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Slow dynamics at the liquid-glass transition

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  • Carmesin, Hans-Otto

Abstract

A fluid with isotropic particles is analyzed from first principles. Below the visco-elastic transition temperature, the relaxation time for the specific heat diverges according to a Vogel-Fulcher law. The reason for the discovered singularity is the volume excluded by a particle. So, the singularity is of quite general nature. Formally, the classical fluid undergoes a phase transition of first order at the singularity. For o-terphenyl, the theory is in agreement with experiments. Comparisons with other properties below the melting temperature are presented and further experiments are suggested.

Suggested Citation

  • Carmesin, Hans-Otto, 1993. "Slow dynamics at the liquid-glass transition," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 201(1), pages 25-29.
    • Handle: RePEc:eee:phsmap:v:201:y:1993:i:1:p:25-29
    DOI: 10.1016/0378-4371(93)90395-K
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