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Optimization of tri-reformer reactor to produce synthesis gas for methanol production using differential evolution (DE) method

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  • Arab Aboosadi, Z.
  • Jahanmiri, A.H.
  • Rahimpour, M.R.

Abstract

This paper presents a study on optimization of a fixed bed tri-reformer reactor (TR). This reactor has been used instead of conventional steam reformer (CSR) and auto thermal reformer (CAR). A theoretical investigation has been performed in order to evaluate the optimal operating conditions and enhancement of methane conversion, hydrogen production and desired H2/CO ratio as a synthesis gas for methanol production. A mathematical heterogeneous model has been used to simulate the reactor. The process performance under steady state conditions was analyzed with respect to key operational parameters (inlet temperature, O2/CH4, CO2/CH4 and steam/CH4 ratios). The influence of these parameters on gas temperature, methane conversion, hydrogen production and H2/CO ratio was investigated. Model validation was carried out by comparison of the reforming model results with industrial data of CSR. Differential evolution (DE) method was applied as a powerful method for optimization. Optimum feed temperature and reactant ratios (CH4/CO2/H2O/O2) are 1100Â K and 1/1.3/2.46/0.47 respectively. The optimized TR has enhanced methane conversion by 3.8% relative to industrial reformers in a single reactor. Methane conversion, hydrogen yield and H2/CO ratio in optimized TR are 97.9%, 1.84 and 1.7 respectively. The optimization results of tri-reformer were compared with the corresponding predictions from process simulation software operated at the same feed conditions.

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  • Arab Aboosadi, Z. & Jahanmiri, A.H. & Rahimpour, M.R., 2011. "Optimization of tri-reformer reactor to produce synthesis gas for methanol production using differential evolution (DE) method," Applied Energy, Elsevier, vol. 88(8), pages 2691-2701, August.
    • Handle: RePEc:eee:appene:v:88:y:2011:i:8:p:2691-2701
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    2. Rei-Yu Chein & Wen-Hwai Hsu, 2018. "Analysis of Syngas Production from Biogas via the Tri-Reforming Process," Energies, MDPI, vol. 11(5), pages 1-18, April.
    3. Wang, Ligang & Yang, Yongping & Dong, Changqing & Morosuk, Tatiana & Tsatsaronis, George, 2014. "Multi-objective optimization of coal-fired power plants using differential evolution," Applied Energy, Elsevier, vol. 115(C), pages 254-264.
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    5. Byun, Manhee & Lim, Dongjun & Lee, Boreum & Kim, Ayeon & Lee, In-Beum & Brigljević, Boris & Lim, Hankwon, 2022. "Economically feasible decarbonization of the Haber-Bosch process through supercritical CO2 Allam cycle integration," Applied Energy, Elsevier, vol. 307(C).
    6. Chein, Rei-Yu & Wang, Chien-Yu & Yu, Ching-Tsung, 2017. "Parametric study on catalytic tri-reforming of methane for syngas production," Energy, Elsevier, vol. 118(C), pages 1-17.
    7. Samira Soleimani & Markus Lehner, 2022. "Tri-Reforming of Methane: Thermodynamics, Operating Conditions, Reactor Technology and Efficiency Evaluation—A Review," Energies, MDPI, vol. 15(19), pages 1-40, September.
    8. Chen, Wei-Hsin & Lin, Shih-Cheng, 2016. "Characterization of catalytic partial oxidation of methane with carbon dioxide utilization and excess enthalpy recovery," Applied Energy, Elsevier, vol. 162(C), pages 1141-1152.
    9. Ganesan, T. & Elamvazuthi, I. & Ku Shaari, Ku Zilati & Vasant, P., 2013. "Swarm intelligence and gravitational search algorithm for multi-objective optimization of synthesis gas production," Applied Energy, Elsevier, vol. 103(C), pages 368-374.
    10. Glotić, Arnel & Zamuda, Aleš, 2015. "Short-term combined economic and emission hydrothermal optimization by surrogate differential evolution," Applied Energy, Elsevier, vol. 141(C), pages 42-56.
    11. Chen, Hsi-Jen & Fan, Chei-Wei & Yu, Chiou-Shia, 2013. "Analysis, synthesis, and design of a one-step dimethyl ether production via a thermodynamic approach," Applied Energy, Elsevier, vol. 101(C), pages 449-456.
    12. Gaber, Christian & Demuth, Martin & Prieler, René & Schluckner, Christoph & Schroettner, Hartmuth & Fitzek, Harald & Hochenauer, Christoph, 2019. "Experimental investigation of thermochemical regeneration using oxy-fuel exhaust gases," Applied Energy, Elsevier, vol. 236(C), pages 1115-1124.

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