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Quantum nonlinear spectroscopy of single nuclear spins

Author

Listed:
  • Jonas Meinel

    (University of Stuttgart
    Max Planck Institute for Solid State Research)

  • Vadim Vorobyov

    (University of Stuttgart)

  • Ping Wang

    (The Chinese University of Hong Kong
    Beijing Normal University)

  • Boris Yavkin

    (University of Stuttgart)

  • Mathias Pfender

    (University of Stuttgart)

  • Hitoshi Sumiya

    (Sumitomo Electric Industries, Ltd.)

  • Shinobu Onoda

    (National Institutes for Quantum and Radiological Science and Technology)

  • Junichi Isoya

    (University of Tsukuba)

  • Ren-Bao Liu

    (The Chinese University of Hong Kong)

  • J. Wrachtrup

    (University of Stuttgart
    Max Planck Institute for Solid State Research)

Abstract

Conventional nonlinear spectroscopy, which use classical probes, can only access a limited set of correlations in a quantum system. Here we demonstrate that quantum nonlinear spectroscopy, in which a quantum sensor and a quantum object are first entangled and the sensor is measured along a chosen basis, can extract arbitrary types and orders of correlations in a quantum system. We measured fourth-order correlations of single nuclear spins that cannot be measured in conventional nonlinear spectroscopy, using sequential weak measurement via a nitrogen-vacancy center in diamond. The quantum nonlinear spectroscopy provides fingerprint features to identify different types of objects, such as Gaussian noises, random-phased AC fields, and quantum spins, which would be indistinguishable in second-order correlations. This work constitutes an initial step toward the application of higher-order correlations to quantum sensing, to examining the quantum foundation (by, e.g., higher-order Leggett-Garg inequality), and to studying quantum many-body physics.

Suggested Citation

  • Jonas Meinel & Vadim Vorobyov & Ping Wang & Boris Yavkin & Mathias Pfender & Hitoshi Sumiya & Shinobu Onoda & Junichi Isoya & Ren-Bao Liu & J. Wrachtrup, 2022. "Quantum nonlinear spectroscopy of single nuclear spins," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32610-8
    DOI: 10.1038/s41467-022-32610-8
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    References listed on IDEAS

    as
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