IDEAS home Printed from https://ideas.repec.org/a/nat/natcom/v14y2023i1d10.1038_s41467-023-39791-w.html
   My bibliography  Save this article

2D MXenes polar catalysts for multi-renewable energy harvesting applications

Author

Listed:
  • Xiaoyang Pan

    (Quanzhou Normal University)

  • Xuhui Yang

    (Fujian Normal University)

  • Maoqing Yu

    (Quanzhou Normal University
    National Engineering Research Center of Chemical Fertilizer Catalyst Fuzhou University)

  • Xiaoxiao Lu

    (Quanzhou Normal University
    Fujian Normal University)

  • Hao Kang

    (Fujian Normal University)

  • Min-Quan Yang

    (Fujian Normal University)

  • Qingrong Qian

    (Fujian Normal University)

  • Xiaojing Zhao

    (Quanzhou Normal University)

  • Shijing Liang

    (National Engineering Research Center of Chemical Fertilizer Catalyst Fuzhou University)

  • Zhenfeng Bian

    (Shanghai Normal University)

Abstract

The synchronous harvesting and conversion of multiple renewable energy sources for chemical fuel production and environmental remediation in a single system is a holy grail in sustainable energy technologies. However, it is challenging to develop advanced energy harvesters that satisfy different working mechanisms. Here, we theoretically and experimentally disclose the use of MXene materials as versatile catalysts for multi-energy utilization. Ti3C2TX MXene shows remarkable catalytic performance for organic pollutant decomposition and H2 production. It outperforms most reported catalysts under the stimulation of light, thermal, and mechanical energy. Moreover, the synergistic effects of piezo-thermal and piezo-photothermal catalysis further improve the performance when using Ti3C2TX. A mechanistic study reveals that hydroxyl and superoxide radicals are produced on the Ti3C2TX under diverse energy stimulation. Furthermore, similar multi-functionality is realized in Ti2CTX, V2CTX, and Nb2CTX MXene materials. This work is anticipated to open a new avenue for multisource renewable energy harvesting using MXene materials.

Suggested Citation

  • Xiaoyang Pan & Xuhui Yang & Maoqing Yu & Xiaoxiao Lu & Hao Kang & Min-Quan Yang & Qingrong Qian & Xiaojing Zhao & Shijing Liang & Zhenfeng Bian, 2023. "2D MXenes polar catalysts for multi-renewable energy harvesting applications," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-39791-w
    DOI: 10.1038/s41467-023-39791-w
    as

    Download full text from publisher

    File URL: https://www.nature.com/articles/s41467-023-39791-w
    File Function: Abstract
    Download Restriction: no

    File URL: https://libkey.io/10.1038/s41467-023-39791-w?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    References listed on IDEAS

