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Higher order gaps in the renormalized band structure of doubly aligned hBN/bilayer graphene moiré superlattice

Author

Listed:
  • Mohit Kumar Jat

    (Indian Institute of Science)

  • Priya Tiwari

    (Department of Condensed Matter Physics, Weizmann Institute of Science)

  • Robin Bajaj

    (Indian Institute of Science)

  • Ishita Shitut

    (Indian Institute of Science)

  • Shinjan Mandal

    (Indian Institute of Science)

  • Kenji Watanabe

    (National Institute for Materials Science)

  • Takashi Taniguchi

    (National Institute for Materials Science)

  • H. R. Krishnamurthy

    (Indian Institute of Science)

  • Manish Jain

    (Indian Institute of Science)

  • Aveek Bid

    (Indian Institute of Science)

Abstract

This paper presents our findings on the recursive band gap engineering of chiral fermions in bilayer graphene doubly aligned with hBN. Using two interfering moiré potentials, we generate a supermoiré pattern that renormalizes the electronic bands of the pristine bilayer graphene, resulting in higher order fractal gaps even at very low energies. These Bragg gaps can be mapped using a unique linear combination of periodic areas within the system. To validate our findings, we use electronic transport measurements to identify the position of these gaps as a function of the carrier density. We establish their agreement with the predicted carrier densities and corresponding quantum numbers obtained using the continuum model. Our study provides strong evidence of the quantization of the momentum-space area of quasi-Brillouin zones in a minimally incommensurate lattice. It fills important gaps in the understanding of band structure engineering of Dirac fermions with a doubly periodic superlattice spinor potential.

Suggested Citation

  • Mohit Kumar Jat & Priya Tiwari & Robin Bajaj & Ishita Shitut & Shinjan Mandal & Kenji Watanabe & Takashi Taniguchi & H. R. Krishnamurthy & Manish Jain & Aveek Bid, 2024. "Higher order gaps in the renormalized band structure of doubly aligned hBN/bilayer graphene moiré superlattice," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-46672-3
    DOI: 10.1038/s41467-024-46672-3
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    as
    1. L. A. Ponomarenko & R. V. Gorbachev & G. L. Yu & D. C. Elias & R. Jalil & A. A. Patel & A. Mishchenko & A. S. Mayorov & C. R. Woods & J. R. Wallbank & M. Mucha-Kruczynski & B. A. Piot & M. Potemski & , 2013. "Cloning of Dirac fermions in graphene superlattices," Nature, Nature, vol. 497(7451), pages 594-597, May.
    2. Filippo Pizzocchero & Lene Gammelgaard & Bjarke S. Jessen & José M. Caridad & Lei Wang & James Hone & Peter Bøggild & Timothy J. Booth, 2016. "The hot pick-up technique for batch assembly of van der Waals heterostructures," Nature Communications, Nature, vol. 7(1), pages 1-10, September.
    3. Rai Moriya & Kei Kinoshita & J. A. Crosse & Kenji Watanabe & Takashi Taniguchi & Satoru Masubuchi & Pilkyung Moon & Mikito Koshino & Tomoki Machida, 2020. "Emergence of orbital angular moment at van Hove singularity in graphene/h-BN moiré superlattice," Nature Communications, Nature, vol. 11(1), pages 1-6, December.
    4. Robin Huber & Max-Niklas Steffen & Martin Drienovsky & Andreas Sandner & Kenji Watanabe & Takashi Taniguchi & Daniela Pfannkuche & Dieter Weiss & Jonathan Eroms, 2022. "Band conductivity oscillations in a gate-tunable graphene superlattice," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    5. C. R. Dean & L. Wang & P. Maher & C. Forsythe & F. Ghahari & Y. Gao & J. Katoch & M. Ishigami & P. Moon & M. Koshino & T. Taniguchi & K. Watanabe & K. L. Shepard & J. Hone & P. Kim, 2013. "Hofstadter’s butterfly and the fractal quantum Hall effect in moiré superlattices," Nature, Nature, vol. 497(7451), pages 598-602, May.
    6. Julien Barrier & Piranavan Kumaravadivel & Roshan Krishna Kumar & L. A. Ponomarenko & Na Xin & Matthew Holwill & Ciaran Mullan & Minsoo Kim & R. V. Gorbachev & M. D. Thompson & J. R. Prance & T. Tanig, 2020. "Long-range ballistic transport of Brown-Zak fermions in graphene superlattices," Nature Communications, Nature, vol. 11(1), pages 1-7, December.
    7. Guorui Chen & Aaron L. Sharpe & Eli J. Fox & Ya-Hui Zhang & Shaoxin Wang & Lili Jiang & Bosai Lyu & Hongyuan Li & Kenji Watanabe & Takashi Taniguchi & Zhiwen Shi & T. Senthil & David Goldhaber-Gordon , 2020. "Publisher Correction: Tunable correlated Chern insulator and ferromagnetism in a moiré superlattice," Nature, Nature, vol. 581(7807), pages 3-3, May.
    8. Guorui Chen & Aaron L. Sharpe & Eli J. Fox & Ya-Hui Zhang & Shaoxin Wang & Lili Jiang & Bosai Lyu & Hongyuan Li & Kenji Watanabe & Takashi Taniguchi & Zhiwen Shi & T. Senthil & David Goldhaber-Gordon , 2020. "Tunable correlated Chern insulator and ferromagnetism in a moiré superlattice," Nature, Nature, vol. 579(7797), pages 56-61, March.
    9. Matthew Yankowitz & K. Watanabe & T. Taniguchi & Pablo San-Jose & Brian J. LeRoy, 2016. "Pressure-induced commensurate stacking of graphene on boron nitride," Nature Communications, Nature, vol. 7(1), pages 1-8, December.
    10. Xingdan Sun & Shihao Zhang & Zhiyong Liu & Honglei Zhu & Jinqiang Huang & Kai Yuan & Zhenhua Wang & Kenji Watanabe & Takashi Taniguchi & Xiaoxi Li & Mengjian Zhu & Jinhai Mao & Teng Yang & Jun Kang & , 2021. "Correlated states in doubly-aligned hBN/graphene/hBN heterostructures," Nature Communications, Nature, vol. 12(1), pages 1-8, December.
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