy, Elsevier, vol. 215(C).
    2. Zainol, Muzakkir Mohammad & Amin, Nor Aishah Saidina & Asmadi, Mohd, 2019. "Kinetics and thermodynamic analysis of levulinic acid esterification using lignin-furfural carbon cryogel catalyst," Renewable Energy, Elsevier, vol. 130(C), pages 547-557.
    3. Jisook Lee & Yongho Son & Kwang Soon Lee & Wangyun Won, 2019. "Economic Analysis and Environmental Impact Assessment of Heat Pump-Assisted Distillation in a Gas Fractionation Unit," Energies, MDPI, vol. 12(5), pages 1-19, March.
    4. Kim, Hyunwoo & Lee, Shinje & Won, Wangyun, 2021. "System-level analyses for the production of 1,6-hexanediol from cellulose," Energy, Elsevier, vol. 214(C).
    5. Ng, Rex T.L. & Maravelias, Christos T., 2017. "Economic and energetic analysis of biofuel supply chains," Applied Energy, Elsevier, vol. 205(C), pages 1571-1582.
    6. Choe, Bomin & Lee, Shinje & Won, Wangyun, 2020. "Process integration and optimization for economical production of commodity chemicals from lignocellulosic biomass," Renewable Energy, Elsevier, vol. 162(C), pages 242-248.
    7. Naqvi, Salman Raza & Tariq, Rumaisa & Hameed, Zeeshan & Ali, Imtiaz & Naqvi, Muhammad & Chen, Wei-Hsin & Ceylan, Selim & Rashid, Harith & Ahmad, Junaid & Taqvi, Syed A. & Shahbaz, Muhammad, 2019. "Pyrolysis of high ash sewage sludge: Kinetics and thermodynamic analysis using Coats-Redfern method," Renewable Energy, Elsevier, vol. 131(C), pages 854-860.
    8. Hansen, Samuel & Mirkouei, Amin & Diaz, Luis A., 2020. "A comprehensive state-of-technology review for upgrading bio-oil to renewable or blended hydrocarbon fuels," Renewable and Sustainable Energy Reviews, Elsevier, vol. 118(C).
    9. Antar, Mohammed & Lyu, Dongmei & Nazari, Mahtab & Shah, Ateeq & Zhou, Xiaomin & Smith, Donald L., 2021. "Biomass for a sustainable bioeconomy: An overview of world biomass production and utilization," Renewable and Sustainable Energy Reviews, Elsevier, vol. 139(C).
    10. Kim, H. & Baek, S. & Won, W., 2022. "Integrative technical, economic, and environmental sustainability analysis for the development process of biomass-derived 2,5-furandicarboxylic acid," Renewable and Sustainable Energy Reviews, Elsevier, vol. 157(C).

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