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A study on the impact of SO2 on CO2 injectivity for CO2 storage in a Canadian saline aquifer

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  • Wang, Zhiyu
  • Wang, Jinsheng
  • Lan, Christopher
  • He, Ian
  • Ko, Vivien
  • Ryan, David
  • Wigston, Andrew

Abstract

Potential effects of SO2 as an impurity on CO2 injectivity for CO2 storage in a targeted sandstone saline aquifer in western Canada were investigated. Batch experiments using rock and brine samples in contact with supercritical CO2 and CO2 mixtures with SO2 were conducted in high-pressure reactors for 45days. The results suggest that SO2 increased precipitation of sodium chloride and calcium sulfate dehydrate, and also increased the dissolution of quartz. Moreover, the precipitation of sodium chloride appeared to be concurrent with the dissolution of quartz, the predominant constituent of the rock. The concurrent precipitation of sodium chloride and dissolution of quartz could be attributed to taking up of water by H4SiO4 that reduces the number of water molecules in the hydration shells of Na+ and Cl− ions in highly concentrated brine. According to this view, the dissolution of quartz, which would be much slower than the reassociation of dissolved sodium chloride ions, is limiting the rate of sodium chloride precipitation. The rate of quartz dissolution was estimated based on the present experimental data, which could be used to assess salt precipitation and determine suitable operation conditions for CO2 injection. The findings of this work should also be applicable to acid gas injection in oil and gas industry.

Suggested Citation

  • Wang, Zhiyu & Wang, Jinsheng & Lan, Christopher & He, Ian & Ko, Vivien & Ryan, David & Wigston, Andrew, 2016. "A study on the impact of SO2 on CO2 injectivity for CO2 storage in a Canadian saline aquifer," Applied Energy, Elsevier, vol. 184(C), pages 329-336.
    • Handle: RePEc:eee:appene:v:184:y:2016:i:c:p:329-336
    DOI: 10.1016/j.apenergy.2016.09.067
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    References listed on IDEAS

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    1. Ziabakhsh-Ganji, Zaman & Kooi, Henk, 2014. "Sensitivity of the CO2 storage capacity of underground geological structures to the presence of SO2 and other impurities," Applied Energy, Elsevier, vol. 135(C), pages 43-52.
    2. Wei, Ning & Li, Xiaochun & Wang, Yan & Zhu, Qianlin & Liu, Shengnan & Liu, Naizhong & Su, Xuebing, 2015. "Geochemical impact of aquifer storage for impure CO2 containing O2 and N2: Tongliao field experiment," Applied Energy, Elsevier, vol. 145(C), pages 198-210.
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    Cited by:

    1. Yang, Yu & Wang, Quanhai & Lu, Xiaofeng & Li, Jianbo & Liu, Zhuo, 2018. "Combustion behaviors and pollutant emission characteristics of low calorific oil shale and its semi-coke in a lab-scale fluidized bed combustor," Applied Energy, Elsevier, vol. 211(C), pages 631-638.
    2. You, Junyu & Ampomah, William & Sun, Qian, 2020. "Co-optimizing water-alternating-carbon dioxide injection projects using a machine learning assisted computational framework," Applied Energy, Elsevier, vol. 279(C).
    3. Fan, Jing-Li & Shen, Shuo & Wei, Shi-Jie & Xu, Mao & Zhang, Xian, 2020. "Near-term CO2 storage potential for coal-fired power plants in China: A county-level source-sink matching assessment," Applied Energy, Elsevier, vol. 279(C).
    4. Seungmo Ko & Sung-Min Kim & Hochang Jang, 2023. "A Simulation Study on Evaluating the Influence of Impurities on Hydrogen Production in Geological Carbon Dioxide Storage," Sustainability, MDPI, vol. 15(18), pages 1-19, September.
    5. Vo Thanh, Hung & Lee, Kang-Kun, 2022. "Application of machine learning to predict CO2 trapping performance in deep saline aquifers," Energy, Elsevier, vol. 239(PE).
    6. Dai, Zhenxue & Zhang, Ye & Bielicki, Jeffrey & Amooie, Mohammad Amin & Zhang, Mingkan & Yang, Changbing & Zou, Youqin & Ampomah, William & Xiao, Ting & Jia, Wei & Middleton, Richard & Zhang, Wen & Sun, 2018. "Heterogeneity-assisted carbon dioxide storage in marine sediments," Applied Energy, Elsevier, vol. 225(C), pages 876-883.
    7. Chen, Long & Xu, Guiyin & Rui, Zhenhua & Alshawabkeh, Akram N., 2019. "Demonstration of a feasible energy-water-environment nexus: Waste sulfur dioxide for water treatment," Applied Energy, Elsevier, vol. 250(C), pages 1011-1022.
    8. Ampomah, W. & Balch, R.S. & Cather, M. & Will, R. & Gunda, D. & Dai, Z. & Soltanian, M.R., 2017. "Optimum design of CO2 storage and oil recovery under geological uncertainty," Applied Energy, Elsevier, vol. 195(C), pages 80-92.

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    More about this item

    Keywords

    CO2 storage; Saline aquifer; SO2; CO2 injectivity;
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