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Catalytic co-pyrolysis of paper biomass and plastic mixtures (HDPE (high density polyethylene), PP (polypropylene) and PET (polyethylene terephthalate)) and product analysis

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  • Chattopadhyay, Jayeeta
  • Pathak, T.S.
  • Srivastava, R.
  • Singh, A.C.

Abstract

Catalytic co-pyrolysis of biomass and plastics (HDPE (high density polyethylene), PP (polypropylene) and PET (polyethylene terephthalate)) has been performed in a fixed-bed reactor in presence of cobalt based alumina, ceria and ceria-alumina catalysts to analyze the product distribution and selectivity. Catalysts are synthesized using co-precipitation method and characterized by BET (Brunauer–Emmett–Teller) surface area and XRD analysis. The effect of catalytic co-pyrolysis at different temperature with product distribution has been evaluated. The results have clearly shown the synergistic effect between biomass and plastics, the liquid products gradually increases forming with rise in the plastic content in the blend. Gaseous products have yielded most during pyrolysis of blend having biomass/plastics ratio of 5:1 with the presence of 40% Co/30% CeO2/30% Al2O3 catalyst with hydrogen gas production touched its peak of 47 vol%. Catalytic performance enhanced with increase with the cobalt loading, with best performance attributing to 40% Co/30% CeO2/30% Al2O3 catalyst.

