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Sensitivity of the CO2 storage capacity of underground geological structures to the presence of SO2 and other impurities

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  • Ziabakhsh-Ganji, Zaman
  • Kooi, Henk

Abstract

Depleted hydrocarbon reservoirs and deep saline aquifers are key targets for geological storage of CO2 to reduce atmospheric CO2 emissions. Most studies in CCS investigate subsurface storage of pure CO2. In this paper we investigate the impact of the presence of other gases (impurities) in the injected CO2 stream on solubility trapping (in the aqueous phase) and volumetric trapping (in the non-aqueous phase, for a wide range of pressure and temperature. Calculations for solubility trapping are based on an equation of state that accurately accounts for the pressure, temperature, gas-compositional (mixtures) and salinity influences on CO2 solubility and brine density. For volumetric trapping the Peng–Robinson equation of state is used, accounting for binary interaction for gas mixtures and density correction. In the analysis, special attention is paid to the impact of SO2, which exhibits anomalous storage effects when compared to other common impurities.

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  • Ziabakhsh-Ganji, Zaman & Kooi, Henk, 2014. "Sensitivity of the CO2 storage capacity of underground geological structures to the presence of SO2 and other impurities," Applied Energy, Elsevier, vol. 135(C), pages 43-52.
    • Handle: RePEc:eee:appene:v:135:y:2014:i:c:p:43-52
    DOI: 10.1016/j.apenergy.2014.08.073
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    References listed on IDEAS

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    1. Li, Didi & Jiang, Xi, 2014. "A numerical study of the impurity effects of nitrogen and sulfur dioxide on the solubility trapping of carbon dioxide geological storage," Applied Energy, Elsevier, vol. 128(C), pages 60-74.
    2. Li, Hailong & Jakobsen, Jana P. & Wilhelmsen, Øivind & Yan, Jinyue, 2011. "PVTxy properties of CO2 mixtures relevant for CO2 capture, transport and storage: Review of available experimental data and theoretical models," Applied Energy, Elsevier, vol. 88(11), pages 3567-3579.
    3. Ziabakhsh-Ganji, Zaman & Kooi, Henk, 2014. "Sensitivity of Joule–Thomson cooling to impure CO2 injection in depleted gas reservoirs," Applied Energy, Elsevier, vol. 113(C), pages 434-451.
    4. Li, H. & Yan, J., 2009. "Evaluating cubic equations of state for calculation of vapor-liquid equilibrium of CO2 and CO2-mixtures for CO2 capture and storage processes," Applied Energy, Elsevier, vol. 86(6), pages 826-836, June.
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    Cited by:

    1. Li, Didi & Zhang, Hongcheng & Li, Yang & Xu, Wenbin & Jiang, Xi, 2018. "Effects of N2 and H2S binary impurities on CO2 geological storage in stratified formation – A sensitivity study," Applied Energy, Elsevier, vol. 229(C), pages 482-492.
    2. Wang, Zhiyu & Wang, Jinsheng & Lan, Christopher & He, Ian & Ko, Vivien & Ryan, David & Wigston, Andrew, 2016. "A study on the impact of SO2 on CO2 injectivity for CO2 storage in a Canadian saline aquifer," Applied Energy, Elsevier, vol. 184(C), pages 329-336.
    3. Sina Omrani & Saeed Mahmoodpour & Behzad Rostami & Mehdi Salehi Sedeh & Ingo Sass, 2021. "Diffusion coefficients of CO2–SO2–water and CO2–N2–water systems and their impact on the CO2 sequestration process: Molecular dynamics and dissolution process simulations," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 11(4), pages 764-779, August.
    4. Wei, Ning & Li, Xiaochun & Wang, Yan & Zhu, Qianlin & Liu, Shengnan & Liu, Naizhong & Su, Xuebing, 2015. "Geochemical impact of aquifer storage for impure CO2 containing O2 and N2: Tongliao field experiment," Applied Energy, Elsevier, vol. 145(C), pages 198-210.
    5. Gimeno, Beatriz & Artal, Manuela & Velasco, Inmaculada & Blanco, Sofía T. & Fernández, Javier, 2017. "Influence of SO2 on CO2 storage for CCS technology: Evaluation of CO2/SO2 co-capture," Applied Energy, Elsevier, vol. 206(C), pages 172-180.

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