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Fabrication and characterization of superhydrophobic polypropylene hollow fiber membranes for carbon dioxide absorption

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  • Lv, Yuexia
  • Yu, Xinhai
  • Jia, Jingjing
  • Tu, Shan-Tung
  • Yan, Jinyue
  • Dahlquist, Erik

Abstract

The membrane wetting by amine absorbents results in performance deterioration of membrane gas absorption system for CO2 post-combustion capture. To solve this problem, in this study, the polypropylene membrane fiber was modified by depositing a rough layer on the surface to improve its hydrophobicity. Weighing the coating homogeneity, hydrophobicity and modification process efficiency, the mixture of cyclohexanone and MEK system was considered as the best non-solvent. The contact angle increased dramatically from 122° to 158° by the modification, thereby obtaining superhydrophobic membrane surface. The membrane–absorbent interaction results demonstrated that the modification treatment effectively enhanced the stability and maintained the superhydrophobicity of fibers contacting with the absorbent. In addition, continuous CO2 absorption experiments for up to 20days were carried out in untreated and modified polypropylene hollow fiber membrane contactors, using 1molL−1 MEA solution as the absorbent. The long-term system operation results indicated that, even though additional mass transfer resistance was introduced by the surface coating, the modified polypropylene hollow fiber membrane contactor was still technically feasible for CO2 capture from the power stations.

Suggested Citation

  • Lv, Yuexia & Yu, Xinhai & Jia, Jingjing & Tu, Shan-Tung & Yan, Jinyue & Dahlquist, Erik, 2012. "Fabrication and characterization of superhydrophobic polypropylene hollow fiber membranes for carbon dioxide absorption," Applied Energy, Elsevier, vol. 90(1), pages 167-174.
    • Handle: RePEc:eee:appene:v:90:y:2012:i:1:p:167-174
    DOI: 10.1016/j.apenergy.2010.12.038
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    1. Zhao, Guoying & Aziz, Baroz & Hedin, Niklas, 2010. "Carbon dioxide adsorption on mesoporous silica surfaces containing amine-like motifs," Applied Energy, Elsevier, vol. 87(9), pages 2907-2913, September.
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    1. Ben-Mansour, R. & Habib, M.A. & Bamidele, O.E. & Basha, M. & Qasem, N.A.A. & Peedikakkal, A. & Laoui, T. & Ali, M., 2016. "Carbon capture by physical adsorption: Materials, experimental investigations and numerical modeling and simulations – A review," Applied Energy, Elsevier, vol. 161(C), pages 225-255.
    2. Li, Bingyun & Duan, Yuhua & Luebke, David & Morreale, Bryan, 2013. "Advances in CO2 capture technology: A patent review," Applied Energy, Elsevier, vol. 102(C), pages 1439-1447.
    3. Yang, Jie & Yu, Xinhai & Yan, Jinyue & Tu, Shan-Tung & Dahlquist, Erik, 2013. "Effects of SO2 on CO2 capture using a hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 112(C), pages 755-764.
    4. Dahlquist, Erik & Naqvi, Muhammad & Thorin, Eva & Yan, Jinyue & Kyprianidis, Konstantinos & Hartwell, Philip, 2017. "Experimental and numerical investigation of pellet and black liquor gasification for polygeneration plant," Applied Energy, Elsevier, vol. 204(C), pages 1055-1064.
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    6. Yan, Shuren & Zhu, Ding & Zhang, Zhiyong & Li, Hai & Chen, Guangjin & Liu, Bei, 2019. "A pilot-scale experimental study on CO2 capture using Zeolitic imidazolate framework-8 slurry under normal pressure," Applied Energy, Elsevier, vol. 248(C), pages 104-114.
    7. Lin, Yi-Feng & Chang, Jun-Min & Ye, Qian & Tung, Kuo-Lun, 2015. "Hydrophobic fluorocarbon-modified silica aerogel tubular membranes with excellent CO2 recovery ability in membrane contactors," Applied Energy, Elsevier, vol. 154(C), pages 21-25.
    8. Lv, Yuexia & Yu, Xinhai & Tu, Shan-Tung & Yan, Jinyue & Dahlquist, Erik, 2012. "Experimental studies on simultaneous removal of CO2 and SO2 in a polypropylene hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 97(C), pages 283-288.
    9. Hyun Sic Park & Dongwoan Kang & Jo Hong Kang & Kwanghwi Kim & Jaehyuk Kim & Hojun Song, 2021. "Selective Sulfur Dioxide Absorption from Simulated Flue Gas Using Various Aqueous Alkali Solutions in a Polypropylene Hollow Fiber Membrane Contactor: Removal Efficiency and Use of Sulfur Dioxide," IJERPH, MDPI, vol. 18(2), pages 1-15, January.
    10. Fang, Zhongqiu & Yu, Xiaochen & Tang, Weiqiang & Yu, Xinhai & Zhao, Shuangliang & Tu, Shan-Tung, 2017. "Denitration by oxidation-absorption with polypropylene hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 206(C), pages 858-868.
    11. Ganapathy, Harish & Steinmayer, Sascha & Shooshtari, Amir & Dessiatoun, Serguei & Ohadi, Michael M. & Alshehhi, Mohamed, 2016. "Process intensification characteristics of a microreactor absorber for enhanced CO2 capture," Applied Energy, Elsevier, vol. 162(C), pages 416-427.
    12. Ganapathy, H. & Shooshtari, A. & Dessiatoun, S. & Alshehhi, M. & Ohadi, M., 2014. "Fluid flow and mass transfer characteristics of enhanced CO2 capture in a minichannel reactor," Applied Energy, Elsevier, vol. 119(C), pages 43-56.
    13. Lin, Yi-Feng & Ko, Chia-Chieh & Chen, Chien-Hua & Tung, Kuo-Lun & Chang, Kai-Shiun & Chung, Tsair-Wang, 2014. "Sol–gel preparation of polymethylsilsesquioxane aerogel membranes for CO2 absorption fluxes in membrane contactors," Applied Energy, Elsevier, vol. 129(C), pages 25-31.
    14. Yan, X.H. & Zhao, T.S. & An, L. & Zhao, G. & Zeng, L., 2015. "A crack-free and super-hydrophobic cathode micro-porous layer for direct methanol fuel cells," Applied Energy, Elsevier, vol. 138(C), pages 331-336.
    15. Enbin Liu & Xudong Lu & Daocheng Wang, 2023. "A Systematic Review of Carbon Capture, Utilization and Storage: Status, Progress and Challenges," Energies, MDPI, vol. 16(6), pages 1-48, March.
    16. Ismail Ismail & Vassilis Gaganis, 2023. "Carbon Capture, Utilization, and Storage in Saline Aquifers: Subsurface Policies, Development Plans, Well Control Strategies and Optimization Approaches—A Review," Clean Technol., MDPI, vol. 5(2), pages 1-29, May.

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