Suggested Citation

  • Chattopadhyay, Jayeeta & Pathak, T.S. & Srivastava, R. & Singh, A.C., 2016. "Catalytic co-pyrolysis of paper biomass and plastic mixtures (HDPE (high density polyethylene), PP (polypropylene) and PET (polyethylene terephthalate)) and product analysis," Energy, Elsevier, vol. 103(C), pages 513-521.
    • Handle: RePEc:eee:energy:v:103:y:2016:i:c:p:513-521
    DOI: 10.1016/j.energy.2016.03.015
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    1. Stančin, H. & Mikulčić, H. & Wang, X. & Duić, N., 2020. "A review on alternative fuels in future energy system," Renewable and Sustainable Energy Reviews, Elsevier, vol. 128(C).
    2. Liu, Rongtang & Liu, Ming & Fan, Peipei & Zhao, Yongliang & Yan, Junjie, 2018. "Thermodynamic study on a novel lignite poly-generation system of electricity-gas-tar integrated with pre-drying and pyrolysis," Energy, Elsevier, vol. 165(PB), pages 140-152.
    3. Al-Rumaihi, Aisha & Shahbaz, Muhammad & Mckay, Gordon & Mackey, Hamish & Al-Ansari, Tareq, 2022. "A review of pyrolysis technologies and feedstock: A blending approach for plastic and biomass towards optimum biochar yield," Renewable and Sustainable Energy Reviews, Elsevier, vol. 167(C).
    4. Park, Young-Kwon & Jung, Jaehun & Ryu, Sumin & Lee, Hyung Won & Siddiqui, Muhammad Zain & Jae, Jungho & Watanabe, Atsushi & Kim, Young-Min, 2019. "Catalytic co-pyrolysis of yellow poplar wood and polyethylene terephthalate over two stage calcium oxide-ZSM-5," Applied Energy, Elsevier, vol. 250(C), pages 1706-1718.
    5. Kawale, Harshal D. & Kishore, Nanda, 2020. "Comparative study on pyrolysis of Delonix Regia, Pinewood sawdust and their co-feed for plausible bio-fuels production," Energy, Elsevier, vol. 203(C).
    6. Choi, Dongho & Jung, Sungyup & Lee, Sang Soo & Lin, Kun-Yi Andrew & Park, Young-Kwon & Kim, Hana & Tsang, Yiu Fai & Kwon, Eilhann E., 2021. "Leveraging carbon dioxide to control the H2/CO ratio in catalytic pyrolysis of fishing net waste," Renewable and Sustainable Energy Reviews, Elsevier, vol. 138(C).
    7. Dmitry Porshnov, 2022. "Evolution of pyrolysis and gasification as waste to energy tools for low carbon economy," Wiley Interdisciplinary Reviews: Energy and Environment, Wiley Blackwell, vol. 11(1), January.
    8. Navarro, M.V. & López, J.M. & Veses, A. & Callén, M.S. & García, T., 2018. "Kinetic study for the co-pyrolysis of lignocellulosic biomass and plastics using the distributed activation energy model," Energy, Elsevier, vol. 165(PA), pages 731-742.
    9. Hemant Ghai & Deepak Sakhuja & Shikha Yadav & Preeti Solanki & Chayanika Putatunda & Ravi Kant Bhatia & Arvind Kumar Bhatt & Sunita Varjani & Yung-Hun Yang & Shashi Kant Bhatia & Abhishek Walia, 2022. "An Overview on Co-Pyrolysis of Biodegradable and Non-Biodegradable Wastes," Energies, MDPI, vol. 15(11), pages 1-27, June.
    10. Lucía Quesada & Mónica Calero de Hoces & M. A. Martín-Lara & Germán Luzón & G. Blázquez, 2020. "Performance of Different Catalysts for the In Situ Cracking of the Oil-Waxes Obtained by the Pyrolysis of Polyethylene Film Waste," Sustainability, MDPI, vol. 12(13), pages 1-15, July.
    11. Chen, Wei-Hsin & Farooq, Wasif & Shahbaz, Muhammad & Naqvi, Salman Raza & Ali, Imtiaz & Al-Ansari, Tareq & Saidina Amin, Nor Aishah, 2021. "Current status of biohydrogen production from lignocellulosic biomass, technical challenges and commercial potential through pyrolysis process," Energy, Elsevier, vol. 226(C).
    12. Jin, Xuanjun & Lee, Jae Hoon & Choi, Joon Weon, 2022. "Catalytic co-pyrolysis of woody biomass with waste plastics: Effects of HZSM-5 and pyrolysis temperature on producing high-value pyrolytic products and reducing wax formation," Energy, Elsevier, vol. 239(PA).
    13. Alexey Paukov & Romen Magaril & Elena Magaril, 2019. "An Investigation of the Feasibility of the Organic Municipal Solid Waste Processing by Coking," Sustainability, MDPI, vol. 11(2), pages 1-13, January.
    14. Stančin, H. & Šafář, M. & Růžičková, J. & Mikulčić, H. & Raclavská, H. & Wang, X. & Duić, N., 2022. "Influence of plastic content on synergistic effect and bio-oil quality from the co-pyrolysis of waste rigid polyurethane foam and sawdust mixture," Renewable Energy, Elsevier, vol. 196(C), pages 1218-1228.
    15. Jiang, Haifeng & Liu, Haipeng & Dong, Jiaxin & Song, Jiaxing & Deng, Sunhua & Chen, Jie & Zhang, Yu & Hong, Wenpeng, 2022. "Enhancing ketones and syngas production by CO2-assisted catalytic pyrolysis of cellulose with the Ce–Co–Na ternary catalyst," Energy, Elsevier, vol. 250(C).
    16. Samal, Biswajit & Vanapalli, Kumar Raja & Dubey, Brajesh Kumar & Bhattacharya, Jayanta & Chandra, Subhash & Medha, Isha, 2021. "Influence of process parameters on thermal characteristics of char from co-pyrolysis of eucalyptus biomass and polystyrene: Its prospects as a solid fuel," Energy, Elsevier, vol. 232(C).
    17. Chen, Rongjie & Lun, Liyong & Cong, Kunlin & Li, Qinghai & Zhang, Yanguo, 2019. "Insights into pyrolysis and co-pyrolysis of tobacco stalk and scrap tire: Thermochemical behaviors, kinetics, and evolved gas analysis," Energy, Elsevier, vol. 183(C), pages 25-34.
    18. Ghulamullah Maitlo & Imran Ali & Hubdar Ali Maitlo & Safdar Ali & Imran Nazir Unar & Muhammad Bilal Ahmad & Darya Khan Bhutto & Ramesh Kumar Karmani & Shamim ur Rehman Naich & Raja Umer Sajjad & Sikan, 2022. "Plastic Waste Recycling, Applications, and Future Prospects for a Sustainable Environment," Sustainability, MDPI, vol. 14(18), pages 1-27, September.
    19. Fivga, Antzela & Dimitriou, Ioanna, 2018. "Pyrolysis of plastic waste for production of heavy fuel substitute: A techno-economic assessment," Energy, Elsevier, vol. 149(C), pages 865-874.

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