IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v16y2025i1d10.1038_s41467-025-59287-z.html
   My bibliography  Save this article

Spin detector for panchromatic circularly polarized light detection

Author

Listed:
  • Lvpeng Yang

    (Huazhong University of Science and Technology)

  • Yerun Gao

    (Huazhong University of Science and Technology)

  • Zhenye Wang

    (Huazhong University of Science and Technology)

  • Long Yang

    (Huazhong University of Science and Technology)

  • Ming Shao

    (Huazhong University of Science and Technology)

Abstract

Circularly polarized light (CPL) detection is crucial for optical communication, bioimaging and quantum computing. However, CPL detectors based on chiral low-dimensional perovskites face a trade-off between optoelectronic performance and CPL discrimination, and typically exhibit a CPL response within a narrow spectral range. Here, we overcome these limitations by integrating three-dimensional (3D) and chiral-two-dimensional (2D) perovskites. The 3D perovskite serving as the photoabsorption layer extends the detection range to 760 nm and enhances optoelectronic responses, while also generating spin-polarized carriers through large Rashba splitting. The chiral-2D perovskite achieves spin filtering efficiency up to 80%. The synergy between spin polarization and chiral-induced spin selectivity processes enables a panchromatic CPL response, with a photocurrent asymmetry factor exceeding 0.28 across the visible spectrum and peaking at 0.35. Furthermore, our detector achieves a detectivity of 3.7×1011 Jones. Our work introduces a spin manipulation strategy for panchromatic CPL detection, expanding the scope of spintronics applications.