    as
    1. Li Ding & Libo Li & Yanchang Liu & Yi Wu & Zong Lu & Junjie Deng & Yanying Wei & Jürgen Caro & Haihui Wang, 2020. "Effective ion sieving with Ti3C2Tx MXene membranes for production of drinking water from seawater," Nature Sustainability, Nature, vol. 3(4), pages 296-302, April.
    2. Huilin You & Yanmin Jia & Zheng Wu & Feifei Wang & Haitao Huang & Yu Wang, 2018. "Room-temperature pyro-catalytic hydrogen generation of 2D few-layer black phosphorene under cold-hot alternation," Nature Communications, Nature, vol. 9(1), pages 1-8, December.
    3. Lingbo Xiao & Xiaoli Xu & Yanmin Jia & Ge Hu & Jun Hu & Biao Yuan & Yi Yu & Guifu Zou, 2021. "Author Correction: Pyroelectric nanoplates for reduction of CO2 to methanol driven by temperature-variation," Nature Communications, Nature, vol. 12(1), pages 1-1, December.
    4. Yanan Ma & Nishuang Liu & Luying Li & Xiaokang Hu & Zhengguang Zou & Jianbo Wang & Shijun Luo & Yihua Gao, 2017. "A highly flexible and sensitive piezoresistive sensor based on MXene with greatly changed interlayer distances," Nature Communications, Nature, vol. 8(1), pages 1-8, December.
    5. Yang Wang & Xinrong Wen & Yanmin Jia & Ming Huang & Feifei Wang & Xuehui Zhang & Yunyang Bai & Guoliang Yuan & Yaojin Wang, 2020. "Piezo-catalysis for nondestructive tooth whitening," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    6. Lingbo Xiao & Xiaoli Xu & Yanmin Jia & Ge Hu & Jun Hu & Biao Yuan & Yi Yu & Guifu Zou, 2021. "Pyroelectric nanoplates for reduction of CO2 to methanol driven by temperature-variation," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    7. Tingting Hou & Qiquan Luo & Qi Li & Hualu Zu & Peixin Cui & Siwei Chen & Yue Lin & Jiajia Chen & Xusheng Zheng & Wenkun Zhu & Shuquan Liang & Jinlong Yang & Liangbing Wang, 2020. "Modulating oxygen coverage of Ti3C2Tx MXenes to boost catalytic activity for HCOOH dehydrogenation," Nature Communications, Nature, vol. 11(1), pages 1-11, December.
    8. Yu-Jiung Lin & Imran Khan & Subhajit Saha & Chih-Cheng Wu & Snigdha Roy Barman & Fu-Cheng Kao & Zong-Hong Lin, 2021. "Thermocatalytic hydrogen peroxide generation and environmental disinfection by Bi2Te3 nanoplates," Nature Communications, Nature, vol. 12(1), pages 1-11, December.
    9. Jianfang Li & Zhaoyang Li & Xiangmei Liu & Changyi Li & Yufeng Zheng & Kelvin Wai Kwok Yeung & Zhenduo Cui & Yanqin Liang & Shengli Zhu & Wenbin Hu & Yajun Qi & Tianjin Zhang & Xianbao Wang & Shuilin , 2021. "Interfacial engineering of Bi2S3/Ti3C2Tx MXene based on work function for rapid photo-excited bacteria-killing," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Yang Wang & Shuhao Wang & Yanze Meng & Zhen Liu & Dijie Li & Yunyang Bai & Guoliang Yuan & Yaojin Wang & Xuehui Zhang & Xiaoguang Li & Xuliang Deng, 2022. "Pyro-catalysis for tooth whitening via oral temperature fluctuation," Nature Communications, Nature, vol. 13(1), pages 1-13, December.
    2. Huilin You & Siqi Li & Yulong Fan & Xuyun Guo & Zezhou Lin & Ran Ding & Xin Cheng & Hao Zhang & Tsz Woon Benedict Lo & Jianhua Hao & Ye Zhu & Hwa-Yaw Tam & Dangyuan Lei & Chi-Hang Lam & Haitao Huang, 2022. "Accelerated pyro-catalytic hydrogen production enabled by plasmonic local heating of Au on pyroelectric BaTiO3 nanoparticles," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    3. Yuqian Qiao & Yingde Xu & Xiangmei Liu & Yufeng Zheng & Bo Li & Yong Han & Zhaoyang Li & Kelvin Wai Kwok Yeung & Yanqin Liang & Shengli Zhu & Zhenduo Cui & Shuilin Wu, 2022. "Microwave assisted antibacterial action of Garcinia nanoparticles on Gram-negative bacteria," Nature Communications, Nature, vol. 13(1), pages 1-13, December.
    4. Zhuomin Zhang & Xuemu Li & Zehua Peng & Xiaodong Yan & Shiyuan Liu & Ying Hong & Yao Shan & Xiaote Xu & Lihan Jin & Bingren Liu & Xinyu Zhang & Yu Chai & Shujun Zhang & Alex K.-Y. Jen & Zhengbao Yang, 2023. "Active self-assembly of piezoelectric biomolecular films via synergistic nanoconfinement and in-situ poling," Nature Communications, Nature, vol. 14(1), pages 1-11, December.
    5. Qian Zhang & Bo Gao & Ling Zhang & Xiaopeng Liu & Jixiang Cui & Yijun Cao & Hongbo Zeng & Qun Xu & Xinwei Cui & Lei Jiang, 2023. "Anomalous water molecular gating from atomic-scale graphene capillaries for precise and ultrafast molecular sieving," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    6. Jaeho Yoon & Hanhwi Jang & Min-Wook Oh & Thomas Hilberath & Frank Hollmann & Yeon Sik Jung & Chan Beum Park, 2022. "Heat-fueled enzymatic cascade for selective oxyfunctionalization of hydrocarbons," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    7. Wang, Hao & Li, Xiaoke & Luo, Boqiu & Wei, Ke & Zeng, Guangyong, 2021. "The MXene/water nanofluids with high stability and photo-thermal conversion for direct absorption solar collectors: A comparative study," Energy, Elsevier, vol. 227(C).
