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Implementation and evaluation for anode purging of a fuel cell based on nitrogen concentration

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  • Chen, Yong-Song
  • Yang, Chih-Wei
  • Lee, Jiunn-Yih

Abstract

When a proton exchange membrane fuel cell is operated in a dead-ended anode mode, its performance gradually decreases due to accumulation of nitrogen and liquid water. Many experimental studies show that nitrogen accumulation is mainly responsible for the performance drop. In this study, a dynamic mathematical model developed in our previous work is employed to predict the nitrogen accumulation in the anode and its corresponding cell voltage. The model is calibrated and validated using experimental data.

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  • Chen, Yong-Song & Yang, Chih-Wei & Lee, Jiunn-Yih, 2014. "Implementation and evaluation for anode purging of a fuel cell based on nitrogen concentration," Applied Energy, Elsevier, vol. 113(C), pages 1519-1524.
    • Handle: RePEc:eee:appene:v:113:y:2014:i:c:p:1519-1524
    DOI: 10.1016/j.apenergy.2013.09.028
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    Cited by:

    1. Wang, Bowen & Deng, Hao & Jiao, Kui, 2018. "Purge strategy optimization of proton exchange membrane fuel cell with anode recirculation," Applied Energy, Elsevier, vol. 225(C), pages 1-13.
    2. Dashti, Isar & Asghari, Saeed & Goudarzi, Mohammad & Meyer, Quentin & Mehrabani-Zeinabad, Arjomand & Brett, Dan J.L., 2019. "Optimization of the performance, operation conditions and purge rate for a dead-ended anode proton exchange membrane fuel cell using an analytical model," Energy, Elsevier, vol. 179(C), pages 173-185.
    3. Zhang, Qinguo & Tong, Zheming & Tong, Shuiguang & Cheng, Zhewu, 2021. "Modeling and dynamic performance research on proton exchange membrane fuel cell system with hydrogen cycle and dead-ended anode," Energy, Elsevier, vol. 218(C).
    4. Ruifeng Guo & Dongfang Chen & Yuehua Li & Wenlong Wu & Song Hu & Xiaoming Xu, 2023. "Anode Nitrogen Concentration Estimation Based on Voltage Variation Characteristics for Proton Exchange Membrane Fuel Cell Stacks," Energies, MDPI, vol. 16(5), pages 1-16, February.
    5. Chen, Ben & Cai, Yonghua & Tu, Zhengkai & Chan, Siew Hwa & Wang, Jun & Yu, Yi, 2017. "Gas purging effect on the degradation characteristic of a proton exchange membrane fuel cell with dead-ended mode operation I. With different electrolytes," Energy, Elsevier, vol. 141(C), pages 40-49.
    6. Alegre, Cinthia & Lozano, Antonio & Manso, Ángel Pérez & Álvarez-Manuel, Laura & Marzo, Florencio Fernández & Barreras, Félix, 2019. "Single cell induced starvation in a high temperature proton exchange membrane fuel cell stack," Applied Energy, Elsevier, vol. 250(C), pages 1176-1189.
    7. Steinberger, Michael & Geiling, Johannes & Oechsner, Richard & Frey, Lothar, 2018. "Anode recirculation and purge strategies for PEM fuel cell operation with diluted hydrogen feed gas," Applied Energy, Elsevier, vol. 232(C), pages 572-582.
    8. Zhang, Caizhi & Liu, Zhitao & Zhang, Xiongwen & Chan, Siew Hwa & Wang, Youyi, 2016. "Dynamic performance of a high-temperature PEM (proton exchange membrane) fuel cell – Modelling and fuzzy control of purging process," Energy, Elsevier, vol. 95(C), pages 425-432.
    9. Xu, Liangfei & Hu, Zunyan & Fang, Chuan & Li, Jianqiu & Hong, Po & Jiang, Hongliang & Guo, Di & Ouyang, Minggao, 2021. "Anode state observation of polymer electrolyte membrane fuel cell based on unscented Kalman filter and relative humidity sensor before flooding," Renewable Energy, Elsevier, vol. 168(C), pages 1294-1307.
