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A study on the activity of CaO-based sorbents for capturing CO2 in clean energy processes

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  • Wang, Jinsheng
  • Manovic, Vasilije
  • Wu, Yinghai
  • Anthony, Edward J.

Abstract

CaO-based regenerative sorbents for CO2 capture in power generation and H2 production are receiving growing attention. A major challenge for this technology is the decay of sorbent activity with increasing number of the sorption/regeneration cycles. Evaluation of long-term sorbent activity currently requires substantial experimental work. In this study, the dependence of the activity on the number of sorption/regeneration cycles is examined, and the apparent dependence on the number of cycles is related to the duration of sorbent regeneration. By relating the decay in activity of the sorbent to its decrease in surface area due to sintering, interesting insights can be drawn. A method for determination of the long-term activity has been proposed, which can greatly reduce the experimental work for sorbent development and process evaluation.

Suggested Citation

  • Wang, Jinsheng & Manovic, Vasilije & Wu, Yinghai & Anthony, Edward J., 2010. "A study on the activity of CaO-based sorbents for capturing CO2 in clean energy processes," Applied Energy, Elsevier, vol. 87(4), pages 1453-1458, April.
    • Handle: RePEc:eee:appene:v:87:y:2010:i:4:p:1453-1458
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    1. Ben-Mansour, R. & Habib, M.A. & Bamidele, O.E. & Basha, M. & Qasem, N.A.A. & Peedikakkal, A. & Laoui, T. & Ali, M., 2016. "Carbon capture by physical adsorption: Materials, experimental investigations and numerical modeling and simulations – A review," Applied Energy, Elsevier, vol. 161(C), pages 225-255.
    2. Sun, Zhao & Chen, Shiyi & Ma, Shiwei & Xiang, Wenguo & Song, Quanbin, 2016. "Simulation of the calcium looping process (CLP) for hydrogen, carbon monoxide and acetylene poly-generation with CO2 capture and COS reduction," Applied Energy, Elsevier, vol. 169(C), pages 642-651.
    3. Perejón, Antonio & Romeo, Luis M. & Lara, Yolanda & Lisbona, Pilar & Martínez, Ana & Valverde, Jose Manuel, 2016. "The Calcium-Looping technology for CO2 capture: On the important roles of energy integration and sorbent behavior," Applied Energy, Elsevier, vol. 162(C), pages 787-807.
    4. Li, Bingyun & Duan, Yuhua & Luebke, David & Morreale, Bryan, 2013. "Advances in CO2 capture technology: A patent review," Applied Energy, Elsevier, vol. 102(C), pages 1439-1447.
    5. Kavosh, Masoud & Patchigolla, Kumar & Anthony, Edward J. & Oakey, John E., 2014. "Carbonation performance of lime for cyclic CO2 capture following limestone calcination in steam/CO2 atmosphere," Applied Energy, Elsevier, vol. 131(C), pages 499-507.
    6. Li, Yingjie & Su, Mengying & Xie, Xin & Wu, Shuimu & Liu, Changtian, 2015. "CO2 capture performance of synthetic sorbent prepared from carbide slag and aluminum nitrate hydrate by combustion synthesis," Applied Energy, Elsevier, vol. 145(C), pages 60-68.
    7. Jiang, Bingbing & Wang, Xianfeng & Gray, McMahan L. & Duan, Yuhua & Luebke, David & Li, Bingyun, 2013. "Development of amino acid and amino acid-complex based solid sorbents for CO2 capture," Applied Energy, Elsevier, vol. 109(C), pages 112-118.
    8. Itskos, Grigorios & Grammelis, Panagiotis & Scala, Fabrizio & Pawlak-Kruczek, Halina & Coppola, Antonio & Salatino, Piero & Kakaras, Emmanuel, 2013. "A comparative characterization study of Ca-looping natural sorbents," Applied Energy, Elsevier, vol. 108(C), pages 373-382.
    9. Valverde, J.M. & Sanchez-Jimenez, P.E. & Perez-Maqueda, L.A. & Quintanilla, M.A.S. & Perez-Vaquero, J., 2014. "Role of crystal structure on CO2 capture by limestone derived CaO subjected to carbonation/recarbonation/calcination cycles at Ca-looping conditions," Applied Energy, Elsevier, vol. 125(C), pages 264-275.
    10. Wang, Wenjing & Li, Yingjie & Xie, Xin & Sun, Rongyue, 2014. "Effect of the presence of HCl on cyclic CO2 capture of calcium-based sorbent in calcium looping process," Applied Energy, Elsevier, vol. 125(C), pages 246-253.
    11. Xie, Xin & Li, Yingjie & Wang, Wenjing & Shi, Lei, 2014. "HCl removal using cycled carbide slag from calcium looping cycles," Applied Energy, Elsevier, vol. 135(C), pages 391-401.
    12. Li, Jia & Tharakan, Pradeep & Macdonald, Douglas & Liang, Xi, 2013. "Technological, economic and financial prospects of carbon dioxide capture in the cement industry," Energy Policy, Elsevier, vol. 61(C), pages 1377-1387.
    13. Lara, Yolanda & Lisbona, Pilar & Martínez, Ana & Romeo, Luis M., 2013. "Design and analysis of heat exchanger networks for integrated Ca-looping systems," Applied Energy, Elsevier, vol. 111(C), pages 690-700.
    14. Jing, Jie-ying & Zhang, Xue-wei & Li, Qing & Li, Ting-yu & Li, Wen-ying, 2018. "Self-activation of CaO/Ca3Al2O6 sorbents by thermally pretreated in CO2 atmosphere," Applied Energy, Elsevier, vol. 220(C), pages 419-425.
    15. Chen, Shiyi & Xiang, Wenguo & Wang, Dong & Xue, Zhipeng, 2012. "Incorporating IGCC and CaO sorption-enhanced process for power generation with CO2 capture," Applied Energy, Elsevier, vol. 95(C), pages 285-294.
    16. Valverde, J.M. & Sanchez-Jimenez, P.E. & Perez-Maqueda, L.A., 2015. "Ca-looping for postcombustion CO2 capture: A comparative analysis on the performances of dolomite and limestone," Applied Energy, Elsevier, vol. 138(C), pages 202-215.
    17. Erans, María & Manovic, Vasilije & Anthony, Edward J., 2016. "Calcium looping sorbents for CO2 capture," Applied Energy, Elsevier, vol. 180(C), pages 722-742.
    18. Mikulčić, Hrvoje & Vujanović, Milan & Duić, Neven, 2013. "Reducing the CO2 emissions in Croatian cement industry," Applied Energy, Elsevier, vol. 101(C), pages 41-48.
    19. Lisbona, Pilar & Martínez, Ana & Romeo, Luis M., 2013. "Hydrodynamical model and experimental results of a calcium looping cycle for CO2 capture," Applied Energy, Elsevier, vol. 101(C), pages 317-322.
    20. Valverde, J.M. & Sanchez-Jimenez, P.E. & Perez-Maqueda, L.A., 2014. "Role of precalcination and regeneration conditions on postcombustion CO2 capture in the Ca-looping technology," Applied Energy, Elsevier, vol. 136(C), pages 347-356.

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    CO2 capture Solid sorbents Long-term or residual activity;

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