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The theory of spin-correlated crystal fields: Application to Gd3+ in C3h symmetry

Author

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  • Tuszyński, J.A.
  • Dixon, J.M.
  • Chatterjee, R.

Abstract

Application of the recently formulated theory of spin-correlated crystal fields is made to the Gd3+ ion in ethysulphate lattices. Detailed calculations of the spin-correlated crystal field contribution to the zero field splitting are found to be of the correct sign but its magnitude is too large. It is comjectured that similar types of mechanisms involving excitations to other sites may be responsible for the discrepancy.

Suggested Citation

  • Tuszyński, J.A. & Dixon, J.M. & Chatterjee, R., 1986. "The theory of spin-correlated crystal fields: Application to Gd3+ in C3h symmetry," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 135(1), pages 213-225.
    • Handle: RePEc:eee:phsmap:v:135:y:1986:i:1:p:213-225
    DOI: 10.1016/0378-4371(86)90113-5
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    References listed on IDEAS

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    1. Chatterjee, R. & Dixon, J.M., 1980. "“Crystal fields” for magnetic ions in metals from itinerant electrons," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 100(1), pages 100-118.
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    1. Tuszyński, J.A. & Dixon, J.M., 1988. "Comments on the origin of relativistic crystal fields," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 147(3), pages 555-566.
    2. Tuszyński, J.A. & Dixon, J.M. & Chatterjee, R., 1984. "The theory of spin correlated crystal fields," Physica A: Statistical Mechanics and its Applications, Elsevier, vol. 127(1), pages 228-240.

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