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A numerical study of the impurity effects of nitrogen and sulfur dioxide on the solubility trapping of carbon dioxide geological storage

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  • Li, Didi
  • Jiang, Xi

Abstract

Three-dimensional numerical simulations are performed to investigate the effects of nitrogen (N2) and sulfur dioxide (SO2) impurities on the solubility trapping mechanism of carbon dioxide (CO2) geological storage. Dissolved CO2 has been suggested to increase the density of the aqueous phase. Results from this study indicate that, when dissolved in the formation water, certain level of the N2 impurity contained in the CO2 streams reduces the density increase, which is the driving force of convection. With a higher N2 concentration, the onset of convection is later and the dissolution rate is smaller. The decay time of convection for the higher N2 concentration case is also delayed. For the co-injection of CO2 and N2, total CO2 dissolved in the formation fluids is less than that of injecting CO2 alone. During the timescale of dissolution, the mobile and buoyant CO2 streams have the potential to leak through the caprock to the atmosphere. It is necessary to reinforce the risk management for safe CO2 storage for the co-injection of CO2 and N2. In contrary to N2, the SO2 impurity is implied to enhance the solubility trapping mechanism and it has more significant effects compared to N2 at the same impurity concentration.

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  • Li, Didi & Jiang, Xi, 2014. "A numerical study of the impurity effects of nitrogen and sulfur dioxide on the solubility trapping of carbon dioxide geological storage," Applied Energy, Elsevier, vol. 128(C), pages 60-74.
    • Handle: RePEc:eee:appene:v:128:y:2014:i:c:p:60-74
    DOI: 10.1016/j.apenergy.2014.04.051
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    References listed on IDEAS

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    1. Li, Hailong & Jakobsen, Jana P. & Wilhelmsen, Øivind & Yan, Jinyue, 2011. "PVTxy properties of CO2 mixtures relevant for CO2 capture, transport and storage: Review of available experimental data and theoretical models," Applied Energy, Elsevier, vol. 88(11), pages 3567-3579.
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    4. Jiang, Xi, 2011. "A review of physical modelling and numerical simulation of long-term geological storage of CO2," Applied Energy, Elsevier, vol. 88(11), pages 3557-3566.
    5. Li, H. & Yan, J., 2009. "Evaluating cubic equations of state for calculation of vapor-liquid equilibrium of CO2 and CO2-mixtures for CO2 capture and storage processes," Applied Energy, Elsevier, vol. 86(6), pages 826-836, June.
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    1. Li, Didi & He, Yao & Zhang, Hongcheng & Xu, Wenbin & Jiang, Xi, 2017. "A numerical study of the impurity effects on CO2 geological storage in layered formation," Applied Energy, Elsevier, vol. 199(C), pages 107-120.
    2. Li, Didi & Jiang, Xi, 2017. "Numerical investigation of the partitioning phenomenon of carbon dioxide and multiple impurities in deep saline aquifers," Applied Energy, Elsevier, vol. 185(P2), pages 1411-1423.
    3. Li, Didi & Zhang, Hongcheng & Li, Yang & Xu, Wenbin & Jiang, Xi, 2018. "Effects of N2 and H2S binary impurities on CO2 geological storage in stratified formation – A sensitivity study," Applied Energy, Elsevier, vol. 229(C), pages 482-492.
    4. Ziabakhsh-Ganji, Zaman & Kooi, Henk, 2014. "Sensitivity of the CO2 storage capacity of underground geological structures to the presence of SO2 and other impurities," Applied Energy, Elsevier, vol. 135(C), pages 43-52.
    5. Wei, Ning & Li, Xiaochun & Wang, Yan & Zhu, Qianlin & Liu, Shengnan & Liu, Naizhong & Su, Xuebing, 2015. "Geochemical impact of aquifer storage for impure CO2 containing O2 and N2: Tongliao field experiment," Applied Energy, Elsevier, vol. 145(C), pages 198-210.

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