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Synthesis chemistry of metal-organic frameworks for CO2 capture and conversion for sustainable energy future

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  • Olajire, Abass A.

Abstract

Metal–organic frameworks (MOFs) have received special attention in recent years as a result of their attractive and unique properties such as structure flexibility, high surface area, tunable pore size and functionalizable organic linkers and metal centres which have led to vast array of promising applications. Their properties can be improved to further enhance their performance by functionalization of the organic linkers, postsyntheic modification, and doping of nanomaterials into their frameworks. In this review, some recent synthetic methods for the preparation of MOFs are discussed, especially those that are applicable to CO2 adsorption. The second part of this paper discusses the applications of MOFs as heterogeneous catalyst for various CO2 conversion processes, with a view to address some of the challenges faced by the current technology of CO2 conversion which tend to be very energy intensive processes with high level of waste emission and cost. The current state of MOF commercialization for niche markets is also discussed.

Suggested Citation

  • Olajire, Abass A., 2018. "Synthesis chemistry of metal-organic frameworks for CO2 capture and conversion for sustainable energy future," Renewable and Sustainable Energy Reviews, Elsevier, vol. 92(C), pages 570-607.
    • Handle: RePEc:eee:rensus:v:92:y:2018:i:c:p:570-607
    DOI: 10.1016/j.rser.2018.04.073
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    Cited by:

    1. Ayesha Rehman & Sarah Farrukh & Arshad Hussain & Erum Pervaiz, 2020. "Synthesis and effect of metal–organic frame works on CO2 adsorption capacity at various pressures: A contemplating review," Energy & Environment, , vol. 31(3), pages 367-388, May.
    2. Chakrabortty, Sankha & Kumar, Ramesh & Nayak, Jayato & Jeon, Byong-Hun & Dargar, Shashi Kant & Tripathy, Suraj K. & Pal, Parimal & Ha, Geon-Soo & Kim, Kwang Ho & Jasiński, Michał, 2023. "Green synthesis of MeOH derivatives through in situ catalytic transformations of captured CO2 in a membrane integrated photo-microreactor system: A state-of-art review for carbon capture and utilizati," Renewable and Sustainable Energy Reviews, Elsevier, vol. 182(C).
    3. Wang, Honglin & Liu, Yanrong & Laaksonen, Aatto & Krook-Riekkola, Anna & Yang, Zhuhong & Lu, Xiaohua & Ji, Xiaoyan, 2020. "Carbon recycling – An immense resource and key to a smart climate engineering: A survey of technologies, cost and impurity impact," Renewable and Sustainable Energy Reviews, Elsevier, vol. 131(C).
    4. Qiao, Yuanting & Bailey, Josh J. & Huang, Qi & Ke, Xuebin & Wu, Chunfei, 2022. "Potential photo-switching sorbents for CO2 capture – A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 158(C).
    5. Alfe, M. & Policicchio, A. & Lisi, L. & Gargiulo, V., 2021. "Solid sorbents for CO2 and CH4 adsorption: The effect of metal organic framework hybridization with graphene-like layers on the gas sorption capacities at high pressure," Renewable and Sustainable Energy Reviews, Elsevier, vol. 141(C).
    6. Tao, Huayu & Qian, Xi & Zhou, Yi & Cheng, Hongfei, 2022. "Research progress of clay minerals in carbon dioxide capture," Renewable and Sustainable Energy Reviews, Elsevier, vol. 164(C).

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