Suggested Citation

  • Lvpeng Yang & Yerun Gao & Zhenye Wang & Long Yang & Ming Shao, 2025. "Spin detector for panchromatic circularly polarized light detection," Nature Communications, Nature, vol. 16(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:16:y:2025:i:1:d:10.1038_s41467-025-59287-z
    DOI: 10.1038/s41467-025-59287-z
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-025-59287-z
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-025-59287-z?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Qi Qian & Huaying Ren & Jingyuan Zhou & Zhong Wan & Jingxuan Zhou & Xingxu Yan & Jin Cai & Peiqi Wang & Bailing Li & Zdenek Sofer & Bo Li & Xidong Duan & Xiaoqing Pan & Yu Huang & Xiangfeng Duan, 2022. "Chiral molecular intercalation superlattices," Nature, Nature, vol. 606(7916), pages 902-908, June.
    2. Xiaojie Liu & Ashish Chanana & Uyen Huynh & Fei Xue & Paul Haney & Steve Blair & Xiaomei Jiang & Z. V. Vardeny, 2020. "Circular photogalvanic spectroscopy of Rashba splitting in 2D hybrid organic–inorganic perovskite multiple quantum wells," Nature Communications, Nature, vol. 11(1), pages 1-8, December.
    3. Jaewang Park & Jongbeom Kim & Hyun-Sung Yun & Min Jae Paik & Eunseo Noh & Hyun Jung Mun & Min Gyu Kim & Tae Joo Shin & Sang Il Seok, 2023. "Controlled growth of perovskite layers with volatile alkylammonium chlorides," Nature, Nature, vol. 616(7958), pages 724-730, April.
    4. Jingying Wang & Chuang Zhang & Haoliang Liu & Ryan McLaughlin & Yaxin Zhai & Shai R. Vardeny & Xiaojie Liu & Stephen McGill & Dmitry Semenov & Hangwen Guo & Ryuichi Tsuchikawa & Vikram V. Deshpande & , 2019. "Spin-optoelectronic devices based on hybrid organic-inorganic trihalide perovskites," Nature Communications, Nature, vol. 10(1), pages 1-6, December.
    5. E. Togan & Y. Chu & A. S. Trifonov & L. Jiang & J. Maze & L. Childress & M. V. G. Dutt & A. S. Sørensen & P. R. Hemmer & A. S. Zibrov & M. D. Lukin, 2010. "Quantum entanglement between an optical photon and a solid-state spin qubit," Nature, Nature, vol. 466(7307), pages 730-734, August.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Bogdan Dryzhakov & Yipeng Tang & Jong Keum & Haile Ambaye & Jinwoo Kim & Tae-Woo Lee & Valeria Lauter & Bin Hu, 2025. "Spin switchable optical phenomena in Rashba band structures through intersystem crossing in momentum space in solution-processing 2D-superlattice perovskite film," Nature Communications, Nature, vol. 16(1), pages 1-10, December.
    2. M. Michiardi & F. Boschini & H.-H. Kung & M. X. Na & S. K. Y. Dufresne & A. Currie & G. Levy & S. Zhdanovich & A. K. Mills & D. J. Jones & J. L. Mi & B. B. Iversen & Ph. Hofmann & A. Damascelli, 2022. "Optical manipulation of Rashba-split 2-dimensional electron gas," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    3. Weilun Li & Mengmeng Hao & Ardeshir Baktash & Lianzhou Wang & Joanne Etheridge, 2023. "The role of ion migration, octahedral tilt, and the A-site cation on the instability of Cs1-xFAxPbI3," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    4. Bingcheng Yu & Jiangjian Shi & Yiming Li & Shan Tan & Yuqi Cui & Fanqi Meng & Huijue Wu & Yanhong Luo & Dongmei Li & Qingbo Meng, 2025. "Regulating three-layer full carbon electrodes to enhance the cell performance of CsPbI3 perovskite solar cells," Nature Communications, Nature, vol. 16(1), pages 1-10, December.
    5. Meng-Hsueh Kuo & Neda Neykova & Ivo Stachiv, 2024. "Overview of the Recent Findings in the Perovskite-Type Structures Used for Solar Cells and Hydrogen Storage," Energies, MDPI, vol. 17(18), pages 1-23, September.
    6. Xue-Guang Chen & Linhan Lin & Guan-Yao Huang & Xiao-Mei Chen & Xiao-Ze Li & Yun-Ke Zhou & Yixuan Zou & Tairan Fu & Peng Li & Zhengcao Li & Hong-Bo Sun, 2024. "Optofluidic crystallithography for directed growth of single-crystalline halide perovskites," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    7. Yuhang Liang & Feng Li & Xiangyuan Cui & Taoyuze Lv & Catherine Stampfl & Simon P. Ringer & Xudong Yang & Jun Huang & Rongkun Zheng, 2024. "Toward stabilization of formamidinium lead iodide perovskites by defect control and composition engineering," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    8. Tianpeng Li & Bin Li & Yingguo Yang & Zuoming Jin & Zhiguo Zhang & Peilin Wang & Liangliang Deng & Yiqiang Zhan & Qinghong Zhang & Jia Liang, 2024. "Metal chalcogenide electron extraction layers for nip-type tin-based perovskite solar cells," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    9. Shuxian Du & Hao Huang & Zhineng Lan & Peng Cui & Liang Li & Min Wang & Shujie Qu & Luyao Yan & Changxu Sun & Yingying Yang & Xinxin Wang & Meicheng Li, 2024. "Inhibiting perovskite decomposition by a creeper-inspired strategy enables efficient and stable perovskite solar cells," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    10. Łukasz Dusanowski & Cornelius Nawrath & Simone L. Portalupi & Michael Jetter & Tobias Huber & Sebastian Klembt & Peter Michler & Sven Höfling, 2022. "Optical charge injection and coherent control of a quantum-dot spin-qubit emitting at telecom wavelengths," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    11. Anil-Kumar Singh & Kévin Martin & Maurizio Mastropasqua Talamo & Axel Houssin & Nicolas Vanthuyne & Narcis Avarvari & Oren Tal, 2025. "Single-molecule junctions map the interplay between electrons and chirality," Nature Communications, Nature, vol. 16(1), pages 1-9, December.
    12. Jiangang Feng & Xi Wang & Jia Li & Haoming Liang & Wen Wen & Ezra Alvianto & Cheng-Wei Qiu & Rui Su & Yi Hou, 2023. "Resonant perovskite solar cells with extended band edge," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    13. Jin Zhou & Shiqiang Fu & Shun Zhou & Lishuai Huang & Cheng Wang & Hongling Guan & Dexin Pu & Hongsen Cui & Chen Wang & Ti Wang & Weiwei Meng & Guojia Fang & Weijun Ke, 2024. "Mixed tin-lead perovskites with balanced crystallization and oxidation barrier for all-perovskite tandem solar cells," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    14. Xia Wang & Qun Yang & Sukriti Singh & Horst Borrmann & Vicky Hasse & Changjiang Yi & Yongkang Li & Marcus Schmidt & Xiaodong Li & Gerhard H. Fecher & Dong Zhou & Binghai Yan & Claudia Felser, 2025. "Topological semimetals with intrinsic chirality as spin-controlling electrocatalysts for the oxygen evolution reaction," Nature Energy, Nature, vol. 10(1), pages 101-109, January.
    15. Yongjin Gan & Guixin Qiu & Chenqing Yan & Zhaoxiang Zeng & Binyi Qin & Xueguang Bi & Yucheng Liu, 2023. "Numerical Analysis on the Effect of the Conduction Band Offset in Dion–Jacobson Perovskite Solar Cells," Energies, MDPI, vol. 16(23), pages 1-13, December.
    16. Tian Chen & Jiangsheng Xie & Bin Wen & Qixin Yin & Ruohao Lin & Shengcai Zhu & Pingqi Gao, 2023. "Inhibition of defect-induced α-to-δ phase transition for efficient and stable formamidinium perovskite solar cells," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    17. Nikhil Mathur & Arunabh Mukherjee & Xingyu Gao & Jialun Luo & Brendan A. McCullian & Tongcang Li & A. Nick Vamivakas & Gregory D. Fuchs, 2022. "Excited-state spin-resonance spectroscopy of V $${}_{{{{{{{{\rm{B}}}}}}}}}^{-}$$ B − defect centers in hexagonal boron nitride," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    18. Haozhe Yang & Eva Schmoranzerová & Pyunghwa Jang & Jayshankar Nath & Thomas Guillet & Isabelle Joumard & Stéphane Auffret & Matthieu Jamet & Petr Němec & Gilles Gaudin & Ioan-Mihai Miron, 2022. "Helicity dependent photoresistance measurement vs. beam-shift thermal gradient," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    19. Sandhya Susarla & Shanglin Hsu & Fernando Gómez-Ortiz & Pablo García-Fernández & Benjamin H. Savitzky & Sujit Das & Piush Behera & Javier Junquera & Peter Ercius & Ramamoorthy Ramesh & Colin Ophus, 2023. "The emergence of three-dimensional chiral domain walls in polar vortices," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
    20. Likai Yang & Sihao Wang & Mohan Shen & Jiacheng Xie & Hong X. Tang, 2023. "Controlling single rare earth ion emission in an electro-optical nanocavity," Nature Communications, Nature, vol. 14(1), pages 1-6, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:16:y:2025:i:1:d:10.1038_s41467-025-59287-z. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.