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New Approach to Fuelization of Herbaceous Lignocelluloses through Simultaneous Saccharification and Fermentation Followed by Photocatalytic Reforming

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  • Masahide Yasuda

    (Department of Applied Chemistry, Faculty of Engineering, University of Miyazaki, Gakuen-Kibanadai Nishi, Miyazaki 889-2192, Japan)

  • Ryo Kurogi

    (Department of Applied Chemistry, Faculty of Engineering, University of Miyazaki, Gakuen-Kibanadai Nishi, Miyazaki 889-2192, Japan)

  • Hikaru Tsumagari

    (Department of Applied Chemistry, Faculty of Engineering, University of Miyazaki, Gakuen-Kibanadai Nishi, Miyazaki 889-2192, Japan)

  • Tsutomu Shiragami

    (Department of Applied Chemistry, Faculty of Engineering, University of Miyazaki, Gakuen-Kibanadai Nishi, Miyazaki 889-2192, Japan)

  • Tomoko Matsumoto

    (Center for Collaborative Research and Community Cooperation, University of Miyazaki, Gakuen-Kibanadai Nishi, Miyazaki 889-2192, Japan)

Abstract

Bio-fuelization of herbaceous lignocelluloses through a simultaneous saccharification and fermentation process (SSF) and photocatalytic reforming (photo-Reform) was examined. The SSF of the alkali-pretreated bamboo, rice straw, and silvergrass was performed in an acetate buffer (pH 5.0) using cellulase, xylanase, and Saccharomyces cerevisiae at 34 °C. Ethanol was produced in 63%–85% yields, while xylose was produced in 74%–97% yields without being fermented because xylose cannot be fermented by S. cerevisiae . After the removal of ethanol from the aqueous SSF solution, the SSF solution was subjected to a photo-Reform step where xylose was transformed into hydrogen by a photocatalytic reaction using Pt-loaded TiO 2 (2 wt % of Pt content) under irradiation by a high pressure mercury lamp. The photo-Reform process produced hydrogen in nearly a yield of ten theoretical equivalents to xylose. Total energy was recovered as ethanol and hydrogen whose combustion energy was 73.4%–91.1% of that of the alkali-pretreated lignocelluloses (holocellulose).

Suggested Citation

  • Masahide Yasuda & Ryo Kurogi & Hikaru Tsumagari & Tsutomu Shiragami & Tomoko Matsumoto, 2014. "New Approach to Fuelization of Herbaceous Lignocelluloses through Simultaneous Saccharification and Fermentation Followed by Photocatalytic Reforming," Energies, MDPI, vol. 7(7), pages 1-11, June.
    • Handle: RePEc:gam:jeners:v:7:y:2014:i:7:p:4087-4097:d:37517
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    References listed on IDEAS

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    1. Balat, Mustafa & Balat, Havva, 2009. "Recent trends in global production and utilization of bio-ethanol fuel," Applied Energy, Elsevier, vol. 86(11), pages 2273-2282, November.
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    1. Yasuda, Masahide & Matsumoto, Tomoko & Yamashita, Toshiaki, 2018. "Sacrificial hydrogen production over TiO2-based photocatalysts: Polyols, carboxylic acids, and saccharides," Renewable and Sustainable Energy Reviews, Elsevier, vol. 81(P2), pages 1627-1635.
    2. Asma Sattar & Chaudhry Arslan & Changying Ji & Sumiyya Sattar & Irshad Ali Mari & Haroon Rashid & Fariha Ilyas, 2016. "Comparing the Bio-Hydrogen Production Potential of Pretreated Rice Straw Co-Digested with Seeded Sludge Using an Anaerobic Bioreactor under Mesophilic Thermophilic Conditions," Energies, MDPI, vol. 9(3), pages 1-14, March.
    3. Vincenzo Palma & Concetta Ruocco & Eugenio Meloni & Antonio Ricca, 2017. "Influence of Catalytic Formulation and Operative Conditions on Coke Deposition over CeO 2 -SiO 2 Based Catalysts for Ethanol Reforming," Energies, MDPI, vol. 10(7), pages 1-13, July.

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