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Lorentz microscopy of optical fields

Author

Listed:
  • John H. Gaida

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Hugo Lourenço-Martins

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Sergey V. Yalunin

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Armin Feist

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Murat Sivis

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

  • Thorsten Hohage

    (University of Göttingen)

  • F. Javier García de Abajo

    (The Barcelona Institute of Science and Technology
    ICREA-Institució Catalana de Recerca i Estudis Avançats)

  • Claus Ropers

    (Max Planck Institute for Multidisciplinary Sciences
    University of Göttingen)

Abstract

In electron microscopy, detailed insights into nanoscale optical properties of materials are gained by spontaneous inelastic scattering leading to electron-energy loss and cathodoluminescence. Stimulated scattering in the presence of external sample excitation allows for mode- and polarization-selective photon-induced near-field electron microscopy (PINEM). This process imprints a spatial phase profile inherited from the optical fields onto the wave function of the probing electrons. Here, we introduce Lorentz-PINEM for the full-field, non-invasive imaging of complex optical near fields at high spatial resolution. We use energy-filtered defocus phase-contrast imaging and iterative phase retrieval to reconstruct the phase distribution of interfering surface-bound modes on a plasmonic nanotip. Our approach is universally applicable to retrieve the spatially varying phase of nanoscale fields and topological modes.

Suggested Citation

  • John H. Gaida & Hugo Lourenço-Martins & Sergey V. Yalunin & Armin Feist & Murat Sivis & Thorsten Hohage & F. Javier García de Abajo & Claus Ropers, 2023. "Lorentz microscopy of optical fields," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-42054-3
    DOI: 10.1038/s41467-023-42054-3
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    References listed on IDEAS

    as
    1. Jan-Wilke Henke & Arslan Sajid Raja & Armin Feist & Guanhao Huang & Germaine Arend & Yujia Yang & F. Jasmin Kappert & Rui Ning Wang & Marcel Möller & Jiahe Pan & Junqiu Liu & Ofer Kfir & Claus Ropers , 2021. "Integrated photonics enables continuous-beam electron phase modulation," Nature, Nature, vol. 600(7890), pages 653-658, December.
    2. Armin Feist & Katharina E. Echternkamp & Jakob Schauss & Sergey V. Yalunin & Sascha Schäfer & Claus Ropers, 2015. "Quantum coherent optical phase modulation in an ultrafast transmission electron microscope," Nature, Nature, vol. 521(7551), pages 200-203, May.
    3. Kangpeng Wang & Raphael Dahan & Michael Shentcis & Yaron Kauffmann & Adi Ben Hayun & Ori Reinhardt & Shai Tsesses & Ido Kaminer, 2020. "Coherent interaction between free electrons and a photonic cavity," Nature, Nature, vol. 582(7810), pages 50-54, June.
    4. X. Z. Yu & Y. Onose & N. Kanazawa & J. H. Park & J. H. Han & Y. Matsui & N. Nagaosa & Y. Tokura, 2010. "Real-space observation of a two-dimensional skyrmion crystal," Nature, Nature, vol. 465(7300), pages 901-904, June.
    5. Emilio A. Nanni & Wenqian R. Huang & Kyung-Han Hong & Koustuban Ravi & Arya Fallahi & Gustavo Moriena & R. J. Dwayne Miller & Franz X. Kärtner, 2015. "Terahertz-driven linear electron acceleration," Nature Communications, Nature, vol. 6(1), pages 1-8, December.
    6. Giulio Guzzinati & Armand Béché & Hugo Lourenço-Martins & Jérôme Martin & Mathieu Kociak & Jo Verbeeck, 2017. "Probing the symmetry of the potential of localized surface plasmon resonances with phase-shaped electron beams," Nature Communications, Nature, vol. 8(1), pages 1-8, April.
    7. J. Krehl & G. Guzzinati & J. Schultz & P. Potapov & D. Pohl & Jérôme Martin & J. Verbeeck & A. Fery & B. Büchner & A. Lubk, 2018. "Spectral field mapping in plasmonic nanostructures with nanometer resolution," Nature Communications, Nature, vol. 9(1), pages 1-6, December.
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