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Recent advances in supercapacitor electrode materials based on MOF-derived transition metal sulfides

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  • Dash, Sweta R.
  • Yadav, Mangal S.
  • Sahoo, Rakesh K.
  • Sharma, A.L.

Abstract

The development of next-generation energy storage technologies demands innovative material design strategies that can meet performance, scalability, and sustainability requirements. Metal-organic frameworks (MOFs) and their derived transition metal sulfides (TMSs) have attracted significant attention in the field of electrochemical supercapacitors due to their highly tunable architectures, extensive surface areas, and excellent electrical conductivity. This review aims to bridge the knowledge gap between electrochemists and researchers working on MOFs and MOF-derived TMSs. It begins by outlining the fundamental concepts of energy storage systems, including various charge storage mechanisms, while highlighting the critical interdependence among material properties, electrode architecture, and device-level parameters that collectively impact performance. The review then delves into the design principles of MOFs and their derived TMSs, focusing on key parameters that determine their effectiveness in high-rate electrochemical energy storage (EES) applications. Furthermore, it provides a comprehensive discussion on the strategies employed to improve the EES performance of MOF-derived TMSs in comparison to conventional TMS materials, along with their practical implementation in supercapacitor technologies. Finally, special attention is given to detailed investigations of charge storage mechanisms, incorporating both in-situ and ex-situ experimental techniques, and their correlation with theoretical insights derived from density functional theory (DFT) calculations.

Suggested Citation

  • Dash, Sweta R. & Yadav, Mangal S. & Sahoo, Rakesh K. & Sharma, A.L., 2026. "Recent advances in supercapacitor electrode materials based on MOF-derived transition metal sulfides," Applied Energy, Elsevier, vol. 408(C).
    • Handle: RePEc:eee:appene:v:408:y:2026:i:c:s0306261926000012
    DOI: 10.1016/j.apenergy.2026.127349
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