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Iron oxide looping for natural gas conversion in a countercurrent moving bed reactor

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  • Zeng, Liang
  • Tong, Andrew
  • Kathe, Mandar
  • Bayham, Samuel
  • Fan, Liang-Shih

Abstract

Chemical looping technologies have the potential to reduce the natural-gas conversion cost in a carbon-constrained scenario. Given the increasing importance of natural gas to global energy supply, this work investigates the application of an iron oxide based chemical looping technology for natural gas conversion. A thermodynamic criterion for selecting iron oxide based oxygen carrier material and designing the reaction system is developed using an adapted Ellingham diagram. Equilibrium modeling for detailed thermodynamic analysis is conducted for verifying the Ellingham diagram analysis. The thermodynamic equilibrium model also establishes a system baseline performance, and experimental proof of concept bench-scale demonstration is investigated. The bench-scale testing is used to characterize the effect of parameters like solids to gas ratio and temperature of the reactor on system performance. An optimal set of operating conditions is identified for further testing on a larger scale.

Suggested Citation

  • Zeng, Liang & Tong, Andrew & Kathe, Mandar & Bayham, Samuel & Fan, Liang-Shih, 2015. "Iron oxide looping for natural gas conversion in a countercurrent moving bed reactor," Applied Energy, Elsevier, vol. 157(C), pages 338-347.
    • Handle: RePEc:eee:appene:v:157:y:2015:i:c:p:338-347
    DOI: 10.1016/j.apenergy.2015.06.029
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    References listed on IDEAS

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    1. Paltsev, Sergey & Jacoby, Henry D. & Reilly, John M. & Ejaz, Qudsia J. & Morris, Jennifer & O'Sullivan, Francis & Rausch, Sebastian & Winchester, Niven & Kragha, Oghenerume, 2011. "The future of U.S. natural gas production, use, and trade," Energy Policy, Elsevier, vol. 39(9), pages 5309-5321, September.
    2. Lyngfelt, Anders, 2014. "Chemical-looping combustion of solid fuels – Status of development," Applied Energy, Elsevier, vol. 113(C), pages 1869-1873.
    3. Tang, Mingchen & Xu, Long & Fan, Maohong, 2015. "Progress in oxygen carrier development of methane-based chemical-looping reforming: A review," Applied Energy, Elsevier, vol. 151(C), pages 143-156.
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    Cited by:

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    2. Nicole Carina Preisner & Marc Linder, 2020. "A Moving Bed Reactor for Thermochemical Energy Storage Based on Metal Oxides," Energies, MDPI, vol. 13(5), pages 1-20, March.
    3. Samuel Bayham & Ronald Breault & Justin Weber, 2017. "Chemical Looping Combustion of Hematite Ore with Methane and Steam in a Fluidized Bed Reactor," Energies, MDPI, vol. 10(8), pages 1-22, August.
    4. Marek, Ewa & Hu, Wenting & Gaultois, Michael & Grey, Clare P. & Scott, Stuart A., 2018. "The use of strontium ferrite in chemical looping systems," Applied Energy, Elsevier, vol. 223(C), pages 369-382.
    5. Tescari, Stefania & Neumann, Nicole Carina & Sundarraj, Pradeepkumar & Moumin, Gkiokchan & Rincon Duarte, Juan Pablo & Linder, Marc & Roeb, Martin, 2022. "Storing solar energy in continuously moving redox particles – Experimental analysis of charging and discharging reactors," Applied Energy, Elsevier, vol. 308(C).
    6. Nicole Carina Preisner & Inga Bürger & Michael Wokon & Marc Linder, 2020. "Numerical Investigations of a Counter-Current Moving Bed Reactor for Thermochemical Energy Storage at High Temperatures," Energies, MDPI, vol. 13(3), pages 1-22, February.
    7. Siriwardane, Ranjani & Riley, Jarrett & Benincosa, William & Bayham, Samuel & Bobek, Michael & Straub, Douglas & Weber, Justin, 2021. "Development of CuFeMnAlO4+δ oxygen carrier with high attrition resistance and 50-kWth methane/air chemical looping combustion tests," Applied Energy, Elsevier, vol. 286(C).

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