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Incorporating IGCC and CaO sorption-enhanced process for power generation with CO2 capture

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  • Chen, Shiyi
  • Xiang, Wenguo
  • Wang, Dong
  • Xue, Zhipeng

Abstract

Integrated gasification combined cycle (IGCC) is a power generation technology to convert solid fuels into electricity. IGCC with CCS is regarded as a promising option to mitigate CO2 emission. In this paper, the CaO sorption-enhanced process is incorporated downstream with coal gasification to produce a hydrogen-rich stream for electricity production and CO2 separation. A WGS-absorber substitutes the high- and low-temperature water–gas shift reactors and desulfurization units in conventional IGCC–CCS to produce a hydrogen-rich stream, which is sent onto a gas turbine. CaO is used as the sorbent to enhance hydrogen production and for CO2 capture. Regeneration of CaO is completed via calcination in a regenerator vessel. The IGCC with CaO sorption-enhanced process is modeled and simulated using Aspen Plus software. Two commercial available gasification technologies, Shell and Texaco, are integrated with the sorption-enhanced process. The results showed IGCC with CaO sorption-enhanced process has a satisfactory system performance. Even though the net electricity efficiency is not as high as expected, just around 30–33%, the system has a high CO2 capture efficiency ∼97% and low pollutant emissions. Moreover, compared with conventional IGCC–CCS, the schematic diagram of the IGCC–CCS process is simplified. Parameters that affect the plant performance are analyzed in the sensitive analysis, including WGS-absorber temperature, H2O/CO ratio, pressure, etc. Some challenges to the system are also discussed.

Suggested Citation

  • Chen, Shiyi & Xiang, Wenguo & Wang, Dong & Xue, Zhipeng, 2012. "Incorporating IGCC and CaO sorption-enhanced process for power generation with CO2 capture," Applied Energy, Elsevier, vol. 95(C), pages 285-294.
    • Handle: RePEc:eee:appene:v:95:y:2012:i:c:p:285-294
    DOI: 10.1016/j.apenergy.2012.02.056
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    13. David Berstad & Geir Skaugen & Simon Roussanaly & Rahul Anantharaman & Petter Nekså & Kristin Jordal & Stian Trædal & Truls Gundersen, 2022. "CO 2 Capture from IGCC by Low-Temperature Synthesis Gas Separation," Energies, MDPI, vol. 15(2), pages 1-24, January.
    14. Valverde, J.M. & Raganati, F. & Quintanilla, M.A.S. & Ebri, J.M.P. & Ammendola, P. & Chirone, R., 2013. "Enhancement of CO2 capture at Ca-looping conditions by high-intensity acoustic fields," Applied Energy, Elsevier, vol. 111(C), pages 538-549.
    15. Esmaili, Ehsan & Mostafavi, Ehsan & Mahinpey, Nader, 2016. "Economic assessment of integrated coal gasification combined cycle with sorbent CO2 capture," Applied Energy, Elsevier, vol. 169(C), pages 341-352.
    16. Gao, Jubao & Cao, Lingdi & Dong, Haifeng & Zhang, Xiangping & Zhang, Suojiang, 2015. "Ionic liquids tailored amine aqueous solution for pre-combustion CO2 capture: Role of imidazolium-based ionic liquids," Applied Energy, Elsevier, vol. 154(C), pages 771-780.
    17. Theo, Wai Lip & Lim, Jeng Shiun & Hashim, Haslenda & Mustaffa, Azizul Azri & Ho, Wai Shin, 2016. "Review of pre-combustion capture and ionic liquid in carbon capture and storage," Applied Energy, Elsevier, vol. 183(C), pages 1633-1663.
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    21. Mansouri Majoumerd, Mohammad & Raas, Han & De, Sudipta & Assadi, Mohsen, 2014. "Estimation of performance variation of future generation IGCC with coal quality and gasification process – Simulation results of EU H2-IGCC project," Applied Energy, Elsevier, vol. 113(C), pages 452-462.
    22. Huang, Yuping & Zheng, Qipeng P. & Fan, Neng & Aminian, Kashy, 2014. "Optimal scheduling for enhanced coal bed methane production through CO2 injection," Applied Energy, Elsevier, vol. 113(C), pages 1475-1483.
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    Keywords

    Coal; IGCC; Sorption-enhanced process; CaO; CO2 capture;
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