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Steam reforming of toluene over nickel catalysts supported on coal gangue ash

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  • Lu, Min
  • Xiong, Zuhong
  • Fang, Kejing
  • Li, Xi
  • Li, Jiqing
  • Li, Tao

Abstract

The development of high performance and low-cost catalyst is very important to remove tar during biomass gasification. Solid waste coal gangue ash (CGA), which mainly contains SiO2, Al2O3, Fe2O3 and CaO, was selected as support for Ni-based catalyst. The prepared low-cost catalysts were characterized suitably by XRD, BET, TPR, SEM, TG and Raman techniques. Toluene was selected as typical biomass tar model compounds to test the catalyst performance and compared with traditional catalysts Ni/Al2O3 and Ni/SiO2. Ni/CGA-1d exhibited the highest catalytic performance with the toluene conversion and H2 yield accounting for 91.5% and 58.2% respectively, at 800 °C. It was showed that the performance of Ni/CGA-1d was higher than traditional catalysts Ni/Al2O3 and Ni/SiO2, and comparable with other polymetallic reforming catalysts. Due to the good resistance of carbon deposition, the Ni/CGA-1d catalyst also performed better catalytic activity stability. The ability should be attributing to the existence of some metal elements such as Fe, Mg, K, Ca et al. in coal gangue ash support.

Suggested Citation

  • Lu, Min & Xiong, Zuhong & Fang, Kejing & Li, Xi & Li, Jiqing & Li, Tao, 2020. "Steam reforming of toluene over nickel catalysts supported on coal gangue ash," Renewable Energy, Elsevier, vol. 160(C), pages 385-395.
    • Handle: RePEc:eee:renene:v:160:y:2020:i:c:p:385-395
    DOI: 10.1016/j.renene.2020.06.012
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    References listed on IDEAS

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    1. Oh, Gunung & Park, Seo Yoon & Seo, Myung Won & Kim, Yong Ku & Ra, Ho Won & Lee, Jae-Goo & Yoon, Sang Jun, 2016. "Ni/Ru–Mn/Al2O3 catalysts for steam reforming of toluene as model biomass tar," Renewable Energy, Elsevier, vol. 86(C), pages 841-847.
    2. Anis, Samsudin & Zainal, Z.A., 2011. "Tar reduction in biomass producer gas via mechanical, catalytic and thermal methods: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(5), pages 2355-2377, June.
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    1. Gao, Ningbo & Salisu, Jamilu & Quan, Cui & Williams, Paul, 2021. "Modified nickel-based catalysts for improved steam reforming of biomass tar: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 145(C).
    2. Li, Jie & Chang, Guozhang & Song, Ke & Hao, Bolun & Wang, Cuiping & Zhang, Jian & Yue, Guangxi & Hu, Shugang, 2023. "Influence of coal bottom ash additives on catalytic reforming of biomass pyrolysis gaseous tar and biochar/steam gasification reactivity," Renewable Energy, Elsevier, vol. 203(C), pages 434-444.

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