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Effect of Ca-based additives on the capture of SO2 during combustion of pulverized lignite

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  • Zacharczuk, Wojciech
  • Andruszkiewicz, Artur
  • Tatarek, Andrzej
  • Alahmer, Ali
  • Alsaqoor, Sameh

Abstract

The effect of different Ca-based additives in lignite on the sulfur removal during combustion has been examined using two Polish lignites. After demineralization, the lignite was loaded with Ca using different Ca-based compounds namely: calcium carbonate (CaCO3), calcium hydroxide Ca(OH)2 and calcium acetate Ca(CH3COO)2. Depending on the calcium compound used, the addition of Ca was by mechanical mixing or impregnation. The experiment was carried out in a laboratory scale drop-tube furnace reactor, under different O2 concentration and temperature range of 800–1100 °C. The results showed that Ca added to the lignite strongly suppressed the emission of SO2 under experimental conditions studied. The sulfur capture efficiency appeared to be independent of the calcium compound used and it increased along with the temperature rising up to 1100 °C. This may indicate that poorly dispersed Ca, prepared by mechanical mixing, offers as high efficiency in sulfur removal as Ca in ion-exchangeable form inserted by impregnation. The influence of mineral matter on the retention of SO2 during combustion was also investigated. It was found that some inorganic species inherently present in lignite, particularly calcium in natural form, reduce SO2 pollution.

Suggested Citation

  • Zacharczuk, Wojciech & Andruszkiewicz, Artur & Tatarek, Andrzej & Alahmer, Ali & Alsaqoor, Sameh, 2021. "Effect of Ca-based additives on the capture of SO2 during combustion of pulverized lignite," Energy, Elsevier, vol. 231(C).
    • Handle: RePEc:eee:energy:v:231:y:2021:i:c:s0360544221012366
    DOI: 10.1016/j.energy.2021.120988
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    1. Capellán-Pérez, Iñigo & Mediavilla, Margarita & de Castro, Carlos & Carpintero, Óscar & Miguel, Luis Javier, 2014. "Fossil fuel depletion and socio-economic scenarios: An integrated approach," Energy, Elsevier, vol. 77(C), pages 641-666.
    2. Li, Zixiang & Miao, Zhengqing & Shen, Xusheng & Li, Jiangtao, 2018. "Effects of momentum ratio and velocity difference on combustion performance in lignite-fired pulverized boiler," Energy, Elsevier, vol. 165(PA), pages 825-839.
    3. Taseska, V. & Markovska, N. & Causevski, A. & Bosevski, T. & Pop-Jordanov, J., 2011. "Greenhouse gases (GHG) emissions reduction in a power system predominantly based on lignite," Energy, Elsevier, vol. 36(4), pages 2266-2270.
    4. Kayahan, Ufuk & Özdoğan, Sibel, 2016. "Oxygen enriched combustion and co-combustion of lignites and biomass in a 30 kWth circulating fluidized bed," Energy, Elsevier, vol. 116(P1), pages 317-328.
    5. Li, Zixiang & Miao, Zhengqing, 2019. "Primary air ratio affects coal utilization mode and NOx emission in lignite pulverized boiler," Energy, Elsevier, vol. 187(C).
    6. Lasek, Janusz A. & Kopczyński, Marcin & Janusz, Marcin & Iluk, Andrzej & Zuwała, Jarosław, 2017. "Combustion properties of torrefied biomass obtained from flue gas-enhanced reactor," Energy, Elsevier, vol. 119(C), pages 362-368.
    7. Qi, Jianhui & Han, Kuihua & Wang, Qian & Gao, Jie, 2017. "Carbonization of biomass: Effect of additives on alkali metals residue, SO2 and NO emission of chars during combustion," Energy, Elsevier, vol. 130(C), pages 560-569.
    8. Kisiela, Anna M. & Czajka, Krzysztof M. & Moroń, Wojciech & Rybak, Wiesław & Andryjowicz, Czesław, 2016. "Unburned carbon from lignite fly ash as an adsorbent for SO2 removal," Energy, Elsevier, vol. 116(P3), pages 1454-1463.
    9. Lidia Gawlik, 2018. "The Polish power industry in energy transformation process," Mineral Economics, Springer;Raw Materials Group (RMG);Luleå University of Technology, vol. 31(1), pages 229-237, May.
    10. You, C.F. & Xu, X.C., 2010. "Coal combustion and its pollution control in China," Energy, Elsevier, vol. 35(11), pages 4467-4472.
    11. Tang, Yuting & Ma, Xiaoqian & Lai, Zhiyi & Zhou, Daoxi & Lin, Hai & Chen, Yong, 2012. "NOx and SO2 emissions from municipal solid waste (MSW) combustion in CO2/O2 atmosphere," Energy, Elsevier, vol. 40(1), pages 300-306.
    12. Han, Kuihua & Gao, Jie & Qi, Jianhui, 2019. "The study of sulphur retention characteristics of biomass briquettes during combustion," Energy, Elsevier, vol. 186(C).
    Full references (including those not matched with items on IDEAS)

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