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CO2 reduction-conversion to precipitates and morphological control through the application of the mineral carbonation mechanism

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  • Park, Sangwon

Abstract

This study aimed to verify CO2 reduction and morphological control of its precipitates by applying the CO2 mineralization mechanism under ambient conditions. In the first stage, CO2 absorption-conversion experiments were performed using three types of amines (mono-ethanolamine, MEA; di-ethanolamine, DEA; and methyl-di-ethanolamine, MDEA) to improve the rate and efficiency of CO2 conversion into metal carbonates. In the second stage, CO2 was re-absorbed and supplied as aqueous CO2, forming MgCO3 and MgCO3(H2O)3 precipitates. The formed MgCO3 was analyzed by X-ray diffraction (XRD) and field emission scanning electron microscope (FE-SEM). In particular, MgCO3 was formed only in the MEA solution although other amines were exposed to the same experimental conditions. Therefore, the results showed that the CO2 precipitate morphology could be controlled by the type of the conversion solution used. This study has significance regarding CO2 reduction and utilization because the emitted CO2 could be stored semi-permanently. Furthermore, the formed MgCO3 could be re-used in various industries through morphology control. Therefore, this study verified the potential of the CO2 mineralization mechanism for CO2 reduction and morphology control.

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  • Park, Sangwon, 2018. "CO2 reduction-conversion to precipitates and morphological control through the application of the mineral carbonation mechanism," Energy, Elsevier, vol. 153(C), pages 413-421.
    • Handle: RePEc:eee:energy:v:153:y:2018:i:c:p:413-421
    DOI: 10.1016/j.energy.2018.04.086
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    References listed on IDEAS

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    1. Park, Sangwon & Song, Kyungsun & Jo, Hwanju, 2017. "Laboratory-scale experiment on a novel mineralization-based method of CO2 capture using alkaline solution," Energy, Elsevier, vol. 124(C), pages 589-598.
    2. Fagerlund, Johan & Nduagu, Experience & Romão, Inês & Zevenhoven, Ron, 2012. "CO2 fixation using magnesium silicate minerals part 1: Process description and performance," Energy, Elsevier, vol. 41(1), pages 184-191.
    3. Zevenhoven, Ron & Slotte, Martin & Åbacka, Jacob & Highfield, James, 2016. "A comparison of CO2 mineral sequestration processes involving a dry or wet carbonation step," Energy, Elsevier, vol. 117(P2), pages 604-611.
    4. Nduagu, Experience & Romão, Inês & Fagerlund, Johan & Zevenhoven, Ron, 2013. "Performance assessment of producing Mg(OH)2 for CO2 mineral sequestration," Applied Energy, Elsevier, vol. 106(C), pages 116-126.
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    6. Teir, Sebastian & Eloneva, Sanni & Fogelholm, Carl-Johan & Zevenhoven, Ron, 2007. "Dissolution of steelmaking slags in acetic acid for precipitated calcium carbonate production," Energy, Elsevier, vol. 32(4), pages 528-539.
    7. Lackner, Klaus S. & Wendt, Christopher H. & Butt, Darryl P. & Joyce, Edward L. & Sharp, David H., 1995. "Carbon dioxide disposal in carbonate minerals," Energy, Elsevier, vol. 20(11), pages 1153-1170.
    8. Park, Sangwon & Lee, Min-Gu & Park, Jinwon, 2013. "CO2 (carbon dioxide) fixation by applying new chemical absorption-precipitation methods," Energy, Elsevier, vol. 59(C), pages 737-742.
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    Cited by:

    1. Zhang, Weifeng & Xu, Yuanlong & Deng, Zhaoxiong & Wang, Qiuhua, 2022. "Experiments on continuous chemical desorption of CO2-rich solutions," Energy, Elsevier, vol. 239(PD).
    2. Baena-Moreno, Francisco M. & Rodríguez-Galán, Mónica & Vega, Fernando & Reina, T.R. & Vilches, Luis F. & Navarrete, Benito, 2019. "Converting CO2 from biogas and MgCl2 residues into valuable magnesium carbonate: A novel strategy for renewable energy production," Energy, Elsevier, vol. 180(C), pages 457-464.
    3. Yafei Zhao & Ken-ichi Itakura, 2023. "A State-of-the-Art Review on Technology for Carbon Utilization and Storage," Energies, MDPI, vol. 16(10), pages 1-22, May.
    4. Naraharisetti, Pavan Kumar & Yeo, Tze Yuen & Bu, Jie, 2019. "New classification of CO2 mineralization processes and economic evaluation," Renewable and Sustainable Energy Reviews, Elsevier, vol. 99(C), pages 220-233.
    5. He, Minyu & Teng, Liumei & Gao, Yuxiang & Rohani, Sohrab & Ren, Shan & Li, Jiangling & Yang, Jian & Liu, Qingcai & Liu, Weizao, 2022. "Simultaneous CO2 mineral sequestration and rutile beneficiation by using titanium-bearing blast furnace slag: Process description and optimization," Energy, Elsevier, vol. 248(C).

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