    8. Kecheng Guan & Yanan Guo & Zhan Li & Yuandong Jia & Qin Shen & Keizo Nakagawa & Tomohisa Yoshioka & Gongping Liu & Wanqin Jin & Hideto Matsuyama, 2023. "Deformation constraints of graphene oxide nanochannels under reverse osmosis," Nature Communications, Nature, vol. 14(1), pages 1-12, December.
    9. Yong Kang & Zhuo Mao & Ying Wang & Chao Pan & Meitong Ou & Hanjie Zhang & Weiwei Zeng & Xiaoyuan Ji, 2022. "Design of a two-dimensional interplanar heterojunction for catalytic cancer therapy," Nature Communications, Nature, vol. 13(1), pages 1-20, December.
    10. Li, Zhijing & Lei, Hui & Mu, Zijun & Zhang, Yuan & Zhang, Jingquan & Zhou, Yigang & Xie, Huaqing & Yu, Wei, 2022. "Reduced graphene oxide composite fiber for solar-driven evaporation and seawater desalination," Renewable Energy, Elsevier, vol. 191(C), pages 932-942.
    11. Yuan Kang & Ting Hu & Yuqi Wang & Kaiqiang He & Zhuyuan Wang & Yvonne Hora & Wang Zhao & Rongming Xu & Yu Chen & Zongli Xie & Huanting Wang & Qinfen Gu & Xiwang Zhang, 2023. "Nanoconfinement enabled non-covalently decorated MXene membranes for ion-sieving," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    12. Jihyun Baek & Qiu Jin & Nathan Scott Johnson & Yue Jiang & Rui Ning & Apurva Mehta & Samira Siahrostami & Xiaolin Zheng, 2022. "Discovery of LaAlO3 as an efficient catalyst for two-electron water electrolysis towards hydrogen peroxide," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    13. Rezakazemi, Mashallah & Arabi Shamsabadi, Ahmad & Lin, Haiqing & Luis, Patricia & Ramakrishna, Seeram & Aminabhavi, Tejraj M., 2021. "Sustainable MXenes-based membranes for highly energy-efficient separations," Renewable and Sustainable Energy Reviews, Elsevier, vol. 143(C).
    14. Ziming Wang & Andy Berbille & Yawei Feng & Site Li & Laipan Zhu & Wei Tang & Zhong Lin Wang, 2022. "Contact-electro-catalysis for the degradation of organic pollutants using pristine dielectric powders," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    15. Rongming Xu & Yuan Kang & Weiming Zhang & Bingcai Pan & Xiwang Zhang, 2023. "Two-dimensional MXene membranes with biomimetic sub-nanochannels for enhanced cation sieving," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    16. Wang, Chengbing & Li, Wei & Li, Zhengtong & Fang, Baizeng, 2020. "Solar thermal harvesting based on self-doped nanocermet: Structural merits, design strategies and applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 134(C).
    17. Xinlei Shi & Xiangqian Fan & Yinbo Zhu & Yang Liu & Peiqi Wu & Renhui Jiang & Bao Wu & Heng-An Wu & He Zheng & Jianbo Wang & Xinyi Ji & Yongsheng Chen & Jiajie Liang, 2022. "Pushing detectability and sensitivity for subtle force to new limits with shrinkable nanochannel structured aerogel," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    18. Rui Ge & Qiuhong Yu & Feng Zhou & Shuhai Liu & Yong Qin, 2023. "Dual-modal piezotronic transistor for highly sensitive vertical force sensing and lateral strain sensing," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    19. Yanzhang Li & Hongyu Wang & Yan Li & Huan Ye & Yanan Zhang & Rongzhang Yin & Haoning Jia & Bingxu Hou & Changqiu Wang & Hongrui Ding & Xiangzhi Bai & Anhuai Lu, 2023. "Electron transfer rules of minerals under pressure informed by machine learning," Nature Communications, Nature, vol. 14(1), pages 1-10, December.
    20. Hong-chao Li & Qiang Wan & Congcong Du & Jiafei Zhao & Fumin Li & Ying Zhang & Yanping Zheng & Mingshu Chen & Kelvin H. L. Zhang & Jianyu Huang & Gang Fu & Sen Lin & Xiaoqing Huang & Haifeng Xiong, 2022. "Layered Pd oxide on PdSn nanowires for boosting direct H2O2 synthesis," Nature Communications, Nature, vol. 13(1), pages 1-10, December.

    More about this item

    Statistics

    Access and download statistics

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-39791-w. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Sonal Shukla or Springer Nature Abstracting and Indexing (email available below). General contact details of provider: http://www.nature.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.