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Germanium-lead perovskite light-emitting diodes

Author

Listed:
  • Dexin Yang

    (Zhejiang University
    Hangzhou Dianzi University)

  • Guoling Zhang

    (Zhejiang University)

  • Runchen Lai

    (Zhejiang University)

  • Yao Cheng

    (Hangzhou Dianzi University)

  • Yaxiao Lian

    (Zhejiang University)

  • Min Rao

    (Hangzhou Dianzi University)

  • Dexuan Huo

    (Hangzhou Dianzi University)

  • Dongchen Lan

    (Zhejiang University)

  • Baodan Zhao

    (Zhejiang University
    Zhejiang University
    University of Cambridge)

  • Dawei Di

    (Zhejiang University
    Zhejiang University
    University of Cambridge)

Abstract

Reducing environmental impact is a key challenge for perovskite optoelectronics, as most high-performance devices are based on potentially toxic lead-halide perovskites. For photovoltaic solar cells, tin-lead (Sn–Pb) perovskite materials provide a promising solution for reducing toxicity. However, Sn–Pb perovskites typically exhibit low luminescence efficiencies, and are not ideal for light-emitting applications. Here we demonstrate highly luminescent germanium-lead (Ge–Pb) perovskite films with photoluminescence quantum efficiencies (PLQEs) of up to ~71%, showing a considerable relative improvement of ~34% over similarly prepared Ge-free, Pb-based perovskite films. In our initial demonstration of Ge–Pb perovskite LEDs, we achieve external quantum efficiencies (EQEs) of up to ~13.1% at high brightness (~1900 cd m−2), a step forward for reduced-toxicity perovskite LEDs. Our findings offer a new solution for developing eco-friendly light-emitting technologies based on perovskite semiconductors.

Suggested Citation

  • Dexin Yang & Guoling Zhang & Runchen Lai & Yao Cheng & Yaxiao Lian & Min Rao & Dexuan Huo & Dongchen Lan & Baodan Zhao & Dawei Di, 2021. "Germanium-lead perovskite light-emitting diodes," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-24616-5
    DOI: 10.1038/s41467-021-24616-5
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    Cited by:

    1. Raj, Praveen Vijaya Raj Pushpa & Nagarajan, Bagathsingh & Schoenherr, Tobias & Ramkumar, M., 2023. "A comparative investigation of a seller’s disaster payment period policy," Transportation Research Part E: Logistics and Transportation Review, Elsevier, vol. 171(C).
    2. E. Klein & E. Fouksman, 2022. "Reparations as a Rightful Share: From Universalism to Redress in Distributive Justice," Development and Change, International Institute of Social Studies, vol. 53(1), pages 31-57, January.

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