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Inter-valley coherent order and isospin fluctuation mediated superconductivity in rhombohedral trilayer graphene

Author

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  • Shubhayu Chatterjee

    (University of California)

  • Taige Wang

    (University of California
    Lawrence Berkeley National Laboratory)

  • Erez Berg

    (Weizmann Institute of Science)

  • Michael P. Zaletel

    (University of California
    Lawrence Berkeley National Laboratory)

Abstract

Superconductivity was recently discovered in rhombohedral trilayer graphene (RTG) in the absence of a moiré potential. Superconductivity is observed proximate to a metallic state with reduced isospin symmetry, but it remains unknown whether this is a coincidence or a key ingredient for superconductivity. Using a Hartree-Fock analysis and constraints from experiments, we argue that the symmetry breaking is inter-valley coherent (IVC) in nature. We evaluate IVC fluctuations as a possible pairing glue, and find that they lead to chiral unconventional superconductivity when the fluctuations are strong. We further elucidate how the inter-valley Hund’s coupling determines the spin-structure of the IVC ground state and breaks the degeneracy between spin-singlet and triplet superconductivity. Remarkably, if the normal state is spin-unpolarized, we find that a ferromagnetic Hund’s coupling favors spin-singlet superconductivity, in agreement with experiments. Instead, if the normal state is spin-polarized, then IVC fluctuations lead to spin-triplet pairing.

Suggested Citation

  • Shubhayu Chatterjee & Taige Wang & Erez Berg & Michael P. Zaletel, 2022. "Inter-valley coherent order and isospin fluctuation mediated superconductivity in rhombohedral trilayer graphene," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-33561-w
    DOI: 10.1038/s41467-022-33561-w
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    1. Xiaobo Lu & Petr Stepanov & Wei Yang & Ming Xie & Mohammed Ali Aamir & Ipsita Das & Carles Urgell & Kenji Watanabe & Takashi Taniguchi & Guangyu Zhang & Adrian Bachtold & Allan H. MacDonald & Dmitri K, 2019. "Superconductors, orbital magnets and correlated states in magic-angle bilayer graphene," Nature, Nature, vol. 574(7780), pages 653-657, October.
    2. Yu Saito & Fangyuan Yang & Jingyuan Ge & Xiaoxue Liu & Takashi Taniguchi & Kenji Watanabe & J. I. A. Li & Erez Berg & Andrea F. Young, 2021. "Isospin Pomeranchuk effect in twisted bilayer graphene," Nature, Nature, vol. 592(7853), pages 220-224, April.
    3. U. Zondiner & A. Rozen & D. Rodan-Legrain & Y. Cao & R. Queiroz & T. Taniguchi & K. Watanabe & Y. Oreg & F. Oppen & Ady Stern & E. Berg & P. Jarillo-Herrero & S. Ilani, 2020. "Cascade of phase transitions and Dirac revivals in magic-angle graphene," Nature, Nature, vol. 582(7811), pages 203-208, June.
    4. Jong Yeon Lee & Eslam Khalaf & Shang Liu & Xiaomeng Liu & Zeyu Hao & Philip Kim & Ashvin Vishwanath, 2019. "Theory of correlated insulating behaviour and spin-triplet superconductivity in twisted double bilayer graphene," Nature Communications, Nature, vol. 10(1), pages 1-10, December.
    5. Jeong Min Park & Yuan Cao & Kenji Watanabe & Takashi Taniguchi & Pablo Jarillo-Herrero, 2021. "Tunable strongly coupled superconductivity in magic-angle twisted trilayer graphene," Nature, Nature, vol. 590(7845), pages 249-255, February.
    6. Harpreet Singh Arora & Robert Polski & Yiran Zhang & Alex Thomson & Youngjoon Choi & Hyunjin Kim & Zhong Lin & Ilham Zaky Wilson & Xiaodong Xu & Jiun-Haw Chu & Kenji Watanabe & Takashi Taniguchi & Jas, 2020. "Superconductivity in metallic twisted bilayer graphene stabilized by WSe2," Nature, Nature, vol. 583(7816), pages 379-384, July.
    7. Haoxin Zhou & Tian Xie & Takashi Taniguchi & Kenji Watanabe & Andrea F. Young, 2021. "Superconductivity in rhombohedral trilayer graphene," Nature, Nature, vol. 598(7881), pages 434-438, October.
    8. Yuan Cao & Valla Fatemi & Shiang Fang & Kenji Watanabe & Takashi Taniguchi & Efthimios Kaxiras & Pablo Jarillo-Herrero, 2018. "Unconventional superconductivity in magic-angle graphene superlattices," Nature, Nature, vol. 556(7699), pages 43-50, April.
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