    10. Bizon, Nicu, 2019. "Fuel saving strategy using real-time switching of the fueling regulators in the proton exchange membrane fuel cell system," Applied Energy, Elsevier, vol. 252(C), pages 1-1.
    11. Hou, Junbo & Yang, Min & Zhang, Junliang, 2020. "Active and passive fuel recirculation for solid oxide and proton exchange membrane fuel cells," Renewable Energy, Elsevier, vol. 155(C), pages 1355-1371.
    12. Esbo, M. Rahimi- & Ranjbar, A.A. & Rahgoshay, S.M., 2020. "Analysis of water management in PEM fuel cell stack at dead-end mode using direct visualization," Renewable Energy, Elsevier, vol. 162(C), pages 212-221.
    13. Kurnia, Jundika C. & Sasmito, Agus P. & Shamim, Tariq, 2019. "Advances in proton exchange membrane fuel cell with dead-end anode operation: A review," Applied Energy, Elsevier, vol. 252(C), pages 1-1.
    14. Yang, Chih-Wei & Chen, Yong-Song, 2014. "A mathematical model to study the performance of a proton exchange membrane fuel cell in a dead-ended anode mode," Applied Energy, Elsevier, vol. 130(C), pages 113-121.
    15. Chen, Dongfang & Pei, Pucheng & Ren, Peng & Song, Xin & Wang, He & Zhang, Lu & Wang, Mingkai, 2022. "Analytical methods for the effect of anode nitrogen concentration on performance and voltage consistency of proton exchange membrane fuel cell stack," Energy, Elsevier, vol. 258(C).
    16. Yu, Wei & Tao, Jiabo & Yu, Xinhai & Zhao, Shuangliang & Tu, Shan-Tung & Liu, Honglai, 2017. "A microreactor with superhydrophobic Pt–Al2O3 catalyst coating concerning oxidation of hydrogen off-gas from fuel cell," Applied Energy, Elsevier, vol. 185(P2), pages 1233-1244.
    17. Tsai, Shang-Wen & Chen, Yong-Song, 2017. "A mathematical model to study the energy efficiency of a proton exchange membrane fuel cell with a dead-ended anode," Applied Energy, Elsevier, vol. 188(C), pages 151-159.
    18. Chen, Ben & Ke, Wandi & Luo, Maji & Wang, Jun & Tu, Zhengkai & Pan, Mu & Zhang, Haining & Liu, Xiaowei & Liu, Wei, 2015. "Operation characteristics and carbon corrosion of PEMFC (Proton exchange membrane fuel cell) with dead-ended anode for high hydrogen utilization," Energy, Elsevier, vol. 91(C), pages 799-806.
    19. Chen, Ben & Zhou, Haoran & He, Shaowen & Meng, Kai & Liu, Yang & Cai, Yonghua, 2021. "Numerical simulation on purge strategy of proton exchange membrane fuel cell with dead-ended anode," Energy, Elsevier, vol. 234(C).
    20. Vasilyev, A. & Andrews, J. & Dunnett, S.J. & Jackson, L.M., 2021. "Dynamic Reliability Assessment of PEM Fuel Cell Systems," Reliability Engineering and System Safety, Elsevier, vol. 210(C).
    21. Liu, Zhiyang & Chen, Jian & Liu, Hao & Yan, Chizhou & Hou, Yang & He, Qinggang & Zhang, Jiujun & Hissel, Daniel, 2020. "Anode purge management for hydrogen utilization and stack durability improvement of PEM fuel cell systems," Applied Energy, Elsevier, vol. 275(C).
    22. Yang, Zirong & Du, Qing & Jia, Zhiwei & Yang, Chunguang & Xuan, Jin & Jiao, Kui, 2019. "A comprehensive proton exchange membrane fuel cell system model integrating various auxiliary subsystems," Applied Energy, Elsevier, vol. 256(C).
    23. Nicu Bizon & Phatiphat Thounthong, 2021. "A Simple and Safe Strategy for Improving the Fuel Economy of a Fuel Cell Vehicle," Mathematics, MDPI, vol. 9(6), pages 1-29, March.
    24. Myo-Eun Kim & Young-Jun Sohn, 2020. "Study on Polymer Electrolyte Fuel Cells with Nonhumidification Using Metal Foam in Dead-Ended Operation," Energies, MDPI, vol. 13(5), pages 1-12, March.

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