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Experimental study on the performance of a vanadium redox flow battery with non-uniformly compressed carbon felt electrode

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  • Wang, Q.
  • Qu, Z.G.
  • Jiang, Z.Y.
  • Yang, W.W.

Abstract

Optimal electrode compression can efficiently reduce electrode contact resistance and enhance species mass transfer so that the performance of vanadium redox flow battery (VRFB) is consequently improved. New designs of VRFB with a serpentine flow field on the current collector and compressed thin electrodes are investigated to increase its power density. In this study, the intrusion ratio, porosity, strain–stress, area specific resistance, hydrodynamic characteristics, and charge/discharge performance of VRFBs are comprehensively characterized under different compression ratios (CRs) which can be adjusted by changing the assembly force. Then, VRFBs using carbon felts with different CRs are tested by experiments, and the influence of electrode compression on VRFB cell performance is quantitatively evaluated. The in-homogeneous compression of carbon felt electrode in a VRFB with a flow field leads to a non-uniform porosity distribution of the electrodes under the channel, intrusion, and rib regions. The intrusion ratio, local average porosity, and permeability at different CRs are obtained. The Kozney–Carman constant of carbon fiber felt is modified by measuring the flow pressure drop through the electrode. The charge/discharge curves are acquired and the corresponding energy efficiencies are calculated under different CRs. It is shown that the charge/discharge time increases with the CR, and the energy efficiency can be improved to a maximum of 19.4% when the CR varies from 0.3% to 41.8%.

Suggested Citation

  • Wang, Q. & Qu, Z.G. & Jiang, Z.Y. & Yang, W.W., 2018. "Experimental study on the performance of a vanadium redox flow battery with non-uniformly compressed carbon felt electrode," Applied Energy, Elsevier, vol. 213(C), pages 293-305.
    • Handle: RePEc:eee:appene:v:213:y:2018:i:c:p:293-305
    DOI: 10.1016/j.apenergy.2018.01.047
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    References listed on IDEAS

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    Cited by:

    1. Messaggi, M. & Canzi, P. & Mereu, R. & Baricci, A. & Inzoli, F. & Casalegno, A. & Zago, M., 2018. "Analysis of flow field design on vanadium redox flow battery performance: Development of 3D computational fluid dynamic model and experimental validation," Applied Energy, Elsevier, vol. 228(C), pages 1057-1070.
    2. Ghimire, Purna C. & Bhattarai, Arjun & Schweiss, Rüdiger & Scherer, Günther G. & Wai, Nyunt & Yan, Qingyu, 2018. "A comprehensive study of electrode compression effects in all vanadium redox flow batteries including locally resolved measurements," Applied Energy, Elsevier, vol. 230(C), pages 974-982.
    3. Yue, Meng & Lv, Zhiqiang & Zheng, Qiong & Li, Xianfeng & Zhang, Huamin, 2019. "Battery assembly optimization: Tailoring the electrode compression ratio based on the polarization analysis in vanadium flow batteries," Applied Energy, Elsevier, vol. 235(C), pages 495-508.
    4. Chin-Lung Hsieh & Po-Hong Tsai & Ning-Yih Hsu & Yong-Song Chen, 2019. "Effect of Compression Ratio of Graphite Felts on the Performance of an All-Vanadium Redox Flow Battery," Energies, MDPI, vol. 12(2), pages 1-11, January.
    5. Wang, Q. & Qu, Z.G. & Jiang, Z.Y. & Yang, W.W., 2018. "Numerical study on vanadium redox flow battery performance with non-uniformly compressed electrode and serpentine flow field," Applied Energy, Elsevier, vol. 220(C), pages 106-116.
    6. Zeng, Yikai & Li, Fenghao & Lu, Fei & Zhou, Xuelong & Yuan, Yanping & Cao, Xiaoling & Xiang, Bo, 2019. "A hierarchical interdigitated flow field design for scale-up of high-performance redox flow batteries," Applied Energy, Elsevier, vol. 238(C), pages 435-441.
    7. Guarnieri, Massimo & Trovò, Andrea & D'Anzi, Angelo & Alotto, Piergiorgio, 2018. "Developing vanadium redox flow technology on a 9-kW 26-kWh industrial scale test facility: Design review and early experiments," Applied Energy, Elsevier, vol. 230(C), pages 1425-1434.
    8. Cheng, Ziqiang & Tenny, Kevin M. & Pizzolato, Alberto & Forner-Cuenca, Antoni & Verda, Vittorio & Chiang, Yet-Ming & Brushett, Fikile R. & Behrou, Reza, 2020. "Data-driven electrode parameter identification for vanadium redox flow batteries through experimental and numerical methods," Applied Energy, Elsevier, vol. 279(C).
    9. Duan, Z.N. & Qu, Z.G. & Wang, Q. & Wang, J.J., 2019. "Structural modification of vanadium redox flow battery with high electrochemical corrosion resistance," Applied Energy, Elsevier, vol. 250(C), pages 1632-1640.
    10. Guarnieri, Massimo & Trovò, Andrea & Picano, Francesco, 2020. "Enhancing the efficiency of kW-class vanadium redox flow batteries by flow factor modulation: An experimental method," Applied Energy, Elsevier, vol. 262(C).

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