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Promotion of hydrate-based CO2 capture from flue gas by additive mixtures (THF (tetrahydrofuran) + TBAB (tetra-n-butyl ammonium bromide))

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  • Yang, Mingjun
  • Jing, Wen
  • Zhao, Jiafei
  • Ling, Zheng
  • Song, Yongchen

Abstract

HBGS (Hydrate-based gas separation) is a potential method for CO2 capture from fossil fuel power plants. High hydrate formation rates and low energy consumption are still the demands for industrial application of HBGS. The promotion effects of three additive mixtures (THF (tetrahydrofuran) + TBAB (tetra-n-butyl ammonium bromide)) on flue gas (CO2/N2) hydrate phase equilibrium and CO2 capture characteristics were experimentally investigated in this study. It was found that hydrate phase equilibrium pressure for the 5% THF + 5% TBAB mixture was almost the same as that for the 5% THF + 10% TBAB mixture. Both the gas consumption and CO2 recovery increased substantially with increases in the mass fractions of THF or/and TBAB. The experimental results also showed that the gas consumption increases with the enhancement of initial pressure. Considering the hydrate phase equilibrium conditions and gas separation efficiency, an additive mixture with a mass fraction of 5% THF + 10% TBAB was found to be a better choice for hydrate-based CO2 capture from flue gas relative to other additive mixtures investigated in this study.

Suggested Citation

  • Yang, Mingjun & Jing, Wen & Zhao, Jiafei & Ling, Zheng & Song, Yongchen, 2016. "Promotion of hydrate-based CO2 capture from flue gas by additive mixtures (THF (tetrahydrofuran) + TBAB (tetra-n-butyl ammonium bromide))," Energy, Elsevier, vol. 106(C), pages 546-553.
    • Handle: RePEc:eee:energy:v:106:y:2016:i:c:p:546-553
    DOI: 10.1016/j.energy.2016.03.092
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    Cited by:

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    5. Chun-Gang Xu & Min Wang & Gang Xu & Xiao-Sen Li & Wei Zhang & Jing Cai & Zhao-Yang Chen, 2021. "The Relationship between Thermal Characteristics and Microstructure/Composition of Carbon Dioxide Hydrate in the Presence of Cyclopentane," Energies, MDPI, vol. 14(4), pages 1-17, February.
    6. Zang, Xiaoya & Wang, Jing & He, Yong & Zhou, Xuebing & Liang, Deqing, 2022. "Formation kinetics and microscopic characteristics of synthesized ternary gas mixture hydrates in TBAB aqueous solutions," Energy, Elsevier, vol. 245(C).
    7. Wang, Yiwei & Deng, Ye & Guo, Xuqiang & Sun, Qiang & Liu, Aixian & Zhang, Guangqing & Yue, Gang & Yang, Lanying, 2018. "Experimental and modeling investigation on separation of methane from coal seam gas (CSG) using hydrate formation," Energy, Elsevier, vol. 150(C), pages 377-395.
    8. Pivezhani, Farzane & Roosta, Hadi & Dashti, Ali & Mazloumi, S. Hossein, 2016. "Investigation of CO2 hydrate formation conditions for determining the optimum CO2 storage rate and energy: Modeling and experimental study," Energy, Elsevier, vol. 113(C), pages 215-226.
    9. Yoro, Kelvin O. & Daramola, Michael O. & Sekoai, Patrick T. & Armah, Edward K. & Wilson, Uwemedimo N., 2021. "Advances and emerging techniques for energy recovery during absorptive CO2 capture: A review of process and non-process integration-based strategies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 147(C).
    10. Kim, Soyoung & Choi, Sung-Deuk & Seo, Yongwon, 2017. "CO2 capture from flue gas using clathrate formation in the presence of thermodynamic promoters," Energy, Elsevier, vol. 118(C), pages 950-956.
    11. Wang, Yiwei & Du, Mei & Guo, Xuqiang & Sun, Qiang & Liu, Aixian & Chen, Bo & Chen, Guangjin & Sun, Changyu & Yang, Lanying, 2017. "Experiments and simulations for continuous recovery of methane from coal seam gas (CSG) utilizing hydrate formation," Energy, Elsevier, vol. 129(C), pages 28-41.
    12. Shi, Lingli & Li, Junhui & He, Yong & Lu, Jingsheng & Long, Zhen & Liang, Deqing, 2023. "Memory effect test and analysis in methane hydrates reformation process," Energy, Elsevier, vol. 272(C).
    13. Dong, Hongsheng & Wang, Jiaqi & Xie, Zhuoxue & Wang, Bin & Zhang, Lunxiang & Shi, Quan, 2021. "Potential applications based on the formation and dissociation of gas hydrates," Renewable and Sustainable Energy Reviews, Elsevier, vol. 143(C).
    14. Lai, Xi & Zhao, Li & Nie, Xianhua & Zhang, Yue & Zhang, Qi, 2023. "Hydrate-based composition separation of R32/R1234yf mixed working fluids applied in composition-adjustable organic Rankine cycle," Energy, Elsevier, vol. 284(C).
    15. Najmus S. Sifat & Yousef Haseli, 2019. "A Critical Review of CO 2 Capture Technologies and Prospects for Clean Power Generation," Energies, MDPI, vol. 12(21), pages 1-33, October.

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