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Landfill gas upgrading with pilot-scale water scrubber: Performance assessment with absorption water recycling

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  • Läntelä, J.
  • Rasi, S.
  • Lehtinen, J.
  • Rintala, J.

Abstract

A pilot-scale counter current absorption process for upgrading municipal solid waste (MSW) landfill gas to produce vehicle fuel was studied using absorption, desorption and drying units and water as an absorbent. Continuous water recycling was used without adding new water to the system. The process parameters were defined by a previous study made with this pilot system. The effect of pressure (20–25bar), temperature (10–25°C) and water flow speed (5.5–11l/min) on the upgrading performance, trace compounds (siloxanes, halogenated compounds) and water quality were investigated. Raw landfill gas flow was kept constant at 7.41Nm3/h. Methane (CH4) and carbon dioxide (CO2) contents in the product gas were 86–90% and 4.5–8.0% with all studied pressures and temperatures. The remaining fraction in product gas was nitrogen (N2) (from 1% to 7%). Organic silicon compounds (siloxanes) were reduced by 16.6% and halogenated compounds similarly by 90.1% by water absorption. From studied process parameters, only water flow speed affected the removal of siloxanes and halogen compounds. The absorbent water pH was between 4.4–4.9, sulphide concentration between 0.1–1.0mg/l and carbonate concentration between 500–1000mg/l. The product gas drying system reduced the siloxane concentration by 99.1% and halogenated compounds by 99.9% compared to the raw landfill gas. In conclusion, the pilot-scale gas upgrading process studied appears to be able to produce gas with high energy content (approx 86–90% methane) using a closed water circulation system. When using a standard gas drying system, all trace compounds can be removed by over 99% compared to raw landfill gas.

Suggested Citation

  • Läntelä, J. & Rasi, S. & Lehtinen, J. & Rintala, J., 2012. "Landfill gas upgrading with pilot-scale water scrubber: Performance assessment with absorption water recycling," Applied Energy, Elsevier, vol. 92(C), pages 307-314.
    • Handle: RePEc:eee:appene:v:92:y:2012:i:c:p:307-314
    DOI: 10.1016/j.apenergy.2011.10.011
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    References listed on IDEAS

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    1. Rasi, S. & Veijanen, A. & Rintala, J., 2007. "Trace compounds of biogas from different biogas production plants," Energy, Elsevier, vol. 32(8), pages 1375-1380.
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    4. Wantz, Eliot & Benizri, David & Dietrich, Nicolas & Hébrard, Gilles, 2022. "Rate-based modeling approach for High Pressure Water Scrubbing with unsteady gas flowrate and multicomponent absorption applied to biogas upgrading," Applied Energy, Elsevier, vol. 312(C).
    5. Ma, Chunyan & Xie, Yujiao & Ji, Xiaoyan & Liu, Chang & Lu, Xiaohua, 2018. "Modeling, simulation and evaluation of biogas upgrading using aqueous choline chloride/urea," Applied Energy, Elsevier, vol. 229(C), pages 1269-1283.
    6. Bacsik, Zoltán & Cheung, Ocean & Vasiliev, Petr & Hedin, Niklas, 2016. "Selective separation of CO2 and CH4 for biogas upgrading on zeolite NaKA and SAPO-56," Applied Energy, Elsevier, vol. 162(C), pages 613-621.
    7. Moioli, Emanuele & Schildhauer, Tilman, 2022. "Negative CO2 emissions from flexible biofuel synthesis: Concepts, potentials, technologies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 158(C).
    8. Wantz, Eliot & Lemonnier, Mathis & Benizri, David & Dietrich, Nicolas & Hébrard, Gilles, 2023. "Innovative high-pressure water scrubber for biogas upgrading at farm-scale using vacuum for water regeneration," Applied Energy, Elsevier, vol. 350(C).
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    11. Gao, Shida & Bo, Cuimei & Li, Jun & Niu, Chao & Lu, Xiaohua, 2020. "Multi-objective optimization and dynamic control of biogas pressurized water scrubbing process," Renewable Energy, Elsevier, vol. 147(P1), pages 2335-2344.
    12. Hosseinipour, Sayed Amir & Mehrpooya, Mehdi, 2019. "Comparison of the biogas upgrading methods as a transportation fuel," Renewable Energy, Elsevier, vol. 130(C), pages 641-655.
    13. Yang, Liangcheng & Ge, Xumeng & Wan, Caixia & Yu, Fei & Li, Yebo, 2014. "Progress and perspectives in converting biogas to transportation fuels," Renewable and Sustainable Energy Reviews, Elsevier, vol. 40(C), pages 1133-1152.
    14. Chen, Man & Zhang, Fang & Zhang, Yan & Zeng, Raymond J., 2013. "Alkali production from bipolar membrane electrodialysis powered by microbial fuel cell and application for biogas upgrading," Applied Energy, Elsevier, vol. 103(C), pages 428-434.
    15. de Arespacochaga, N. & Valderrama, C. & Raich-Montiu, J. & Crest, M. & Mehta, S. & Cortina, J.L., 2015. "Understanding the effects of the origin, occurrence, monitoring, control, fate and removal of siloxanes on the energetic valorization of sewage biogas—A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 52(C), pages 366-381.

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