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Light helicity detector based on 2D magnetic semiconductor CrI3

Author

Listed:
  • Xing Cheng

    (Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Zhixuan Cheng

    (Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Cong Wang

    (Renmin University of China)

  • Minglai Li

    (Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Pingfan Gu

    (Peking University
    Collaborative Innovation Center of Quantum Matter)

  • Shiqi Yang

    (Peking University)

  • Yanping Li

    (Peking University)

  • Kenji Watanabe

    (National Institute for Materials Science, 1-1 Namiki)

  • Takashi Taniguchi

    (National Institute for Materials Science, 1-1 Namiki)

  • Wei Ji

    (Renmin University of China)

  • Lun Dai

    (Peking University
    Collaborative Innovation Center of Quantum Matter
    Peking University Yangtze Delta Institute of Optoelectronics)

Abstract

Two-dimensional magnetic semiconductors provide a platform for studying physical phenomena at atomically thin limit, and promise magneto-optoelectronic devices application. Here, we report light helicity detectors based on graphene-CrI3-graphene vdW heterostructures. We investigate the circularly polarized light excited current and reflective magnetic circular dichroism (RMCD) under various magnetic fields in both monolayer and multilayer CrI3 devices. The devices exhibit clear helicity-selective photoresponse behavior determined by the magnetic state of CrI3. We also find abnormal negative photocurrents at higher bias in both monolayer and multilayer CrI3. A possible explanation is proposed for this phenomenon. Our work reveals the interplay between magnetic and optoelectronic properties in CrI3 and paves the way to developing spin-optoelectronic devices.

Suggested Citation

  • Xing Cheng & Zhixuan Cheng & Cong Wang & Minglai Li & Pingfan Gu & Shiqi Yang & Yanping Li & Kenji Watanabe & Takashi Taniguchi & Wei Ji & Lun Dai, 2021. "Light helicity detector based on 2D magnetic semiconductor CrI3," Nature Communications, Nature, vol. 12(1), pages 1-6, December.
  • Handle: RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-27218-3
    DOI: 10.1038/s41467-021-27218-3
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    References listed on IDEAS

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    1. Shuangzan Lu & Deping Guo & Zhengbo Cheng & Yanping Guo & Cong Wang & Jinghao Deng & Yusong Bai & Cheng Tian & Linwei Zhou & Youguo Shi & Jun He & Wei Ji & Chendong Zhang, 2023. "Controllable dimensionality conversion between 1D and 2D CrCl3 magnetic nanostructures," Nature Communications, Nature, vol. 14(1), pages 1-8, December.

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