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Thermally stable iron based redox catalysts for the thermo-chemical hydrogen generation from water

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  • Song, Lee-hwa
  • Kang, Hyun Woo
  • Park, Seung Bin

Abstract

Redox materials with high thermal stabilities, comprising iron oxide with alumina were synthesized from ultrasonic spray pyrolysis method. Their catalytic activities towards the redox evolution of hydrogen from water were evaluated and compared with that of pure iron oxide, which decreased rapidly after 1 cycle due to its low thermal stability. The samples containing alumina sustained their total and relative hydrogen evolutions over three redox cycles, while maintaining their original surface morphologies, thus demonstrating their thermal stability.

Suggested Citation

  • Song, Lee-hwa & Kang, Hyun Woo & Park, Seung Bin, 2012. "Thermally stable iron based redox catalysts for the thermo-chemical hydrogen generation from water," Energy, Elsevier, vol. 42(1), pages 313-320.
    • Handle: RePEc:eee:energy:v:42:y:2012:i:1:p:313-320
    DOI: 10.1016/j.energy.2012.03.051
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    References listed on IDEAS

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    Cited by:

    1. Rhodes, Nathan R. & Bobek, Michael M. & Allen, Kyle M. & Hahn, David W., 2015. "Investigation of long term reactive stability of ceria for use in solar thermochemical cycles," Energy, Elsevier, vol. 89(C), pages 924-931.
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    3. Lange, M. & Roeb, M. & Sattler, C. & Pitz-Paal, R., 2014. "T–S diagram efficiency analysis of two-step thermochemical cycles for solar water splitting under various process conditions," Energy, Elsevier, vol. 67(C), pages 298-308.

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