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Analysis of the transient response and durability characteristics of a proton exchange membrane fuel cell with different micro-porous layer penetration thicknesses

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  • Cho, Junhyun
  • Park, Jaeman
  • Oh, Hwanyeong
  • Min, Kyoungdoug
  • Lee, Eunsook
  • Jyoung, Jy-Young

Abstract

The optimal design of the gas diffusion layer (GDL) of proton exchange membrane fuel cells is crucial because it directly determines the mass transport mechanism of the reactants and products. In this study, the micro-porous layer (MPL) penetration thickness, which affects the pore size profile through the GDL, is varied as the design parameter of the GDL. The cell performance is investigated under various humidity conditions, and the water permeability characteristics are studied. In addition, the accelerated carbon corrosion stress test is conducted to determine the effect of MPL penetration on GDL degradation. GDLs with large MPL penetration thickness show better performance in the high-current–density region due to the enhanced management of water resulting from a balanced capillary pressure gradient. However, the loss of penetrated MPL parts is observed due to the low binding force between the MPL and the GDL substrate.

Suggested Citation

  • Cho, Junhyun & Park, Jaeman & Oh, Hwanyeong & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2013. "Analysis of the transient response and durability characteristics of a proton exchange membrane fuel cell with different micro-porous layer penetration thicknesses," Applied Energy, Elsevier, vol. 111(C), pages 300-309.
    • Handle: RePEc:eee:appene:v:111:y:2013:i:c:p:300-309
    DOI: 10.1016/j.apenergy.2013.05.022
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    5. Chiu, Yu-Jen & Leon Yu, T., 2014. "A discrete Fourier transform-based fuel concentration and permeation sensing scheme for low temperature fuel cells," Applied Energy, Elsevier, vol. 121(C), pages 123-131.
    6. Sim, Jaebong & Kang, Minsoo & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2022. "Effects of carbon corrosion on proton exchange membrane fuel cell performance using two durability evaluation methods," Renewable Energy, Elsevier, vol. 190(C), pages 959-970.
    7. Wang, Qianqian & Tang, Fumin & Li, Bing & Dai, Haifeng & Zheng, Jim P. & Zhang, Cunman & Ming, Pingwen, 2022. "Investigation of the thermal responses under gas channel and land inside proton exchange membrane fuel cell with assembly pressure," Applied Energy, Elsevier, vol. 308(C).
    8. Qiu, Diankai & Peng, Linfa & Yi, Peiyun & Lehnert, Werner & Lai, Xinmin, 2021. "Review on proton exchange membrane fuel cell stack assembly: Quality evaluation, assembly method, contact behavior and process design," Renewable and Sustainable Energy Reviews, Elsevier, vol. 152(C).
    9. Deng, Hao & Wang, Dawei & Xie, Xu & Zhou, Yibo & Yin, Yan & Du, Qing & Jiao, Kui, 2016. "Modeling of hydrogen alkaline membrane fuel cell with interfacial effect and water management optimization," Renewable Energy, Elsevier, vol. 91(C), pages 166-177.
    10. Kong, Im Mo & Choi, Jong Won & Kim, Sung Il & Lee, Eun Sook & Kim, Min Soo, 2015. "Experimental study on the self-humidification effect in proton exchange membrane fuel cells containing double gas diffusion backing layer," Applied Energy, Elsevier, vol. 145(C), pages 345-353.
    11. Park, Jaeman & Oh, Hwanyeong & Lee, Yoo Il & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2016. "Effect of the pore size variation in the substrate of the gas diffusion layer on water management and fuel cell performance," Applied Energy, Elsevier, vol. 171(C), pages 200-212.
    12. Marco Mariani & Andrea Basso Peressut & Saverio Latorrata & Riccardo Balzarotti & Maurizio Sansotera & Giovanni Dotelli, 2021. "The Role of Fluorinated Polymers in the Water Management of Proton Exchange Membrane Fuel Cells: A Review," Energies, MDPI, vol. 14(24), pages 1-17, December.
    13. Yang, Yange & Li, Xiang & Chu, Tiankuo & Li, Bing & Zhang, Cunman, 2022. "Property evolution of gas diffusion layer and performance shrink of fuel cell during operation," Renewable Energy, Elsevier, vol. 194(C), pages 596-603.
    14. Sim, Jaebong & Kang, Minsoo & Oh, Hwanyeong & Lee, Eunsook & Jyoung, Jy-Young & Min, Kyoungdoug, 2022. "The effect of gas diffusion layer on electrochemical effective reaction area of catalyst layer and water discharge capability," Renewable Energy, Elsevier, vol. 197(C), pages 932-942.
    15. Oh, Hwanyeong & Park, Jaeman & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2015. "Effects of pore size gradient in the substrate of a gas diffusion layer on the performance of a proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 149(C), pages 186-193.
    16. Pei, Pucheng & Chen, Huicui, 2014. "Main factors affecting the lifetime of Proton Exchange Membrane fuel cells in vehicle applications: A review," Applied Energy, Elsevier, vol. 125(C), pages 60-75.
    17. Chen, Qin & Zhang, Guobin & Zhang, Xuzhong & Sun, Cheng & Jiao, Kui & Wang, Yun, 2021. "Thermal management of polymer electrolyte membrane fuel cells: A review of cooling methods, material properties, and durability," Applied Energy, Elsevier, vol. 286(C).
    18. Lin, Rui & Diao, Xiaoyu & Ma, Tiancai & Tang, Shenghao & Chen, Liang & Liu, Dengcheng, 2019. "Optimized microporous layer for improving polymer exchange membrane fuel cell performance using orthogonal test design," Applied Energy, Elsevier, vol. 254(C).
    19. Deng, Hao & Wang, Dawei & Wang, Renfang & Xie, Xu & Yin, Yan & Du, Qing & Jiao, Kui, 2016. "Effect of electrode design and operating condition on performance of hydrogen alkaline membrane fuel cell," Applied Energy, Elsevier, vol. 183(C), pages 1272-1278.

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